Direct observation of van der Waals stacking-dependent interlayer magnetism

Controlling the crystal structure is a powerful approach for manipulating the fundamental properties of solids. In van der Waals materials, this control can be achieved by modifying the stacking order through rotation and translation between the layers. Here, we observed stacking-dependent interlaye...

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Vydané v:Science (American Association for the Advancement of Science) Ročník 366; číslo 6468; s. 983
Hlavní autori: Chen, Weijiong, Sun, Zeyuan, Wang, Zhongjie, Gu, Lehua, Xu, Xiaodong, Wu, Shiwei, Gao, Chunlei
Médium: Journal Article
Jazyk:English
Vydavateľské údaje: United States 22.11.2019
ISSN:1095-9203, 1095-9203
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Shrnutí:Controlling the crystal structure is a powerful approach for manipulating the fundamental properties of solids. In van der Waals materials, this control can be achieved by modifying the stacking order through rotation and translation between the layers. Here, we observed stacking-dependent interlayer magnetism in the two-dimensional (2D) magnetic semiconductor chromium tribromide (CrBr ), which was enabled by the successful growth of its monolayer and bilayer through molecular beam epitaxy. Using in situ spin-polarized scanning tunneling microscopy and spectroscopy, we directly correlate the atomic lattice structure with the observed magnetic order. Although the individual monolayer CrBr is ferromagnetic, the interlayer coupling in bilayer depends on the stacking order and can be either ferromagnetic or antiferromagnetic. Our observations pave the way for manipulating 2D magnetism with layer twist angle control.
Bibliografia:ObjectType-Article-1
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ISSN:1095-9203
1095-9203
DOI:10.1126/science.aav1937