Synergistic effect on thermal behavior during co-pyrolysis of lignocellulosic biomass model components blend with bituminous coal

•Co-pyrolysis behavior of lignocellulosic biomass components and bituminous coal was explored.•Positive and/or negative synergistic effects were observed during co-pyrolysis of the mixtures.•Kinetic parameter was solved via using model-free method (Kissinger–Akahira–Sunose).•Nonadditivity performanc...

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Veröffentlicht in:	Bioresource technology Jg. 169; S. 220 - 228
Hauptverfasser:	Wu, Zhiqiang, Wang, Shuzhong, Zhao, Jun, Chen, Lin, Meng, Haiyu
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Kidlington Elsevier Ltd 01.10.2014 Elsevier
Schlagworte:	activation energy Biological and medical sciences Biomass Biotechnology - methods carbon footprint cellulose Cellulose - chemistry Co-pyrolysis Coal Coal - analysis Fundamental and applied biological sciences. Psychology hemicellulose Hot Temperature Kinetics lignin Lignin - chemistry lignocellulose Lignocellulosic biomass Polysaccharides - chemistry prediction pyrolysis synergism Synergistic effect temperature thermal properties Thermogravimetry Co-pyrolysis Synergistic effect Kinetics Lignocellulosic biomass Coal Pyrolysis Thermal behavior Lignocellulosics Biomass Modeling Synergism Mixture Bituminous coal
ISSN:	0960-8524, 1873-2976, 1873-2976
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Abstract	•Co-pyrolysis behavior of lignocellulosic biomass components and bituminous coal was explored.•Positive and/or negative synergistic effects were observed during co-pyrolysis of the mixtures.•Kinetic parameter was solved via using model-free method (Kissinger–Akahira–Sunose).•Nonadditivity performance on the activation energy values of the mixtures was observed. Co-thermochemical conversion of lignocellulosic biomass and coal has been investigated as an effective way to reduce the carbon footprint. Successful evaluating on thermal behavior of the co-pyrolysis is prerequisite for predicting performance and optimizing efficiency of this process. In this paper, pyrolysis and kinetics characteristics of three kinds of lignocellulosic biomass model components (cellulose, hemicellulose, and lignin) blended with a kind of Chinese bituminous coal were explored by thermogravimetric analyzer and Kissinger–Akahira–Sunose method. The results indicated that the addition of model compounds had different synergistic effects on thermal behavior of the bituminous coal. The cellulose showed positive synergistic effects on the thermal decomposition of the coal bituminous coal with lower char yield than calculated value. For hemicellulose and lignin, whether positive or negative synergistic was related to the mixed ratio and temperature range. The distribution of the average activation energy values for the mixtures showed nonadditivity performance.
AbstractList	Co-thermochemical conversion of lignocellulosic biomass and coal has been investigated as an effective way to reduce the carbon footprint. Successful evaluating on thermal behavior of the co-pyrolysis is prerequisite for predicting performance and optimizing efficiency of this process. In this paper, pyrolysis and kinetics characteristics of three kinds of lignocellulosic biomass model components (cellulose, hemicellulose, and lignin) blended with a kind of Chinese bituminous coal were explored by thermogravimetric analyzer and Kissinger-Akahira-Sunose method. The results indicated that the addition of model compounds had different synergistic effects on thermal behavior of the bituminous coal. The cellulose showed positive synergistic effects on the thermal decomposition of the coal bituminous coal with lower char yield than calculated value. For hemicellulose and lignin, whether positive or negative synergistic was related to the mixed ratio and temperature range. The distribution of the average activation energy values for the mixtures showed nonadditivity performance.Co-thermochemical conversion of lignocellulosic biomass and coal has been investigated as an effective way to reduce the carbon footprint. Successful evaluating on thermal behavior of the co-pyrolysis is prerequisite for predicting performance and optimizing efficiency of this process. In this paper, pyrolysis and kinetics characteristics of three kinds of lignocellulosic biomass model components (cellulose, hemicellulose, and lignin) blended with a kind of Chinese bituminous coal were explored by thermogravimetric analyzer and Kissinger-Akahira-Sunose method. The results indicated that the addition of model compounds had different synergistic effects on thermal behavior of the bituminous coal. The cellulose showed positive synergistic effects on the thermal decomposition of the coal bituminous coal with lower char yield than calculated value. For hemicellulose and lignin, whether positive or negative synergistic was related to the mixed ratio and temperature range. The distribution of the average activation energy values for the mixtures showed nonadditivity performance. Co-thermochemical conversion of lignocellulosic biomass and coal has been investigated as an effective way to reduce the carbon footprint. Successful evaluating on thermal behavior of the co-pyrolysis is prerequisite for predicting performance and optimizing efficiency of this process. In this paper, pyrolysis and kinetics characteristics of three kinds of lignocellulosic biomass model components (cellulose, hemicellulose, and lignin) blended with a kind of Chinese bituminous coal were explored by thermogravimetric analyzer and Kissinger–Akahira–Sunose method. The results indicated that the addition of model compounds had different synergistic effects on thermal behavior of the bituminous coal. The cellulose showed positive synergistic effects on the thermal decomposition of the coal bituminous coal with lower char yield than calculated value. For hemicellulose and lignin, whether positive or negative synergistic was related to the mixed ratio and temperature range. The distribution of the average activation energy values for the mixtures showed nonadditivity performance. •Co-pyrolysis behavior of lignocellulosic biomass components and bituminous coal was explored.•Positive and/or negative synergistic effects were observed during co-pyrolysis of the mixtures.•Kinetic parameter was solved via using model-free method (Kissinger–Akahira–Sunose).•Nonadditivity performance on the activation energy values of the mixtures was observed. Co-thermochemical conversion of lignocellulosic biomass and coal has been investigated as an effective way to reduce the carbon footprint. Successful evaluating on thermal behavior of the co-pyrolysis is prerequisite for predicting performance and optimizing efficiency of this process. In this paper, pyrolysis and kinetics characteristics of three kinds of lignocellulosic biomass model components (cellulose, hemicellulose, and lignin) blended with a kind of Chinese bituminous coal were explored by thermogravimetric analyzer and Kissinger–Akahira–Sunose method. The results indicated that the addition of model compounds had different synergistic effects on thermal behavior of the bituminous coal. The cellulose showed positive synergistic effects on the thermal decomposition of the coal bituminous coal with lower char yield than calculated value. For hemicellulose and lignin, whether positive or negative synergistic was related to the mixed ratio and temperature range. The distribution of the average activation energy values for the mixtures showed nonadditivity performance.
Author	Zhao, Jun Meng, Haiyu Wu, Zhiqiang Wang, Shuzhong Chen, Lin
Author_xml	– sequence: 1 givenname: Zhiqiang surname: Wu fullname: Wu, Zhiqiang – sequence: 2 givenname: Shuzhong surname: Wang fullname: Wang, Shuzhong email: szwang@aliyun.com – sequence: 3 givenname: Jun surname: Zhao fullname: Zhao, Jun – sequence: 4 givenname: Lin surname: Chen fullname: Chen, Lin – sequence: 5 givenname: Haiyu surname: Meng fullname: Meng, Haiyu
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Keywords	Co-pyrolysis Synergistic effect Kinetics Lignocellulosic biomass Coal Pyrolysis Thermal behavior Lignocellulosics Biomass Modeling Synergism Mixture Bituminous coal
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Snippet	•Co-pyrolysis behavior of lignocellulosic biomass components and bituminous coal was explored.•Positive and/or negative synergistic effects were observed... Co-thermochemical conversion of lignocellulosic biomass and coal has been investigated as an effective way to reduce the carbon footprint. Successful...
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SubjectTerms	activation energy Biological and medical sciences Biomass Biotechnology - methods carbon footprint cellulose Cellulose - chemistry Co-pyrolysis Coal Coal - analysis Fundamental and applied biological sciences. Psychology hemicellulose Hot Temperature Kinetics lignin Lignin - chemistry lignocellulose Lignocellulosic biomass Polysaccharides - chemistry prediction pyrolysis synergism Synergistic effect temperature thermal properties Thermogravimetry
Title	Synergistic effect on thermal behavior during co-pyrolysis of lignocellulosic biomass model components blend with bituminous coal
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