Engineering Dual Single‐Atom Sites on 2D Ultrathin N‐doped Carbon Nanosheets Attaining Ultra‐Low‐Temperature Zinc‐Air Battery

Herein, a novel dual single‐atom catalyst comprising adjacent Fe‐N4 and Mn‐N4 sites on 2D ultrathin N‐doped carbon nanosheets with porous structure (FeMn‐DSAC) was constructed as the cathode for a flexible low‐temperature Zn‐air battery (ZAB). FeMn‐DSAC exhibits remarkable bifunctional activities fo...

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Veröffentlicht in:	Angewandte Chemie International Edition Jg. 61; H. 12; S. e202115219 - n/a
Hauptverfasser:	Cui, Tingting, Wang, Yun‐Peng, Ye, Tong, Wu, Jiao, Chen, Zhiqiang, Li, Jiong, Lei, Yongpeng, Wang, Dingsheng, Li, Yadong
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Germany Wiley Subscription Services, Inc 14.03.2022
Ausgabe:	International ed. in English
Schlagworte:	Air temperature Bifunctional electrocatalyst Carbon Catalysts Catalytic activity Chemical reduction Density functional theory Dual single-atom catalyst Low temperature Manganese Mass transfer Metal air batteries Nanosheets Oxygen Oxygen evolution reactions Oxygen reduction reactions Room temperature Specific capacity Zinc Zn-air battery Bifunctional electrocatalyst Nanosheets Zn-air battery Dual single-atom catalyst Low-temperature
ISSN:	1433-7851, 1521-3773, 1521-3773
Online-Zugang:	Volltext
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Abstract	Herein, a novel dual single‐atom catalyst comprising adjacent Fe‐N4 and Mn‐N4 sites on 2D ultrathin N‐doped carbon nanosheets with porous structure (FeMn‐DSAC) was constructed as the cathode for a flexible low‐temperature Zn‐air battery (ZAB). FeMn‐DSAC exhibits remarkable bifunctional activities for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). Control experiments and density functional theory calculations reveal that the catalytic activity arises from the cooperative effect of the Fe/Mn dual‐sites aiding *OOH dissociation as well as the porous 2D nanosheet structure promoting active sits exposure and mass transfer during the reaction process. The excellent bifunctional activity of FeMn‐DSAC enables the ZAB to operate efficiently at ultra‐low temperature of −40 °C, delivering 30 mW cm−2 peak power density and retaining up to 86 % specific capacity from the room temperature counterpart. A Fe/Mn dual single‐atom catalyst with an excellent bifunctional activity is prepared as the cathode for a flexible low‐temperature Zn‐air battery (ZAB). Profiting from the combined Fe/Mn dual‐site effect as well as the porous 2D nanosheet structure, the ZAB could operate efficiently at the ultra‐low temperature of −40 °C.
AbstractList	Herein, a novel dual single-atom catalyst comprising adjacent Fe-N4 and Mn-N4 sites on 2D ultrathin N-doped carbon nanosheets with porous structure (FeMn-DSAC) was constructed as the cathode for a flexible low-temperature Zn-air battery (ZAB). FeMn-DSAC exhibits remarkable bifunctional activities for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). Control experiments and density functional theory calculations reveal that the catalytic activity arises from the cooperative effect of the Fe/Mn dual-sites aiding OOH dissociation as well as the porous 2D nanosheet structure promoting active sits exposure and mass transfer during the reaction process. The excellent bifunctional activity of FeMn-DSAC enables the ZAB to operate efficiently at ultra-low temperature of -40 °C, delivering 30 mW cm-2 peak power density and retaining up to 86 % specific capacity from the room temperature counterpart.Herein, a novel dual single-atom catalyst comprising adjacent Fe-N4 and Mn-N4 sites on 2D ultrathin N-doped carbon nanosheets with porous structure (FeMn-DSAC) was constructed as the cathode for a flexible low-temperature Zn-air battery (ZAB). FeMn-DSAC exhibits remarkable bifunctional activities for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). Control experiments and density functional theory calculations reveal that the catalytic activity arises from the cooperative effect of the Fe/Mn dual-sites aiding OOH dissociation as well as the porous 2D nanosheet structure promoting active sits exposure and mass transfer during the reaction process. The excellent bifunctional activity of FeMn-DSAC enables the ZAB to operate efficiently at ultra-low temperature of -40 °C, delivering 30 mW cm-2 peak power density and retaining up to 86 % specific capacity from the room temperature counterpart. Herein, a novel dual single‐atom catalyst comprising adjacent Fe‐N4 and Mn‐N4 sites on 2D ultrathin N‐doped carbon nanosheets with porous structure (FeMn‐DSAC) was constructed as the cathode for a flexible low‐temperature Zn‐air battery (ZAB). FeMn‐DSAC exhibits remarkable bifunctional activities for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). Control experiments and density functional theory calculations reveal that the catalytic activity arises from the cooperative effect of the Fe/Mn dual‐sites aiding OOH dissociation as well as the porous 2D nanosheet structure promoting active sits exposure and mass transfer during the reaction process. The excellent bifunctional activity of FeMn‐DSAC enables the ZAB to operate efficiently at ultra‐low temperature of −40 °C, delivering 30 mW cm−2 peak power density and retaining up to 86 % specific capacity from the room temperature counterpart. A Fe/Mn dual single‐atom catalyst with an excellent bifunctional activity is prepared as the cathode for a flexible low‐temperature Zn‐air battery (ZAB). Profiting from the combined Fe/Mn dual‐site effect as well as the porous 2D nanosheet structure, the ZAB could operate efficiently at the ultra‐low temperature of −40 °C. Herein, a novel dual single-atom catalyst comprising adjacent Fe-N and Mn-N sites on 2D ultrathin N-doped carbon nanosheets with porous structure (FeMn-DSAC) was constructed as the cathode for a flexible low-temperature Zn-air battery (ZAB). FeMn-DSAC exhibits remarkable bifunctional activities for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). Control experiments and density functional theory calculations reveal that the catalytic activity arises from the cooperative effect of the Fe/Mn dual-sites aiding OOH dissociation as well as the porous 2D nanosheet structure promoting active sits exposure and mass transfer during the reaction process. The excellent bifunctional activity of FeMn-DSAC enables the ZAB to operate efficiently at ultra-low temperature of -40 °C, delivering 30 mW cm peak power density and retaining up to 86 % specific capacity from the room temperature counterpart. Herein, a novel dual single‐atom catalyst comprising adjacent Fe‐N 4 and Mn‐N 4 sites on 2D ultrathin N‐doped carbon nanosheets with porous structure (FeMn‐DSAC) was constructed as the cathode for a flexible low‐temperature Zn‐air battery (ZAB). FeMn‐DSAC exhibits remarkable bifunctional activities for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). Control experiments and density functional theory calculations reveal that the catalytic activity arises from the cooperative effect of the Fe/Mn dual‐sites aiding OOH dissociation as well as the porous 2D nanosheet structure promoting active sits exposure and mass transfer during the reaction process. The excellent bifunctional activity of FeMn‐DSAC enables the ZAB to operate efficiently at ultra‐low temperature of −40 °C, delivering 30 mW cm −2 peak power density and retaining up to 86 % specific capacity from the room temperature counterpart. Herein, a novel dual single‐atom catalyst comprising adjacent Fe‐N4 and Mn‐N4 sites on 2D ultrathin N‐doped carbon nanosheets with porous structure (FeMn‐DSAC) was constructed as the cathode for a flexible low‐temperature Zn‐air battery (ZAB). FeMn‐DSAC exhibits remarkable bifunctional activities for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). Control experiments and density functional theory calculations reveal that the catalytic activity arises from the cooperative effect of the Fe/Mn dual‐sites aiding OOH dissociation as well as the porous 2D nanosheet structure promoting active sits exposure and mass transfer during the reaction process. The excellent bifunctional activity of FeMn‐DSAC enables the ZAB to operate efficiently at ultra‐low temperature of −40 °C, delivering 30 mW cm−2 peak power density and retaining up to 86 % specific capacity from the room temperature counterpart.
Author	Li, Yadong Wu, Jiao Li, Jiong Wang, Dingsheng Lei, Yongpeng Cui, Tingting Wang, Yun‐Peng Ye, Tong Chen, Zhiqiang
Author_xml	– sequence: 1 givenname: Tingting surname: Cui fullname: Cui, Tingting organization: Tsinghua University – sequence: 2 givenname: Yun‐Peng surname: Wang fullname: Wang, Yun‐Peng organization: Central South University – sequence: 3 givenname: Tong surname: Ye fullname: Ye, Tong organization: Central South University – sequence: 4 givenname: Jiao surname: Wu fullname: Wu, Jiao organization: Central South University – sequence: 5 givenname: Zhiqiang surname: Chen fullname: Chen, Zhiqiang organization: Tsinghua University – sequence: 6 givenname: Jiong surname: Li fullname: Li, Jiong organization: Chinese Academy of Science – sequence: 7 givenname: Yongpeng surname: Lei fullname: Lei, Yongpeng email: lypkd@163.com organization: Central South University – sequence: 8 givenname: Dingsheng orcidid: 0000-0003-0074-7633 surname: Wang fullname: Wang, Dingsheng email: wangdingsheng@mail.tsinghua.edu.cn organization: Tsinghua University – sequence: 9 givenname: Yadong surname: Li fullname: Li, Yadong organization: Tsinghua University
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/34994045$$D View this record in MEDLINE/PubMed
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Snippet	Herein, a novel dual single‐atom catalyst comprising adjacent Fe‐N4 and Mn‐N4 sites on 2D ultrathin N‐doped carbon nanosheets with porous structure (FeMn‐DSAC)... Herein, a novel dual single‐atom catalyst comprising adjacent Fe‐N 4 and Mn‐N 4 sites on 2D ultrathin N‐doped carbon nanosheets with porous structure... Herein, a novel dual single-atom catalyst comprising adjacent Fe-N and Mn-N sites on 2D ultrathin N-doped carbon nanosheets with porous structure (FeMn-DSAC)... Herein, a novel dual single-atom catalyst comprising adjacent Fe-N4 and Mn-N4 sites on 2D ultrathin N-doped carbon nanosheets with porous structure (FeMn-DSAC)...
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SubjectTerms	Air temperature Bifunctional electrocatalyst Carbon Catalysts Catalytic activity Chemical reduction Density functional theory Dual single-atom catalyst Low temperature Manganese Mass transfer Metal air batteries Nanosheets Oxygen Oxygen evolution reactions Oxygen reduction reactions Room temperature Specific capacity Zinc Zn-air battery
Title	Engineering Dual Single‐Atom Sites on 2D Ultrathin N‐doped Carbon Nanosheets Attaining Ultra‐Low‐Temperature Zinc‐Air Battery
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