Achieving 37.1% Green Electroluminescent Efficiency and 0.09 eV Full Width at Half Maximum Based on a Ternary Boron‐Oxygen‐Nitrogen Embedded Polycyclic Aromatic System

Herein, a ternary boron‐oxygen‐nitrogen embedded polycyclic aromatic hydrocarbon with multiple resonance thermally activated delayed fluorescence (MR‐TADF), namely DBNO, is developed by adopting the para boron‐π‐boron and para oxygen‐π‐oxygen strategy. The designed molecule presents a vivid green em...

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Published in:	Angewandte Chemie International Edition Vol. 61; no. 23; pp. e202200337 - n/a
Main Authors:	Cai, Xinliang, Xue, Jianan, Li, Chenglong, Liang, Baoyan, Ying, Ao, Tan, Yao, Gong, Shaolong, Wang, Yue
Format:	Journal Article
Language:	English
Published:	WEINHEIM Wiley 07.06.2022 Wiley Subscription Services, Inc
Edition:	International ed. in English
Subjects:	Aromatic hydrocarbons Boron Chemistry Chemistry, Multidisciplinary Dipole moments Electroluminescence Emission spectra Emissions Emitters Light emitting diodes Molecular structure Multiple Resonance Effect Narrowband Narrowband Emission Nitrogen Organic Light-Emitting Diodes Oxygen Photoluminescence Photons Physical Sciences Polycyclic Aromatic Hydrocarbon Quantum efficiency Science & Technology Thermally Activated Delayed fluorescence Thermally Activated Delayed fluorescence LIGHT-EMITTING-DIODES Polycyclic Aromatic Hydrocarbon Narrowband Emission Organic Light-Emitting Diodes Multiple Resonance Effect ACTIVATED DELAYED FLUORESCENCE EMITTERS
ISSN:	1433-7851, 1521-3773, 1521-3773
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Abstract	Herein, a ternary boron‐oxygen‐nitrogen embedded polycyclic aromatic hydrocarbon with multiple resonance thermally activated delayed fluorescence (MR‐TADF), namely DBNO, is developed by adopting the para boron‐π‐boron and para oxygen‐π‐oxygen strategy. The designed molecule presents a vivid green emission with a high photoluminescence quantum yield (96 %) and an extremely narrow full width at half maximum (FWHM) of 19 nm/0.09 eV, which surpasses all previously reported green TADF emitters to date. In addition, the long molecular structure along the transition dipole moment direction endows it with a high horizontal emitting dipole ratio of 96 %. The organic light‐emitting diode (OLED) based on DBNO reveals a narrowband green emission with a peak at 504 nm and a FWHM of 24 nm/0.12 eV. Particularly, a significantly improved device performance is achieved by the TADF‐sensitization (hyperfluorescence) mechanism, presenting a FWHM of 27 nm and a maximum external quantum efficiency (EQE) of 37.1 %. A ternary B−O−N embedded multiple resonance thermally activated delayed fluorescence emitter is developed based on the para B‐π‐B and O‐π‐O strategy. It exhibits a narrowband green emission with a full width at half maximum (FWHM) of 19 nm/0.09 eV and a preferential horizontal dipole ratio of 96 %. The corresponding organic light‐emitting diode (OLED) emits green light with a FWHM of 27 nm and a high external quantum efficiency (EQE) of 37.1 %.
AbstractList	Herein, a ternary boron-oxygen-nitrogen embedded polycyclic aromatic hydrocarbon with multiple resonance thermally activated delayed fluorescence (MR-TADF), namely DBNO, is developed by adopting the para boron-pi-boron and para oxygen-pi-oxygen strategy. The designed molecule presents a vivid green emission with a high photoluminescence quantum yield (96 %) and an extremely narrow full width at half maximum (FWHM) of 19 nm/0.09 eV, which surpasses all previously reported green TADF emitters to date. In addition, the long molecular structure along the transition dipole moment direction endows it with a high horizontal emitting dipole ratio of 96 %. The organic light-emitting diode (OLED) based on DBNO reveals a narrowband green emission with a peak at 504 nm and a FWHM of 24 nm/0.12 eV. Particularly, a significantly improved device performance is achieved by the TADF-sensitization (hyperfluorescence) mechanism, presenting a FWHM of 27 nm and a maximum external quantum efficiency (EQE) of 37.1 %. Herein, a ternary boron‐oxygen‐nitrogen embedded polycyclic aromatic hydrocarbon with multiple resonance thermally activated delayed fluorescence (MR‐TADF), namely DBNO, is developed by adopting the para boron‐π‐boron and para oxygen‐π‐oxygen strategy. The designed molecule presents a vivid green emission with a high photoluminescence quantum yield (96 %) and an extremely narrow full width at half maximum (FWHM) of 19 nm/0.09 eV, which surpasses all previously reported green TADF emitters to date. In addition, the long molecular structure along the transition dipole moment direction endows it with a high horizontal emitting dipole ratio of 96 %. The organic light‐emitting diode (OLED) based on DBNO reveals a narrowband green emission with a peak at 504 nm and a FWHM of 24 nm/0.12 eV. Particularly, a significantly improved device performance is achieved by the TADF‐sensitization (hyperfluorescence) mechanism, presenting a FWHM of 27 nm and a maximum external quantum efficiency (EQE) of 37.1 %. Herein, a ternary boron‐oxygen‐nitrogen embedded polycyclic aromatic hydrocarbon with multiple resonance thermally activated delayed fluorescence (MR‐TADF), namely DBNO, is developed by adopting the para boron‐π‐boron and para oxygen‐π‐oxygen strategy. The designed molecule presents a vivid green emission with a high photoluminescence quantum yield (96 %) and an extremely narrow full width at half maximum (FWHM) of 19 nm/0.09 eV, which surpasses all previously reported green TADF emitters to date. In addition, the long molecular structure along the transition dipole moment direction endows it with a high horizontal emitting dipole ratio of 96 %. The organic light‐emitting diode (OLED) based on DBNO reveals a narrowband green emission with a peak at 504 nm and a FWHM of 24 nm/0.12 eV. Particularly, a significantly improved device performance is achieved by the TADF‐sensitization (hyperfluorescence) mechanism, presenting a FWHM of 27 nm and a maximum external quantum efficiency (EQE) of 37.1 %. Herein, a ternary boron-oxygen-nitrogen embedded polycyclic aromatic hydrocarbon with multiple resonance thermally activated delayed fluorescence (MR-TADF), namely DBNO, is developed by adopting the para boron-π-boron and para oxygen-π-oxygen strategy. The designed molecule presents a vivid green emission with a high photoluminescence quantum yield (96 %) and an extremely narrow full width at half maximum (FWHM) of 19 nm/0.09 eV, which surpasses all previously reported green TADF emitters to date. In addition, the long molecular structure along the transition dipole moment direction endows it with a high horizontal emitting dipole ratio of 96 %. The organic light-emitting diode (OLED) based on DBNO reveals a narrowband green emission with a peak at 504 nm and a FWHM of 24 nm/0.12 eV. Particularly, a significantly improved device performance is achieved by the TADF-sensitization (hyperfluorescence) mechanism, presenting a FWHM of 27 nm and a maximum external quantum efficiency (EQE) of 37.1 %.Herein, a ternary boron-oxygen-nitrogen embedded polycyclic aromatic hydrocarbon with multiple resonance thermally activated delayed fluorescence (MR-TADF), namely DBNO, is developed by adopting the para boron-π-boron and para oxygen-π-oxygen strategy. The designed molecule presents a vivid green emission with a high photoluminescence quantum yield (96 %) and an extremely narrow full width at half maximum (FWHM) of 19 nm/0.09 eV, which surpasses all previously reported green TADF emitters to date. In addition, the long molecular structure along the transition dipole moment direction endows it with a high horizontal emitting dipole ratio of 96 %. The organic light-emitting diode (OLED) based on DBNO reveals a narrowband green emission with a peak at 504 nm and a FWHM of 24 nm/0.12 eV. Particularly, a significantly improved device performance is achieved by the TADF-sensitization (hyperfluorescence) mechanism, presenting a FWHM of 27 nm and a maximum external quantum efficiency (EQE) of 37.1 %. Herein, a ternary boron‐oxygen‐nitrogen embedded polycyclic aromatic hydrocarbon with multiple resonance thermally activated delayed fluorescence (MR‐TADF), namely DBNO, is developed by adopting the para boron‐π‐boron and para oxygen‐π‐oxygen strategy. The designed molecule presents a vivid green emission with a high photoluminescence quantum yield (96 %) and an extremely narrow full width at half maximum (FWHM) of 19 nm/0.09 eV, which surpasses all previously reported green TADF emitters to date. In addition, the long molecular structure along the transition dipole moment direction endows it with a high horizontal emitting dipole ratio of 96 %. The organic light‐emitting diode (OLED) based on DBNO reveals a narrowband green emission with a peak at 504 nm and a FWHM of 24 nm/0.12 eV. Particularly, a significantly improved device performance is achieved by the TADF‐sensitization (hyperfluorescence) mechanism, presenting a FWHM of 27 nm and a maximum external quantum efficiency (EQE) of 37.1 %. A ternary B−O−N embedded multiple resonance thermally activated delayed fluorescence emitter is developed based on the para B‐π‐B and O‐π‐O strategy. It exhibits a narrowband green emission with a full width at half maximum (FWHM) of 19 nm/0.09 eV and a preferential horizontal dipole ratio of 96 %. The corresponding organic light‐emitting diode (OLED) emits green light with a FWHM of 27 nm and a high external quantum efficiency (EQE) of 37.1 %.
ArticleNumber	202200337
Author	Xue, Jianan Liang, Baoyan Ying, Ao Tan, Yao Wang, Yue Gong, Shaolong Cai, Xinliang Li, Chenglong
Author_xml	– sequence: 1 givenname: Xinliang surname: Cai fullname: Cai, Xinliang organization: Jilin University – sequence: 2 givenname: Jianan surname: Xue fullname: Xue, Jianan organization: Jilin University – sequence: 3 givenname: Chenglong orcidid: 0000-0003-2523-6151 surname: Li fullname: Li, Chenglong email: chenglongli@jlu.edu.cn organization: Jilin University – sequence: 4 givenname: Baoyan surname: Liang fullname: Liang, Baoyan email: liangby@jihualab.ac.cn organization: Jihua Laboratory – sequence: 5 givenname: Ao surname: Ying fullname: Ying, Ao organization: Wuhan University – sequence: 6 givenname: Yao surname: Tan fullname: Tan, Yao organization: Wuhan University – sequence: 7 givenname: Shaolong surname: Gong fullname: Gong, Shaolong organization: Wuhan University – sequence: 8 givenname: Yue surname: Wang fullname: Wang, Yue email: yuewang@jlu.edu.cn organization: Jilin University
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/35302704$$D View this record in MEDLINE/PubMed
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Keywords	Thermally Activated Delayed fluorescence LIGHT-EMITTING-DIODES Polycyclic Aromatic Hydrocarbon Narrowband Emission Organic Light-Emitting Diodes Multiple Resonance Effect ACTIVATED DELAYED FLUORESCENCE EMITTERS
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SubjectTerms	Aromatic hydrocarbons Boron Chemistry Chemistry, Multidisciplinary Dipole moments Electroluminescence Emission spectra Emissions Emitters Light emitting diodes Molecular structure Multiple Resonance Effect Narrowband Narrowband Emission Nitrogen Organic Light-Emitting Diodes Oxygen Photoluminescence Photons Physical Sciences Polycyclic Aromatic Hydrocarbon Quantum efficiency Science & Technology Thermally Activated Delayed fluorescence
Title	Achieving 37.1% Green Electroluminescent Efficiency and 0.09 eV Full Width at Half Maximum Based on a Ternary Boron‐Oxygen‐Nitrogen Embedded Polycyclic Aromatic System
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