Modeling photomolecular effect using generalized boundary conditions for Maxwell equations

We recently demonstrated via experiments in hydrogels and at a single air-water interface the photomolecular effect: photons directly cleaving off water molecular clusters in the visible spectrum where bulk water has negligible absorption. To model single interface experiments, here we re-derive gen...

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Vydáno v:	Communications physics Ročník 7; číslo 1; s. 330 - 10
Hlavní autor:	Chen, Gang
Médium:	Journal Article
Jazyk:	angličtina
Vydáno:	London Nature Publishing Group UK 10.10.2024 Nature Publishing Group Nature Portfolio
Témata:	639/624/400/1100 639/766/400/1100 Absorptance Absorption Absorptivity Boundary conditions Electromagnetic fields Maxwell's equations Molecular clusters Parameter modification Photoelectricity Photons Physics Physics and Astronomy Trends Visible spectrum
ISSN:	2399-3650, 2399-3650
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Abstract	We recently demonstrated via experiments in hydrogels and at a single air-water interface the photomolecular effect: photons directly cleaving off water molecular clusters in the visible spectrum where bulk water has negligible absorption. To model single interface experiments, here we re-derive generalized boundary conditions for Maxwell equations by assuming a transition region of the electromagnetic fields across the interface, leading naturally to the Feibelman parameters used before to describe surface photoelectric and surface plasmon effects on metals. This generalization leads to modifications of the Fresnel coefficients and an expression for the surface absorptance that can reasonably explain trends in our single-interface experimental data on the angle and polarization dependence of the beam deflection. Our work provides further support for the existence of the photomolecular effect, suggests that surface absorption should exist in many materials, and lays a foundation for assessing the impacts of such surface absorption based on the Maxwell equations. The newly discovered photomolecular effect reveals that photons can evaporate water clusters in the visible spectrum where bulk water absorbs little. This work generalizes boundary conditions for Maxwell’s equations with Feibelman parameters and presents modified Fresnel coefficients and interfacial absorptance predicting trends consistent with experiments.
AbstractList	Abstract We recently demonstrated via experiments in hydrogels and at a single air-water interface the photomolecular effect: photons directly cleaving off water molecular clusters in the visible spectrum where bulk water has negligible absorption. To model single interface experiments, here we re-derive generalized boundary conditions for Maxwell equations by assuming a transition region of the electromagnetic fields across the interface, leading naturally to the Feibelman parameters used before to describe surface photoelectric and surface plasmon effects on metals. This generalization leads to modifications of the Fresnel coefficients and an expression for the surface absorptance that can reasonably explain trends in our single-interface experimental data on the angle and polarization dependence of the beam deflection. Our work provides further support for the existence of the photomolecular effect, suggests that surface absorption should exist in many materials, and lays a foundation for assessing the impacts of such surface absorption based on the Maxwell equations. We recently demonstrated via experiments in hydrogels and at a single air-water interface the photomolecular effect: photons directly cleaving off water molecular clusters in the visible spectrum where bulk water has negligible absorption. To model single interface experiments, here we re-derive generalized boundary conditions for Maxwell equations by assuming a transition region of the electromagnetic fields across the interface, leading naturally to the Feibelman parameters used before to describe surface photoelectric and surface plasmon effects on metals. This generalization leads to modifications of the Fresnel coefficients and an expression for the surface absorptance that can reasonably explain trends in our single-interface experimental data on the angle and polarization dependence of the beam deflection. Our work provides further support for the existence of the photomolecular effect, suggests that surface absorption should exist in many materials, and lays a foundation for assessing the impacts of such surface absorption based on the Maxwell equations.The newly discovered photomolecular effect reveals that photons can evaporate water clusters in the visible spectrum where bulk water absorbs little. This work generalizes boundary conditions for Maxwell’s equations with Feibelman parameters and presents modified Fresnel coefficients and interfacial absorptance predicting trends consistent with experiments. We recently demonstrated via experiments in hydrogels and at a single air-water interface the photomolecular effect: photons directly cleaving off water molecular clusters in the visible spectrum where bulk water has negligible absorption. To model single interface experiments, here we re-derive generalized boundary conditions for Maxwell equations by assuming a transition region of the electromagnetic fields across the interface, leading naturally to the Feibelman parameters used before to describe surface photoelectric and surface plasmon effects on metals. This generalization leads to modifications of the Fresnel coefficients and an expression for the surface absorptance that can reasonably explain trends in our single-interface experimental data on the angle and polarization dependence of the beam deflection. Our work provides further support for the existence of the photomolecular effect, suggests that surface absorption should exist in many materials, and lays a foundation for assessing the impacts of such surface absorption based on the Maxwell equations. The newly discovered photomolecular effect reveals that photons can evaporate water clusters in the visible spectrum where bulk water absorbs little. This work generalizes boundary conditions for Maxwell’s equations with Feibelman parameters and presents modified Fresnel coefficients and interfacial absorptance predicting trends consistent with experiments.
ArticleNumber	330
Author	Chen, Gang
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Cites_doi	10.1103/PhysRevB.7.3464 10.2307/3578211 10.1103/PhysRevB.34.547 10.1103/PhysRevLett.115.193901 10.1038/s41467-023-38420-w 10.1016/0079-6816(82)90001-6 10.1073/pnas.2312751120 10.7498/aps.70.20211025 10.1143/JJAP.28.L1880 10.1103/PhysRevLett.54.1956 10.1038/s41467-019-13820-z 10.1116/1.580455 10.1038/s41565-018-0097-z 10.1039/C8EE00567B 10.1073/pnas.2320844121 10.1038/s41560-018-0260-7 10.1103/PhysRevB.14.762 10.1016/0039-6028(71)90272-X 10.1038/ncomms5449 10.1002/smll.201401071 10.1016/0039-6028(80)90599-3 10.1002/1521-3773(20010518)40:10<1808::AID-ANIE1808>3.0.CO;2-1 10.1103/PhysRevLett.34.1092 10.1038/s41586-019-1803-1 10.1103/PhysRevB.37.6711 10.1063/1.469505 10.1021/cr040377d 10.1080/00018737800101424 10.1063/1.473820 10.1103/PhysRevB.39.10714 10.1063/1.4945760 10.1007/978-1-4757-5107-9
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Snippet	We recently demonstrated via experiments in hydrogels and at a single air-water interface the photomolecular effect: photons directly cleaving off water... Abstract We recently demonstrated via experiments in hydrogels and at a single air-water interface the photomolecular effect: photons directly cleaving off...
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SubjectTerms	639/624/400/1100 639/766/400/1100 Absorptance Absorption Absorptivity Boundary conditions Electromagnetic fields Maxwell's equations Molecular clusters Parameter modification Photoelectricity Photons Physics Physics and Astronomy Trends Visible spectrum
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Title	Modeling photomolecular effect using generalized boundary conditions for Maxwell equations
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