Selective Bifunctional Catalytic Conversion of Cellulose over Reshaped Ni Particles at the Tip of Carbon Nanofibers

Access to cellulose: Carbon nanofibers grown over Ni supported on γ‐Al2O3 act as efficient catalysts for the one‐pot conversion of cellulose to sugar alcohols, owing to the enhanced accessibility of the water‐insoluble substrate towards the active catalytic sites. The new catalyst design concept yie...

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Vydáno v:	ChemSusChem Ročník 3; číslo 6; s. 698 - 701
Hlavní autoři:	Van de Vyver, Stijn, Geboers, Jan, Dusselier, Michiel, Schepers, Hans, Vosch, Tom, Zhang, Liang, Van Tendeloo, Gustaaf, Jacobs, Pierre A., Sels, Bert F.
Médium:	Journal Article
Jazyk:	angličtina
Vydáno:	Weinheim WILEY-VCH Verlag 21.06.2010 WILEY‐VCH Verlag
Témata:	carbohydrates Carbon Catalysis cellulose Cellulose - chemistry heterogeneous catalysis Nanofibers - chemistry nanostructures nickel Nickel - chemistry Sorbitol - chemical synthesis Sugar Alcohols - chemical synthesis
ISSN:	1864-5631, 1864-564X, 1864-564X
On-line přístup:	Získat plný text
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Abstract	Access to cellulose: Carbon nanofibers grown over Ni supported on γ‐Al2O3 act as efficient catalysts for the one‐pot conversion of cellulose to sugar alcohols, owing to the enhanced accessibility of the water‐insoluble substrate towards the active catalytic sites. The new catalyst design concept yields unprecedented results for selective cellulose conversion using inexpensive Ni catalysts.
AbstractList	Access to cellulose: Carbon nanofibers grown over Ni supported on γ‐Al2O3 act as efficient catalysts for the one‐pot conversion of cellulose to sugar alcohols, owing to the enhanced accessibility of the water‐insoluble substrate towards the active catalytic sites. The new catalyst design concept yields unprecedented results for selective cellulose conversion using inexpensive Ni catalysts.
Author	Sels, Bert F. Schepers, Hans Vosch, Tom Zhang, Liang Geboers, Jan Van Tendeloo, Gustaaf Dusselier, Michiel Van de Vyver, Stijn Jacobs, Pierre A.
Author_xml	– sequence: 1 givenname: Stijn surname: Van de Vyver fullname: Van de Vyver, Stijn organization: Center for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Heverlee (Belgium), Fax: (+32) 1632-1998 – sequence: 2 givenname: Jan surname: Geboers fullname: Geboers, Jan organization: Center for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Heverlee (Belgium), Fax: (+32) 1632-1998 – sequence: 3 givenname: Michiel surname: Dusselier fullname: Dusselier, Michiel organization: Center for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Heverlee (Belgium), Fax: (+32) 1632-1998 – sequence: 4 givenname: Hans surname: Schepers fullname: Schepers, Hans organization: Center for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Heverlee (Belgium), Fax: (+32) 1632-1998 – sequence: 5 givenname: Tom surname: Vosch fullname: Vosch, Tom organization: Department of Chemistry, Katholieke Universiteit Leuven, Celestijnenlaan 200F, 3001 Heverlee (Belgium) – sequence: 6 givenname: Liang surname: Zhang fullname: Zhang, Liang organization: Center for Electron Microscopy for Materials Science, University of Antwerp, Groenenborgerlaan 171, 2020 Antwerp (Belgium) – sequence: 7 givenname: Gustaaf surname: Van Tendeloo fullname: Van Tendeloo, Gustaaf organization: Center for Electron Microscopy for Materials Science, University of Antwerp, Groenenborgerlaan 171, 2020 Antwerp (Belgium) – sequence: 8 givenname: Pierre A. surname: Jacobs fullname: Jacobs, Pierre A. email: bert.sels@biw.kuleuven.be organization: Center for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Heverlee (Belgium), Fax: (+32) 1632-1998 – sequence: 9 givenname: Bert F. surname: Sels fullname: Sels, Bert F. email: pierre.jacobs@biw.kuleuven.be organization: Center for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Heverlee (Belgium), Fax: (+32) 1632-1998
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SubjectTerms	carbohydrates Carbon Catalysis cellulose Cellulose - chemistry heterogeneous catalysis Nanofibers - chemistry nanostructures nickel Nickel - chemistry Sorbitol - chemical synthesis Sugar Alcohols - chemical synthesis
Title	Selective Bifunctional Catalytic Conversion of Cellulose over Reshaped Ni Particles at the Tip of Carbon Nanofibers
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