Apportionment of black carbon in the South Shetland Islands, Antarctic Peninsula

Simultaneous time series measurements of black carbon (BC), aerosol particle number (ANC), radon, and SEM‐EDS analysis for total carbon were collected at the Brazilian Antarctic station Ferraz, northwest of the Antarctic Peninsula (62°05′S, 58°23.5′W) for the years of 1993, 1997, and 1998. A new dat...

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Vydané v:	Journal of Geophysical Research. D. Atmospheres Ročník 111; číslo D3
Hlavní autori:	Pereira, Enio Bueno, Evangelista, Heitor, Pereira, Kely Cristine Dalia, Cavalcanti, Iracema F. A., Setzer, Alberto W.
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	Washington, DC Blackwell Publishing Ltd 16.02.2006 American Geophysical Union
Predmet:	aerosol Antarctica atmospheric pollution biomass burning black carbon Earth sciences Earth, ocean, space Exact sciences and technology radon Brazil Antarctica Scotia Sea South Shetland Islands Scotia Sea Islands Antarctic Peninsula Antarctica, Antarctic Peninsula Antarctica, South Shetland Is South America radon aerosols Soot Wind velocity global Low level jet principal components analysis coupling Winter carbon Spring(season) polar regions particles scanning electron microscopy models Regional scope Time series concentration transport loading Long term contamination new data Shielding effect circulation Antarctic Ocean Vegetation fire
ISSN:	0148-0227, 2156-2202
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Abstract	Simultaneous time series measurements of black carbon (BC), aerosol particle number (ANC), radon, and SEM‐EDS analysis for total carbon were collected at the Brazilian Antarctic station Ferraz, northwest of the Antarctic Peninsula (62°05′S, 58°23.5′W) for the years of 1993, 1997, and 1998. A new data screening technique was applied in an effort to distinguish long‐range from local contaminations of BC. Analyses of data revealed a small increase in BC concentration during winter‐to‐spring seasons. The mean annual BC concentration of 8.3 ng m−3 was consistent with global model estimates for this region. The intermittent coupling mechanism between the regional circulation of the low‐level jets and the passages of the frontal systems explained the transport of BC from areas of burning biomass in Brazil to the northern Antarctic Peninsula. Principal component analysis applied to BC, Radon, ANC, and meteorological data presented significant factor loadings linking BC with 222Rn and with wind velocity corroborating with this hypothesis.
AbstractList	Simultaneous time series measurements of black carbon (BC), aerosol particle number (ANC), radon, and SEM-EDS analysis for total carbon were collected at the Brazilian Antarctic station Ferraz, northwest of the Antarctic Peninsula (62 degree 05'S, 58 degree 23.5'W) for the years of 1993, 1997, and 1998. A new data screening technique was applied in an effort to distinguish long-range from local contaminations of BC. Analyses of data revealed a small increase in BC concentration during winter-to-spring seasons. The mean annual BC concentration of 8.3 ng m super(-3) was consistent with global model estimates for this region. The intermittent coupling mechanism between the regional circulation of the low- level jets and the passages of the frontal systems explained the transport of BC from areas of burning biomass in Brazil to the northern Antarctic Peninsula. Principal component analysis applied to BC, Radon, ANC, and meteorological data presented significant factor loadings linking BC with super(222)Rn and with wind velocity corroborating with this hypothesis. Simultaneous time series measurements of black carbon (BC), aerosol particle number (ANC), radon, and SEM‐EDS analysis for total carbon were collected at the Brazilian Antarctic station Ferraz, northwest of the Antarctic Peninsula (62°05′S, 58°23.5′W) for the years of 1993, 1997, and 1998. A new data screening technique was applied in an effort to distinguish long‐range from local contaminations of BC. Analyses of data revealed a small increase in BC concentration during winter‐to‐spring seasons. The mean annual BC concentration of 8.3 ng m −3 was consistent with global model estimates for this region. The intermittent coupling mechanism between the regional circulation of the low‐level jets and the passages of the frontal systems explained the transport of BC from areas of burning biomass in Brazil to the northern Antarctic Peninsula. Principal component analysis applied to BC, Radon, ANC, and meteorological data presented significant factor loadings linking BC with 222 Rn and with wind velocity corroborating with this hypothesis. Simultaneous time series measurements of black carbon (BC), aerosol particle number (ANC), radon, and SEM-EDS analysis for total carbon were collected at the Brazilian Antarctic station Ferraz, northwest of the Antarctic Peninsula (62'05'S, 58'23.5'W) for the years of 1993, 1997, and 1998. A new data screening technique was applied in an effort to distinguish long-range from local contaminations of BC. Analyses of data revealed a small increase in BC concentration during winter-to-spring seasons. The mean annual BC concentration of 8.3 ng m-3 was consistent with global model estimates for this region. The intermittent coupling mechanism between the regional circulation of the low- level jets and the passages of the frontal systems explained the transport of BC from areas of burning biomass in Brazil to the northern Antarctic Peninsula. Principal component analysis applied to BC, Radon, ANC, and meteorological data presented significant factor loadings linking BC with 222Rn and with wind velocity corroborating with this hypothesis. Simultaneous time series measurements of black carbon (BC), aerosol particle number (ANC), radon, and SEM‐EDS analysis for total carbon were collected at the Brazilian Antarctic station Ferraz, northwest of the Antarctic Peninsula (62°05′S, 58°23.5′W) for the years of 1993, 1997, and 1998. A new data screening technique was applied in an effort to distinguish long‐range from local contaminations of BC. Analyses of data revealed a small increase in BC concentration during winter‐to‐spring seasons. The mean annual BC concentration of 8.3 ng m−3 was consistent with global model estimates for this region. The intermittent coupling mechanism between the regional circulation of the low‐level jets and the passages of the frontal systems explained the transport of BC from areas of burning biomass in Brazil to the northern Antarctic Peninsula. Principal component analysis applied to BC, Radon, ANC, and meteorological data presented significant factor loadings linking BC with 222Rn and with wind velocity corroborating with this hypothesis.
Author	Pereira, Kely Cristine Dalia Cavalcanti, Iracema F. A. Pereira, Enio Bueno Setzer, Alberto W. Evangelista, Heitor
Author_xml	– sequence: 1 givenname: Enio Bueno surname: Pereira fullname: Pereira, Enio Bueno email: eniobp@cptec.inpe.br organization: Center for Weather Forecasts and Climate Studies, National Institute for Space Science, Cachoeira Paulista, São Paulo, Brazil – sequence: 2 givenname: Heitor surname: Evangelista fullname: Evangelista, Heitor organization: Laboratory of Radioecology and Global Change, State University of Rio de Janeiro, Rio de Janeiro, RJ, Brazil – sequence: 3 givenname: Kely Cristine Dalia surname: Pereira fullname: Pereira, Kely Cristine Dalia organization: Laboratory of Radioecology and Global Change, State University of Rio de Janeiro, Rio de Janeiro, RJ, Brazil – sequence: 4 givenname: Iracema F. A. surname: Cavalcanti fullname: Cavalcanti, Iracema F. A. organization: Center for Weather Forecasts and Climate Studies, National Institute for Space Science, Cachoeira Paulista, São Paulo, Brazil – sequence: 5 givenname: Alberto W. surname: Setzer fullname: Setzer, Alberto W. organization: Center for Weather Forecasts and Climate Studies, National Institute for Space Science, Cachoeira Paulista, São Paulo, Brazil
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Snippet	Simultaneous time series measurements of black carbon (BC), aerosol particle number (ANC), radon, and SEM‐EDS analysis for total carbon were collected at the... Simultaneous time series measurements of black carbon (BC), aerosol particle number (ANC), radon, and SEM-EDS analysis for total carbon were collected at the...
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SubjectTerms	aerosol Antarctica atmospheric pollution biomass burning black carbon Earth sciences Earth, ocean, space Exact sciences and technology radon
Title	Apportionment of black carbon in the South Shetland Islands, Antarctic Peninsula
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