Single- or double A-site cations in A3Bi2I9 bismuth perovskites: What is the suitable choice?

Investigations on the effect of single or double A-site cation engineering on the photovoltaic performance of bismuth perovskite-inspired materials (A 3 Bi 2 I 9 ) are rare. Herein, we report novel single- and double-cation based bismuth perovskite-inspired materials developed by (1) completely repl...

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Veröffentlicht in:	Journal of materials research Jg. 36; H. 9; S. 1794 - 1804
Hauptverfasser:	Ünlü, Feray, Kulkarni, Ashish, Lê, Khan, Bohr, Christoph, Bliesener, Andrea, Öz, Seren Dilara, Jena, Ajay Kumar, Ando, Yoichi, Miyasaka, Tsutomu, Kirchartz, Thomas, Mathur, Sanjay
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Cham Springer International Publishing 14.05.2021 Springer Nature B.V
Schlagworte:	Applied and Technical Physics Biomaterials Bismuth Cations Cesium Chemistry and Materials Science Crystal structure Efficiency Energy conversion efficiency Energy gap Engineering Inorganic Chemistry Invited Paper Lithium Materials Engineering Materials research Materials Science Morphology Nanotechnology Perovskites Reduction Rubidium Sodium Thin films Toxicity Energy generation Photovoltaic Perovskites Chemical composition Sustainability Bi
ISSN:	0884-2914, 2044-5326
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Abstract	Investigations on the effect of single or double A-site cation engineering on the photovoltaic performance of bismuth perovskite-inspired materials (A 3 Bi 2 I 9 ) are rare. Herein, we report novel single- and double-cation based bismuth perovskite-inspired materials developed by (1) completely replacing CH 3 NH 3 + (methylammonium, MA + ) in MA 3 Bi 2 I 9 with various organic cations such as CH(NH 2 ) 2 + (formamidinium, FA + ), (CH 3 ) 2 NH 2 + (dimethylammonium, DMA + ), C(NH 2 ) 3 + (guanidinium, GA + ) and inorganic cations such as cesium (Cs + ), rubidium (Rb + ), potassium (K + ), sodium (Na + ) and lithium (Li + ) and (2) partially replacing MA + with Cs + in different stoichiometric ratios. Compared to single-cation based bismuth perovskite devices, the double-cation bismuth perovskite device showed an increment in the device power conversion efficiency (PCE) up to 1.5% crediting to the reduction in the bandgap. This is the first study demonstrating double-cation based bismuth perovskite showing bandgap reduction and increment in device efficiency and opens up the possibilities towards compositional engineering for improved device performance. Graphic Abstract
AbstractList	Investigations on the effect of single or double A-site cation engineering on the photovoltaic performance of bismuth perovskite-inspired materials (A3Bi2I9) are rare. Herein, we report novel single- and double-cation based bismuth perovskite-inspired materials developed by (1) completely replacing CH3NH3+ (methylammonium, MA+) in MA3Bi2I9 with various organic cations such as CH(NH2)2+ (formamidinium, FA+), (CH3)2NH2+ (dimethylammonium, DMA+), C(NH2)3+ (guanidinium, GA+) and inorganic cations such as cesium (Cs+), rubidium (Rb+), potassium (K+), sodium (Na+) and lithium (Li+) and (2) partially replacing MA+ with Cs+ in different stoichiometric ratios. Compared to single-cation based bismuth perovskite devices, the double-cation bismuth perovskite device showed an increment in the device power conversion efficiency (PCE) up to 1.5% crediting to the reduction in the bandgap. This is the first study demonstrating double-cation based bismuth perovskite showing bandgap reduction and increment in device efficiency and opens up the possibilities towards compositional engineering for improved device performance.Graphic Abstract Investigations on the effect of single or double A-site cation engineering on the photovoltaic performance of bismuth perovskite-inspired materials (A 3 Bi 2 I 9 ) are rare. Herein, we report novel single- and double-cation based bismuth perovskite-inspired materials developed by (1) completely replacing CH 3 NH 3 + (methylammonium, MA + ) in MA 3 Bi 2 I 9 with various organic cations such as CH(NH 2 ) 2 + (formamidinium, FA + ), (CH 3 ) 2 NH 2 + (dimethylammonium, DMA + ), C(NH 2 ) 3 + (guanidinium, GA + ) and inorganic cations such as cesium (Cs + ), rubidium (Rb + ), potassium (K + ), sodium (Na + ) and lithium (Li + ) and (2) partially replacing MA + with Cs + in different stoichiometric ratios. Compared to single-cation based bismuth perovskite devices, the double-cation bismuth perovskite device showed an increment in the device power conversion efficiency (PCE) up to 1.5% crediting to the reduction in the bandgap. This is the first study demonstrating double-cation based bismuth perovskite showing bandgap reduction and increment in device efficiency and opens up the possibilities towards compositional engineering for improved device performance. Graphic Abstract
Author	Kirchartz, Thomas Ünlü, Feray Miyasaka, Tsutomu Jena, Ajay Kumar Kulkarni, Ashish Lê, Khan Öz, Seren Dilara Ando, Yoichi Bohr, Christoph Bliesener, Andrea Mathur, Sanjay
Author_xml	– sequence: 1 givenname: Feray surname: Ünlü fullname: Ünlü, Feray organization: Department for Chemistry, Institute of Inorganic Chemistry, University of Cologne – sequence: 2 givenname: Ashish surname: Kulkarni fullname: Kulkarni, Ashish organization: IEK5-Photovoltaics, Forschungszentrum Jülich – sequence: 3 givenname: Khan surname: Lê fullname: Lê, Khan organization: Department for Chemistry, Institute of Inorganic Chemistry, University of Cologne – sequence: 4 givenname: Christoph surname: Bohr fullname: Bohr, Christoph organization: Department for Chemistry, Institute of Inorganic Chemistry, University of Cologne – sequence: 5 givenname: Andrea surname: Bliesener fullname: Bliesener, Andrea organization: Physics Institute II, University of Cologne – sequence: 6 givenname: Seren Dilara surname: Öz fullname: Öz, Seren Dilara organization: Department for Chemistry, Institute of Inorganic Chemistry, University of Cologne – sequence: 7 givenname: Ajay Kumar surname: Jena fullname: Jena, Ajay Kumar organization: Graduate School of Engineering, Toin University of Yokohama – sequence: 8 givenname: Yoichi surname: Ando fullname: Ando, Yoichi organization: Physics Institute II, University of Cologne – sequence: 9 givenname: Tsutomu surname: Miyasaka fullname: Miyasaka, Tsutomu organization: Graduate School of Engineering, Toin University of Yokohama – sequence: 10 givenname: Thomas surname: Kirchartz fullname: Kirchartz, Thomas organization: IEK5-Photovoltaics, Forschungszentrum Jülich, Faculty of Engineering and CENIDE, University of Duisburg-Essen – sequence: 11 givenname: Sanjay surname: Mathur fullname: Mathur, Sanjay email: sanjay.mathur@uni-koeln.de organization: Department for Chemistry, Institute of Inorganic Chemistry, University of Cologne
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SubjectTerms	Applied and Technical Physics Biomaterials Bismuth Cations Cesium Chemistry and Materials Science Crystal structure Efficiency Energy conversion efficiency Energy gap Engineering Inorganic Chemistry Invited Paper Lithium Materials Engineering Materials research Materials Science Morphology Nanotechnology Perovskites Reduction Rubidium Sodium Thin films Toxicity
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Title	Single- or double A-site cations in A3Bi2I9 bismuth perovskites: What is the suitable choice?
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