Intrinsic Catalytic Activity versus Effective Light Usage--A Reply to Professor Kisch's Comments
Breaking the impasse: Earlier this year Maschmeyer and Che outlined an approach for normalizing and comparing the apparent quantum yields (AQY) for hydrogen photogeneration catalyzed by semiconductor powders. In the plot of photocatalyst concentration versus AQY they proposed that the linear region...
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| Published in: | Angewandte Chemie (International ed.) Vol. 49; no. 50; pp. 9590 - 9591 |
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| Main Authors: | , |
| Format: | Journal Article |
| Language: | English |
| Published: |
Weinheim
Wiley-VCH Verlag
10.12.2010
WILEY-VCH Verlag WILEY‐VCH Verlag |
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| ISSN: | 1433-7851, 1521-3773 |
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| Abstract | Breaking the impasse: Earlier this year Maschmeyer and Che outlined an approach for normalizing and comparing the apparent quantum yields (AQY) for hydrogen photogeneration catalyzed by semiconductor powders. In the plot of photocatalyst concentration versus AQY they proposed that the linear region was the most appropriate region for comparison. In his Correspondence Kisch refutes this proposal and states that the area at the onset of the plateau region (B) in a plot of catalyst concentration versus reaction rate is relevant. Maschmeyer and Che explain their rationale and conclude that the discussion has arisen because of different emphases in studying photocatalysis. |
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| AbstractList | Breaking the impasse: Earlier this year Maschmeyer and Che outlined an approach for normalizing and comparing the apparent quantum yields (AQY) for hydrogen photogeneration catalyzed by semiconductor powders. In the plot of photocatalyst concentration versus AQY they proposed that the linear region was the most appropriate region for comparison. In his Correspondence Kisch refutes this proposal and states that the area at the onset of the plateau region (B) in a plot of catalyst concentration versus reaction rate is relevant. Maschmeyer and Che explain their rationale and conclude that the discussion has arisen because of different emphases in studying photocatalysis. |
| Author | Maschmeyer, Thomas Che, Michel |
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| Cites_doi | 10.1002/anie.200903921 10.1351/pac199971020321 10.1021/ie901753k 10.1002/ange.200903921 |
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| References | T. Maschmeyer, M. Che, Angew. Chem. 2010, 122, 1578 A. Salinaro, A. V. Emeline, J. C. Zhao, H. Hidaka, V. K. Ryabchuk, N. Serpone, Pure Appl. Chem. 1999, 71, 321. G. Sagawe, M. L. Satuf, R. J. Brandi, J. P. Muschner, C. Federer, O. M. Alfano, D. Bahnemann and A. E. Cassano, Ind. Eng. Chem. Res. 2010, 49, 6898. Angew. Chem. Int. Ed. 2010, 49, 1536. 2010; 49 1999; 71 2010 2010; 122 49 e_1_2_2_3_3 e_1_2_2_4_2 Maschmeyer T. (e_1_2_2_3_2) 2010; 122 e_1_2_2_5_2 e_1_2_2_6_2 e_1_2_2_1_2 e_1_2_2_2_2 e_1_2_2_7_2 |
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| Title | Intrinsic Catalytic Activity versus Effective Light Usage--A Reply to Professor Kisch's Comments |
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