A Hybrid Supercapacitor based on Porous Carbon and the Metal‐Organic Framework MIL‐100(Fe)

Composite supercapacitor electrodes based on carbon nanotubes, carbon black, and a metal–organic framework with iron(III) coordination centers [MIL‐100(Fe), MIL‐88B(Fe), or MIL‐53(Fe)] were prepared and tested with several aqueous electrolytes. A correlation between hydrated ion size and the electri...

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Veröffentlicht in:	ChemElectroChem Jg. 1; H. 7; S. 1182 - 1188
Hauptverfasser:	Campagnol, Nicolò, Romero‐Vara, Ricardo, Deleu, Willem, Stappers, Linda, Binnemans, Koen, De Vos, Dirk E., Fransaer, Jan
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Weinheim WILEY‐VCH Verlag 15.07.2014 John Wiley & Sons, Inc
Schlagworte:	Aqueous electrolytes Capacitors Carbon Carbon nanotubes Electrodes Electrolytes Energy storage hybrid supercapacitors Metal-organic frameworks nanotubes organic–inorganic hybrid composites Supercapacitors
ISSN:	2196-0216, 2196-0216
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Abstract	Composite supercapacitor electrodes based on carbon nanotubes, carbon black, and a metal–organic framework with iron(III) coordination centers [MIL‐100(Fe), MIL‐88B(Fe), or MIL‐53(Fe)] were prepared and tested with several aqueous electrolytes. A correlation between hydrated ion size and the electric response of the electrodes was found, which sheds light on how these materials work as energy‐storage devices. MIL‐100(Fe) shows the most promising results, and the capacitance obtained with the samples in the solutions used is higher than that of a mixture of carbon and nanotubes in the same solution. Unfortunately, shortcomings due to reductive dissolution still hamper the long‐term cyclability of the electrodes. Charged and ready: Composite supercapacitor electrodes based on metal–organic frameworks and carbon nanotubes are tested with environmentally friendly electrolytes. The energy‐storage mechanism followed by these materials is explored and explained, and promising results are obtained with the electrodes.
AbstractList	Composite supercapacitor electrodes based on carbon nanotubes, carbon black, and a metal–organic framework with iron(III) coordination centers [MIL‐100(Fe), MIL‐88B(Fe), or MIL‐53(Fe)] were prepared and tested with several aqueous electrolytes. A correlation between hydrated ion size and the electric response of the electrodes was found, which sheds light on how these materials work as energy‐storage devices. MIL‐100(Fe) shows the most promising results, and the capacitance obtained with the samples in the solutions used is higher than that of a mixture of carbon and nanotubes in the same solution. Unfortunately, shortcomings due to reductive dissolution still hamper the long‐term cyclability of the electrodes. Composite supercapacitor electrodes based on carbon nanotubes, carbon black, and a metal–organic framework with iron(III) coordination centers [MIL‐100(Fe), MIL‐88B(Fe), or MIL‐53(Fe)] were prepared and tested with several aqueous electrolytes. A correlation between hydrated ion size and the electric response of the electrodes was found, which sheds light on how these materials work as energy‐storage devices. MIL‐100(Fe) shows the most promising results, and the capacitance obtained with the samples in the solutions used is higher than that of a mixture of carbon and nanotubes in the same solution. Unfortunately, shortcomings due to reductive dissolution still hamper the long‐term cyclability of the electrodes. Charged and ready: Composite supercapacitor electrodes based on metal–organic frameworks and carbon nanotubes are tested with environmentally friendly electrolytes. The energy‐storage mechanism followed by these materials is explored and explained, and promising results are obtained with the electrodes. Composite supercapacitor electrodes based on carbon nanotubes, carbon black, and a metal-organic framework with iron(III) coordination centers [MIL-100(Fe), MIL-88B(Fe), or MIL-53(Fe)] were prepared and tested with several aqueous electrolytes. A correlation between hydrated ion size and the electric response of the electrodes was found, which sheds light on how these materials work as energy-storage devices. MIL-100(Fe) shows the most promising results, and the capacitance obtained with the samples in the solutions used is higher than that of a mixture of carbon and nanotubes in the same solution. Unfortunately, shortcomings due to reductive dissolution still hamper the long-term cyclability of the electrodes. Charged and ready: Composite supercapacitor electrodes based on metal-organic frameworks and carbon nanotubes are tested with environmentally friendly electrolytes. The energy-storage mechanism followed by these materials is explored and explained, and promising results are obtained with the electrodes.
Author	De Vos, Dirk E. Fransaer, Jan Campagnol, Nicolò Stappers, Linda Deleu, Willem Romero‐Vara, Ricardo Binnemans, Koen
Author_xml	– sequence: 1 givenname: Nicolò surname: Campagnol fullname: Campagnol, Nicolò – sequence: 2 givenname: Ricardo surname: Romero‐Vara fullname: Romero‐Vara, Ricardo – sequence: 3 givenname: Willem surname: Deleu fullname: Deleu, Willem – sequence: 4 givenname: Linda surname: Stappers fullname: Stappers, Linda – sequence: 5 givenname: Koen surname: Binnemans fullname: Binnemans, Koen – sequence: 6 givenname: Dirk E. surname: De Vos fullname: De Vos, Dirk E. – sequence: 7 givenname: Jan surname: Fransaer fullname: Fransaer, Jan email: Jan.Fransaer@mtm.kuleuven.be
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ContentType	Journal Article
Copyright	Copyright © 2014 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim Copyright © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
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Snippet	Composite supercapacitor electrodes based on carbon nanotubes, carbon black, and a metal–organic framework with iron(III) coordination centers [MIL‐100(Fe),... Composite supercapacitor electrodes based on carbon nanotubes, carbon black, and a metal-organic framework with iron(III) coordination centers [MIL-100(Fe),...
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SubjectTerms	Aqueous electrolytes Capacitors Carbon Carbon nanotubes Electrodes Electrolytes Energy storage hybrid supercapacitors Metal-organic frameworks nanotubes organic–inorganic hybrid composites Supercapacitors
Title	A Hybrid Supercapacitor based on Porous Carbon and the Metal‐Organic Framework MIL‐100(Fe)
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