2,7-Carbazole Derived Organoboron Compounds: Synthesis and Molecular Fluorescence
Triarylboranes have drawn much attention in OLEDs owing to their remarkable solid-state luminescence properties. Here two new A-D-A type compounds, 2,7-bis(dimesitylboryl)-N-ethyl-carbazole (BCz) using triarylborane as electron acceptor and carbazole as electron donor while 2,7-bis((4-(dimesitylbory...
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| Vydáno v: | Frontiers in chemistry Ročník 9; s. 754298 |
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Frontiers Media S.A
22.10.2021
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| Abstract | Triarylboranes have drawn much attention in OLEDs owing to their remarkable solid-state luminescence properties. Here two new A-D-A type compounds, 2,7-bis(dimesitylboryl)-N-ethyl-carbazole (BCz) using triarylborane as electron acceptor and carbazole as electron donor while 2,7-bis((4-(dimesitylboryl)phenyl)ethynyl)-9-ethyl-carbazole (BPACz) using phenylacetylene as extra conjugated bridge, have been synthesized and their photoluminescence related properties in various states have been investigated both experimentally and theoretically. Both compounds show blue emission with high quantum yields, being potential candidates for blue OLED materials. |
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| AbstractList | Triarylboranes have drawn much attention in OLEDs owing to their remarkable solid-state luminescence properties. Here two new A-D-A type compounds, 2,7-bis(dimesitylboryl)-N-ethyl-carbazole (BCz) using triarylborane as electron acceptor and carbazole as electron donor while 2,7-bis((4-(dimesitylboryl)phenyl)ethynyl)-9-ethyl-carbazole (BPACz) using phenylacetylene as extra conjugated bridge, have been synthesized and their photoluminescence related properties in various states have been investigated both experimentally and theoretically. Both compounds show blue emission with high quantum yields, being potential candidates for blue OLED materials. Triarylboranes have drawn much attention in OLEDs owing to their remarkable solid-state luminescence properties. Here two new A-D-A type compounds, 2,7-bis(dimesitylboryl)-N-ethyl-carbazole (BCz) using triarylborane as electron acceptor and carbazole as electron donor while 2,7-bis((4-(dimesitylboryl)phenyl)ethynyl)-9-ethyl-carbazole (BPACz) using phenylacetylene as extra conjugated bridge, have been synthesized and their photoluminescence related properties in various states have been investigated both experimentally and theoretically. Both compounds show blue emission with high quantum yields, being potential candidates for blue OLED materials.Triarylboranes have drawn much attention in OLEDs owing to their remarkable solid-state luminescence properties. Here two new A-D-A type compounds, 2,7-bis(dimesitylboryl)-N-ethyl-carbazole (BCz) using triarylborane as electron acceptor and carbazole as electron donor while 2,7-bis((4-(dimesitylboryl)phenyl)ethynyl)-9-ethyl-carbazole (BPACz) using phenylacetylene as extra conjugated bridge, have been synthesized and their photoluminescence related properties in various states have been investigated both experimentally and theoretically. Both compounds show blue emission with high quantum yields, being potential candidates for blue OLED materials. |
| Author | Zhang, Yufeng Wei, Juan Ji, Lei Tan, Leibo Shi, Junqing Chen, Minhui Wu, Lin Shi, Shanglong |
| AuthorAffiliation | Frontiers Science Center for Flexible Electronics, Xi’an Institute of Flexible Electronics (IFE) and Xi’an Institute of Biomedical Materials and Engineering, Northwestern Polytechnical University, Xi’an , China |
| AuthorAffiliation_xml | – name: Frontiers Science Center for Flexible Electronics, Xi’an Institute of Flexible Electronics (IFE) and Xi’an Institute of Biomedical Materials and Engineering, Northwestern Polytechnical University, Xi’an , China |
| Author_xml | – sequence: 1 givenname: Minhui surname: Chen fullname: Chen, Minhui – sequence: 2 givenname: Juan surname: Wei fullname: Wei, Juan – sequence: 3 givenname: Yufeng surname: Zhang fullname: Zhang, Yufeng – sequence: 4 givenname: Lin surname: Wu fullname: Wu, Lin – sequence: 5 givenname: Leibo surname: Tan fullname: Tan, Leibo – sequence: 6 givenname: Shanglong surname: Shi fullname: Shi, Shanglong – sequence: 7 givenname: Junqing surname: Shi fullname: Shi, Junqing – sequence: 8 givenname: Lei surname: Ji fullname: Ji, Lei |
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| Cites_doi | 10.1039/c2cs35016e 10.1021/cr050966z 10.1039/c6tc01353h 10.1002/chem.200500948 10.1021/ar900072u 10.1016/s0010-8545(06)00151-2 10.1002/anie.202007610 10.1038/nmat2623 10.1002/chem.202005302 10.1002/adma.200801023 10.1002/jcc.22885 10.1002/adom.201700340 10.1021/ja0023332 10.1002/chem.200501096 10.1021/acsami.7b05615 10.1021/ja3048656 10.1063/1.464913 10.1021/jp1057463 10.1021/ja01566a076 10.1016/j.matt.2020.01.023 10.1039/c6sc04245g 10.1021/acs.jpcc.7b08060 10.1103/physrevb.37.785 10.1016/j.tetlet.2016.09.072 10.1002/chem.200900864 10.1002/anie.202016786 10.1063/1.3532844 10.1007/978-1-4615-7658-7 10.1002/adom.201800385 10.1021/cr900401a 10.1016/j.molstruc.2007.03.036 10.1016/s0927-796x(02)00093-1 10.1021/acs.jpcc.8b01579 10.1021/cr100026f 10.3390/molecules22091522 10.1002/anie.200604935 10.1021/ja9817343 |
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| Title | 2,7-Carbazole Derived Organoboron Compounds: Synthesis and Molecular Fluorescence |
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