Influence of ejection temperature on structure and glass transition behavior for Zr-based rapidly quenched disordered alloys

We examined the influence of ejection liquid temperature (Tel) on the structure, thermal stability and crystallization of ZrAlNiCu ribbons prepared by the melt-spinning technique. The increase in Tel was found to cause the formation of an oxide phase on the ribbon surface, more loose atomic configur...

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Published in:	Acta Materialia Vol. 116; pp. 370 - 381
Main Authors:	Wang, X.H., Inoue, A., Kong, F.L., Zhu, S.L., Stoica, M., Kaban, I., Chang, C.T., Shalaan, E., Al-Marzouki, F., Eckert, J.
Format:	Journal Article
Language:	English Japanese
Published:	Elsevier Ltd 01.09.2016 Elsevier BV
Subjects:	Alloys Atomic configuration Atomic structure Crystallization Ejection Ejection liquid temperature Glass transition info:eu-repo/classification/ddc/670 Liquids Melt spinning Rapidly quenched alloys Ribbons Supercooled liquid region Zirconium Glass transition Ejection liquid temperature Atomic configuration Rapidly quenched alloys Supercooled liquid region
ISSN:	1359-6454, 1873-2453
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Abstract	We examined the influence of ejection liquid temperature (Tel) on the structure, thermal stability and crystallization of ZrAlNiCu ribbons prepared by the melt-spinning technique. The increase in Tel was found to cause the formation of an oxide phase on the ribbon surface, more loose atomic configurations, the absence of glass transition (GT) and supercooled liquid (SL) region, and the rise of crystallization temperature. The changes in the GT and SL region occur reversibly by controlling the Tel. Neither the change in alloy composition except oxygen nor the difference in crystallized phases is seen. Their hardness increases significantly by the disappearance of GT and SL region. The reversible changes in the appearance and disappearance of GT and SL region was found for different Zr-based glassy ribbons, being independent of alloy compositions. The disappearance is presumably due to the change in atomic configurations from high-coordinated to less-coordinated atomic packing in the melt-spun ribbons by freezing high-temperature liquid. The observed phenomenon of the reversible changes provides a novel opportunity for deep understanding of mutual correlations among liquid structure, GT, stability of SL and bulk glass-forming ability for metallic alloys. [Display omitted]
AbstractList	We examined the influence of ejection liquid temperature (T el) on the structure, thermal stability and crystallization of Zr-Al-Ni-Cu ribbons prepared by the melt-spinning technique. The increase in T el was found to cause the formation of an oxide phase on the ribbon surface, more loose atomic configurations, the absence of glass transition (GT) and supercooled liquid (SL) region, and the rise of crystallization temperature. The changes in the GT and SL region occur reversibly by controlling the T el. Neither the change in alloy composition except oxygen nor the difference in crystallized phases is seen. Their hardness increases significantly by the disappearance of GT and SL region. The reversible changes in the appearance and disappearance of GT and SL region was found for different Zr-based glassy ribbons, being independent of alloy compositions. The disappearance is presumably due to the change in atomic configurations from high-coordinated to less-coordinated atomic packing in the melt-spun ribbons by freezing high-temperature liquid. The observed phenomenon of the reversible changes provides a novel opportunity for deep understanding of mutual correlations among liquid structure, GT, stability of SL and bulk glass-forming ability for metallic alloys. We examined the influence of ejection liquid temperature (Tel) on the structure, thermal stability and crystallization of ZrAlNiCu ribbons prepared by the melt-spinning technique. The increase in Tel was found to cause the formation of an oxide phase on the ribbon surface, more loose atomic configurations, the absence of glass transition (GT) and supercooled liquid (SL) region, and the rise of crystallization temperature. The changes in the GT and SL region occur reversibly by controlling the Tel. Neither the change in alloy composition except oxygen nor the difference in crystallized phases is seen. Their hardness increases significantly by the disappearance of GT and SL region. The reversible changes in the appearance and disappearance of GT and SL region was found for different Zr-based glassy ribbons, being independent of alloy compositions. The disappearance is presumably due to the change in atomic configurations from high-coordinated to less-coordinated atomic packing in the melt-spun ribbons by freezing high-temperature liquid. The observed phenomenon of the reversible changes provides a novel opportunity for deep understanding of mutual correlations among liquid structure, GT, stability of SL and bulk glass-forming ability for metallic alloys. [Display omitted]
Author	Stoica, M. Wang, X.H. Shalaan, E. Kong, F.L. Chang, C.T. Eckert, J. Inoue, A. Zhu, S.L. Kaban, I. Al-Marzouki, F.
Author_xml	– sequence: 1 givenname: X.H. surname: Wang fullname: Wang, X.H. organization: School of Materials Science and Engineering, Tianjin University, Tianjin, 300072, China – sequence: 2 givenname: A. surname: Inoue fullname: Inoue, A. email: inoue@jiu.ac.jp organization: School of Materials Science and Engineering, Tianjin University, Tianjin, 300072, China – sequence: 3 givenname: F.L. surname: Kong fullname: Kong, F.L. organization: International Institute of Green Materials, Josai International University, Togane, 283-8555, Japan – sequence: 4 givenname: S.L. surname: Zhu fullname: Zhu, S.L. organization: School of Materials Science and Engineering, Tianjin University, Tianjin, 300072, China – sequence: 5 givenname: M. surname: Stoica fullname: Stoica, M. organization: IFW Dresden, Institute for Complex Materials, Helmholtzstr. 20, 01069, Germany – sequence: 6 givenname: I. surname: Kaban fullname: Kaban, I. organization: IFW Dresden, Institute for Complex Materials, Helmholtzstr. 20, 01069, Germany – sequence: 7 givenname: C.T. surname: Chang fullname: Chang, C.T. organization: Ningbo Institute of Materials Technology and Engineering, Ningbo, 315201, China – sequence: 8 givenname: E. surname: Shalaan fullname: Shalaan, E. organization: Department of Physics, King Abdulaziz University, Jeddah, 22254, Saudi Arabia – sequence: 9 givenname: F. surname: Al-Marzouki fullname: Al-Marzouki, F. organization: Department of Physics, King Abdulaziz University, Jeddah, 22254, Saudi Arabia – sequence: 10 givenname: J. surname: Eckert fullname: Eckert, J. organization: Erich Schmid Institute of Materials Science, Austrian Academy of Sciences, Jahnstraβe 12, A-8700, Leoben, Austria
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Keywords	Glass transition Ejection liquid temperature Atomic configuration Rapidly quenched alloys Supercooled liquid region
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Snippet	We examined the influence of ejection liquid temperature (Tel) on the structure, thermal stability and crystallization of ZrAlNiCu ribbons prepared by the... We examined the influence of ejection liquid temperature (T el) on the structure, thermal stability and crystallization of Zr-Al-Ni-Cu ribbons prepared by the...
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SubjectTerms	Alloys Atomic configuration Atomic structure Crystallization Ejection Ejection liquid temperature Glass transition info:eu-repo/classification/ddc/670 Liquids Melt spinning Rapidly quenched alloys Ribbons Supercooled liquid region Zirconium
Title	Influence of ejection temperature on structure and glass transition behavior for Zr-based rapidly quenched disordered alloys
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