A review and perspective on molybdenum-based electrocatalysts for hydrogen evolution reaction

Water electrolysis has been considered as a sustainable way for producing renewable energy of hydrogen. However, this process requires a low-cost and high-efficient hydrogen evolution reaction (HER) catalyst to improve the overall reaction efficiency. Molybdenum (Mo)-based electrocatalysts are regar...

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Published in:	Rare metals Vol. 39; no. 4; pp. 335 - 351
Main Authors:	Hua, Wei, Sun, Huan-Huan, Xu, Fei, Wang, Jian-Gan
Format:	Journal Article
Language:	English
Published:	Beijing Nonferrous Metals Society of China 01.04.2020 Springer Nature B.V
Subjects:	Biomaterials Borides Catalysts Catalytic activity Chemistry and Materials Science Electrocatalysts Electrolysis Energy Hydrogen evolution reaction Hydrogen evolution reactions Hydrogen-based energy Materials Engineering Materials Science Metallic Materials Molybdenum Molybdenum base alloys Molybdenum carbide Molybdenum oxides Molybdenum sulfides Mo‐based materials Nanoscale Science and Technology Phosphides Physical Chemistry Selenides Water splitting Hydrogen evolution reaction Water splitting Electrocatalysts Mo-based materials
ISSN:	1001-0521, 1867-7185
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Abstract	Water electrolysis has been considered as a sustainable way for producing renewable energy of hydrogen. However, this process requires a low-cost and high-efficient hydrogen evolution reaction (HER) catalyst to improve the overall reaction efficiency. Molybdenum (Mo)-based electrocatalysts are regarded as the promising candidates to replace the benchmark but expensive Pt-based HER catalysts, due to their high activity and stability in a wide pH range. In this review, we present a comprehensive and critical summary on the recent progress in the Mo-based electrodes for HER, including molybdenum alloys, molybdenum sulfides, molybdenum selenides, molybdenum carbides, molybdenum phosphides, molybdenum borides, molybdenum nitrides, and molybdenum oxides. Particular attention is mainly focused on the synthetic methods of Mo-based materials, the strategies for increasing the catalytic activity, and the relationship between structure/composition and electrocatalytic performance. Finally, the future development and perspectives of Mo-based electrocatalysts toward high HER performance are proposed. Graphic abstract
AbstractList	Water electrolysis has been considered as a sustainable way for producing renewable energy of hydrogen. However, this process requires a low‐cost and high‐efficient hydrogen evolution reaction (HER) catalyst to improve the overall reaction efficiency. Molybdenum (Mo)‐based electrocatalysts are regarded as the promising candidates to replace the benchmark but expensive Pt‐based HER catalysts, due to their high activity and stability in a wide pH range. In this review, we present a comprehensive and critical summary on the recent progress in the Mo‐based electrodes for HER, including molybdenum alloys, molybdenum sulfides, molybdenum selenides, molybdenum carbides, molybdenum phosphides, molybdenum borides, molybdenum nitrides, and molybdenum oxides. Particular attention is mainly focused on the synthetic methods of Mo‐based materials, the strategies for increasing the catalytic activity, and the relationship between structure/composition and electrocatalytic performance. Finally, the future development and perspectives of Mo‐based electrocatalysts toward high HER performance are proposed. Water electrolysis has been considered as a sustainable way for producing renewable energy of hydrogen. However, this process requires a low-cost and high-efficient hydrogen evolution reaction (HER) catalyst to improve the overall reaction efficiency. Molybdenum (Mo)-based electrocatalysts are regarded as the promising candidates to replace the benchmark but expensive Pt-based HER catalysts, due to their high activity and stability in a wide pH range. In this review, we present a comprehensive and critical summary on the recent progress in the Mo-based electrodes for HER, including molybdenum alloys, molybdenum sulfides, molybdenum selenides, molybdenum carbides, molybdenum phosphides, molybdenum borides, molybdenum nitrides, and molybdenum oxides. Particular attention is mainly focused on the synthetic methods of Mo-based materials, the strategies for increasing the catalytic activity, and the relationship between structure/composition and electrocatalytic performance. Finally, the future development and perspectives of Mo-based electrocatalysts toward high HER performance are proposed.Graphic abstract Water electrolysis has been considered as a sustainable way for producing renewable energy of hydrogen. However, this process requires a low‐cost and high‐efficient hydrogen evolution reaction (HER) catalyst to improve the overall reaction efficiency. Molybdenum (Mo)‐based electrocatalysts are regarded as the promising candidates to replace the benchmark but expensive Pt‐based HER catalysts, due to their high activity and stability in a wide pH range. In this review, we present a comprehensive and critical summary on the recent progress in the Mo‐based electrodes for HER, including molybdenum alloys, molybdenum sulfides, molybdenum selenides, molybdenum carbides, molybdenum phosphides, molybdenum borides, molybdenum nitrides, and molybdenum oxides. Particular attention is mainly focused on the synthetic methods of Mo‐based materials, the strategies for increasing the catalytic activity, and the relationship between structure/composition and electrocatalytic performance. Finally, the future development and perspectives of Mo‐based electrocatalysts toward high HER performance are proposed. Graphic Water electrolysis has been considered as a sustainable way for producing renewable energy of hydrogen. However, this process requires a low-cost and high-efficient hydrogen evolution reaction (HER) catalyst to improve the overall reaction efficiency. Molybdenum (Mo)-based electrocatalysts are regarded as the promising candidates to replace the benchmark but expensive Pt-based HER catalysts, due to their high activity and stability in a wide pH range. In this review, we present a comprehensive and critical summary on the recent progress in the Mo-based electrodes for HER, including molybdenum alloys, molybdenum sulfides, molybdenum selenides, molybdenum carbides, molybdenum phosphides, molybdenum borides, molybdenum nitrides, and molybdenum oxides. Particular attention is mainly focused on the synthetic methods of Mo-based materials, the strategies for increasing the catalytic activity, and the relationship between structure/composition and electrocatalytic performance. Finally, the future development and perspectives of Mo-based electrocatalysts toward high HER performance are proposed. Graphic abstract
Author	Wang, Jian-Gan Hua, Wei Sun, Huan-Huan Xu, Fei
Author_xml	– sequence: 1 givenname: Wei surname: Hua fullname: Hua, Wei organization: State Key Laboratory of Solidification Processing, Center for Nano Energy Materials, School of Materials Science and Engineering, Northwestern Polytechnical University, Shaanxi Joint Laboratory of Graphene (NPU) – sequence: 2 givenname: Huan-Huan surname: Sun fullname: Sun, Huan-Huan organization: State Key Laboratory of Solidification Processing, Center for Nano Energy Materials, School of Materials Science and Engineering, Northwestern Polytechnical University, Shaanxi Joint Laboratory of Graphene (NPU) – sequence: 3 givenname: Fei surname: Xu fullname: Xu, Fei organization: State Key Laboratory of Solidification Processing, Center for Nano Energy Materials, School of Materials Science and Engineering, Northwestern Polytechnical University, Shaanxi Joint Laboratory of Graphene (NPU) – sequence: 4 givenname: Jian-Gan orcidid: 0000-0001-5582-0573 surname: Wang fullname: Wang, Jian-Gan email: wangjiangan@nwpu.edu.cn organization: State Key Laboratory of Solidification Processing, Center for Nano Energy Materials, School of Materials Science and Engineering, Northwestern Polytechnical University, Shaanxi Joint Laboratory of Graphene (NPU)
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Keywords	Hydrogen evolution reaction Water splitting Electrocatalysts Mo-based materials
Language	English
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PublicationCentury	2000
PublicationDate	April 2020
PublicationDateYYYYMMDD	2020-04-01
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PublicationDecade	2020
PublicationPlace	Beijing
PublicationPlace_xml	– name: Beijing
PublicationTitle	Rare metals
PublicationTitleAbbrev	Rare Met
PublicationYear	2020
Publisher	Nonferrous Metals Society of China Springer Nature B.V
Publisher_xml	– name: Nonferrous Metals Society of China – name: Springer Nature B.V
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Snippet	Water electrolysis has been considered as a sustainable way for producing renewable energy of hydrogen. However, this process requires a low-cost and... Water electrolysis has been considered as a sustainable way for producing renewable energy of hydrogen. However, this process requires a low‐cost and...
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SubjectTerms	Biomaterials Borides Catalysts Catalytic activity Chemistry and Materials Science Electrocatalysts Electrolysis Energy Hydrogen evolution reaction Hydrogen evolution reactions Hydrogen-based energy Materials Engineering Materials Science Metallic Materials Molybdenum Molybdenum base alloys Molybdenum carbide Molybdenum oxides Molybdenum sulfides Mo‐based materials Nanoscale Science and Technology Phosphides Physical Chemistry Selenides Water splitting
Title	A review and perspective on molybdenum-based electrocatalysts for hydrogen evolution reaction
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