Mechanism of visible-light photoisomerization of a rhenium(I) carbonyl-diimine complex

The mechanism of photoisomerization of a Re(I) carbonyl-diimine complex under visible-light irradiation is deciphered by means of ab initio calculations. By highlighting the key role of triplet states as well as spin-orbit and vibronic couplings, we provide a clear picture of this complicated multi-...

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Veröffentlicht in:Chemical communications (Cambridge, England) Jg. 46; H. 43; S. 8225
Hauptverfasser: Gindensperger, Etienne, Köppel, Horst, Daniel, Chantal
Format: Journal Article
Sprache:Englisch
Veröffentlicht: England 21.11.2010
ISSN:1364-548X, 1364-548X
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Zusammenfassung:The mechanism of photoisomerization of a Re(I) carbonyl-diimine complex under visible-light irradiation is deciphered by means of ab initio calculations. By highlighting the key role of triplet states as well as spin-orbit and vibronic couplings, we provide a clear picture of this complicated multi-step process.
Bibliographie:ObjectType-Article-1
SourceType-Scholarly Journals-1
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ISSN:1364-548X
1364-548X
DOI:10.1039/c0cc02661a