Application of Zinc-Based Metal-Organic Framework ZIF-8 on Paper: A Pilot Study on Visual Appearance and Effectiveness

Paper and cellulose-based materials are known for their sensitivity to humidity, which can create stresses among fibres and increase fragility. More importantly, humidity can lead to the formation of mould and stains, compromising both aesthetic value and long-term preservation, particularly for his...

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Vydané v:	Polymers Ročník 17; číslo 10; s. 1369
Hlavní autori:	Balliana, Eleonora, Marchand, Mathilde, Di Matteo, Valentina, Ballarin, Barbara, Cassani, Maria Cristina, Panzavolta, Silvia, Zendri, Elisabetta
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	Switzerland MDPI AG 16.05.2025 MDPI
Predmet:	Antimicrobial agents Bacteria Cellulose Climate change Commercial printing industry Cultural heritage Effectiveness Food packaging Fragility Historic preservation Humidity Infrared analysis Metal industry Metal-organic frameworks Microorganisms Nanomaterials Nanoparticles Physical properties Printing industry Spectrum analysis VOCs Volatile organic compounds X-ray fluorescence X-ray spectroscopy Zeolites Zinc Italy Germany California metal–organic framework ZIF-8 FTIR morphological characterisation paper application XRD XRF
ISSN:	2073-4360, 2073-4360
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Abstract	Paper and cellulose-based materials are known for their sensitivity to humidity, which can create stresses among fibres and increase fragility. More importantly, humidity can lead to the formation of mould and stains, compromising both aesthetic value and long-term preservation, particularly for historical documents and books. This study explored the application of in situ prepared Zeolitic Imidazolate Framework (ZIF-8), a zinc-based MOF, on paper as a potential antimicrobial material. Hand-made and commercially printed papers were tested to assess the effective deposition and formation of the ZIF-8 network, with a focus on both visual appearance and physicochemical characteristics. X-ray fluorescence and diffraction, infrared spectroscopy, and scanning electron microscopy analysis confirmed the successful formation of the ZIF-8 network in all papers. The Zn content varied, as expected, depending on application time and paper characteristics. All treated papers exhibited minor variations in brilliance and showed slightly increased rigidity. The formation of white spots linked to Zn accumulation was observed, particularly in printed books where colourimetric and microscopic variations were more pronounced.
AbstractList	Paper and cellulose-based materials are known for their sensitivity to humidity, which can create stresses among fibres and increase fragility. More importantly, humidity can lead to the formation of mould and stains, compromising both aesthetic value and long-term preservation, particularly for historical documents and books. This study explored the application of in situ prepared Zeolitic Imidazolate Framework (ZIF-8), a zinc-based MOF, on paper as a potential antimicrobial material. Hand-made and commercially printed papers were tested to assess the effective deposition and formation of the ZIF-8 network, with a focus on both visual appearance and physicochemical characteristics. X-ray fluorescence and diffraction, infrared spectroscopy, and scanning electron microscopy analysis confirmed the successful formation of the ZIF-8 network in all papers. The Zn content varied, as expected, depending on application time and paper characteristics. All treated papers exhibited minor variations in brilliance and showed slightly increased rigidity. The formation of white spots linked to Zn accumulation was observed, particularly in printed books where colourimetric and microscopic variations were more pronounced. Paper and cellulose-based materials are known for their sensitivity to humidity, which can create stresses among fibres and increase fragility. More importantly, humidity can lead to the formation of mould and stains, compromising both aesthetic value and long-term preservation, particularly for historical documents and books. This study explored the application of in situ prepared Zeolitic Imidazolate Framework (ZIF-8), a zinc-based MOF, on paper as a potential antimicrobial material. Hand-made and commercially printed papers were tested to assess the effective deposition and formation of the ZIF-8 network, with a focus on both visual appearance and physicochemical characteristics. X-ray fluorescence and diffraction, infrared spectroscopy, and scanning electron microscopy analysis confirmed the successful formation of the ZIF-8 network in all papers. The Zn content varied, as expected, depending on application time and paper characteristics. All treated papers exhibited minor variations in brilliance and showed slightly increased rigidity. The formation of white spots linked to Zn accumulation was observed, particularly in printed books where colourimetric and microscopic variations were more pronounced.Paper and cellulose-based materials are known for their sensitivity to humidity, which can create stresses among fibres and increase fragility. More importantly, humidity can lead to the formation of mould and stains, compromising both aesthetic value and long-term preservation, particularly for historical documents and books. This study explored the application of in situ prepared Zeolitic Imidazolate Framework (ZIF-8), a zinc-based MOF, on paper as a potential antimicrobial material. Hand-made and commercially printed papers were tested to assess the effective deposition and formation of the ZIF-8 network, with a focus on both visual appearance and physicochemical characteristics. X-ray fluorescence and diffraction, infrared spectroscopy, and scanning electron microscopy analysis confirmed the successful formation of the ZIF-8 network in all papers. The Zn content varied, as expected, depending on application time and paper characteristics. All treated papers exhibited minor variations in brilliance and showed slightly increased rigidity. The formation of white spots linked to Zn accumulation was observed, particularly in printed books where colourimetric and microscopic variations were more pronounced.
Audience	Academic
Author	Cassani, Maria Cristina Di Matteo, Valentina Zendri, Elisabetta Ballarin, Barbara Panzavolta, Silvia Balliana, Eleonora Marchand, Mathilde
AuthorAffiliation	2 Department of Industrial Chemistry “Toso Montanari”, University of Bologna, Via Piero Gobetti 85, 40129 Bologna, Italy; valentina.dimatteo5@unibo.it (V.D.M.); barbara.ballarin@unibo.it (B.B.); maria.cassani@unibo.it (M.C.C.) 3 Department of Chemistry “G. Ciamician”, University of Bologna, Via Selmi 2, 40126 Bologna, Italy; silvia.panzavolta@unibo.it 1 Department of Environmental Sciences and Statistics, Ca’ Foscari University Venice, Via Torino 155/b, 30170 Venice, Italy; mathilde22marchand@gmail.com
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Snippet	Paper and cellulose-based materials are known for their sensitivity to humidity, which can create stresses among fibres and increase fragility. More...
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SubjectTerms	Antimicrobial agents Bacteria Cellulose Climate change Commercial printing industry Cultural heritage Effectiveness Food packaging Fragility Historic preservation Humidity Infrared analysis Metal industry Metal-organic frameworks Microorganisms Nanomaterials Nanoparticles Physical properties Printing industry Spectrum analysis VOCs Volatile organic compounds X-ray fluorescence X-ray spectroscopy Zeolites Zinc
Title	Application of Zinc-Based Metal-Organic Framework ZIF-8 on Paper: A Pilot Study on Visual Appearance and Effectiveness
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