Impact of mixing state on aerosol optical properties during severe wildfires over the Euro-Mediterranean region

The impact of mixing state of particles from biomass burning on aerosol optical properties (aerosol optical depth (AOD) and single-scattering albedo (SSA)) is studied over the Euro- Mediterranean region during the severe fire event in the Balkans between 20 and 31 July 2007, also characterized by hi...

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Veröffentlicht in:	Atmospheric environment (1994) Jg. 220; S. 117042
Hauptverfasser:	Majdi, Marwa, Kim, Youngseob, Turquety, Solene, Sartelet, Karine
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Elsevier Ltd 01.01.2020 Elsevier
Schlagworte:	Aerosol optical properties aerosols Balkans biomass burning Black carbon carbon Core-shell dust Environmental Engineering Environmental Sciences governmental programs and projects Hydrophilic Hydrophobic hydrophobicity Mediterranean region Mixing state optical properties organic compounds particulates wildfires Mediterranean region Balkans Hydrophilic Mixing state Aerosol optical properties Black carbon Core-shell Hydrophobic hydrophilic hydrophobic black carbon mixing state core-shell
ISSN:	1352-2310, 1873-2844
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Abstract	The impact of mixing state of particles from biomass burning on aerosol optical properties (aerosol optical depth (AOD) and single-scattering albedo (SSA)) is studied over the Euro- Mediterranean region during the severe fire event in the Balkans between 20 and 31 July 2007, also characterized by high dust concentrations. When the mixing state is resolved in chemistry-transport models, chemical compounds are grouped for computational reasons, and internal mixing is assumed within each group. Up to six groups are defined here (dust, black carbon, two inorganic groups and two organic groups). The influence of different grouping assumptions is studied here and compared to the influence of the distribution of black carbon (BC) in particles (“pure homogeneous” representation and “core-shell” one), and the influence of modeling the water absorbed by both inorganic and organic compounds. The comparisons of simulated AODs to observations from the surface network AERONET show that AOD is slightly underestimated when aerosol compounds are assumed to be externally mixed and slightly overestimated when they are assumed to be internally mixed. The mixing state of dust with other compounds, as well as the distribution of BC in particles, strongly influence the optical properties. The impact of the mixing state on AOD is higher than the impact of the distribution of BC in particles, reaching 8–12% on average over the fire regions and 16% in the fire plume. Analysis related to the impact of particle mixing state and BC distribution on SSA shows results similar to AOD. The impact of the mixing state on SSA can reach −8.5% over the fire regions and it is higher than the impact of the BC representation, which is lower than 2%. At the location of fires, water absorbed by inorganics and organics is shown to influence the AOD by about 2%, which is in the lower range of the influence of water on AOD over the region (between 0 and 40%). This low influence of water on AOD during fire is due to assumptions made in the modelling, where most of secondary organic aerosols formed during fires are assumed to be hydrophobic. •Water absorbed by inorganics and organics enhances optical properties.•Mixing-state representation matters more than black-carbon distribution in particles.•The mixing state of dust needs to be considered separately from other compounds.
AbstractList	The impact of mixing state of particles from biomass burning on aerosol optical properties (aerosol optical depth (AOD) and single-scattering albedo (SSA)) is studied over the Euro- Mediterranean region during the severe fire event in the Balkans between 20 and 31 July 2007, also characterized by high dust concentrations. When the mixing state is resolved in chemistry-transport models, chemical compounds are grouped for computational reasons, and internal mixing is assumed within each group. Up to six groups are defined here (dust, black carbon, two inorganic groups and two organic groups). The influence of different grouping assumptions is studied here and compared to the influence of the distribution of black carbon (BC) in particles (“pure homogeneous” representation and “core-shell” one), and the influence of modeling the water absorbed by both inorganic and organic compounds. The comparisons of simulated AODs to observations from the surface network AERONET show that AOD is slightly underestimated when aerosol compounds are assumed to be externally mixed and slightly overestimated when they are assumed to be internally mixed. The mixing state of dust with other compounds, as well as the distribution of BC in particles, strongly influence the optical properties. The impact of the mixing state on AOD is higher than the impact of the distribution of BC in particles, reaching 8–12% on average over the fire regions and 16% in the fire plume. Analysis related to the impact of particle mixing state and BC distribution on SSA shows results similar to AOD. The impact of the mixing state on SSA can reach −8.5% over the fire regions and it is higher than the impact of the BC representation, which is lower than 2%. At the location of fires, water absorbed by inorganics and organics is shown to influence the AOD by about 2%, which is in the lower range of the influence of water on AOD over the region (between 0 and 40%). This low influence of water on AOD during fire is due to assumptions made in the modelling, where most of secondary organic aerosols formed during fires are assumed to be hydrophobic. The impact of mixing state of particles from biomass burning on aerosol optical properties (aerosol optical depth (AOD) and single-scattering albedo (SSA)) is studied over the Euro- Mediterranean region during the severe fire event in the Balkans between 20 and 31 July 2007, also characterized by high dust concentrations. When the mixing state is resolved in chemistry-transport models, chemical compounds are grouped for computational reasons, and internal mixing is assumed within each group. Up to six groups are defined here (dust, black carbon, two inorganic groups and two organic groups). The influence of different grouping assumptions is studied here and compared to the influence of the distribution of black carbon (BC) in particles (“pure homogeneous” representation and “core-shell” one), and the influence of modeling the water absorbed by both inorganic and organic compounds. The comparisons of simulated AODs to observations from the surface network AERONET show that AOD is slightly underestimated when aerosol compounds are assumed to be externally mixed and slightly overestimated when they are assumed to be internally mixed. The mixing state of dust with other compounds, as well as the distribution of BC in particles, strongly influence the optical properties. The impact of the mixing state on AOD is higher than the impact of the distribution of BC in particles, reaching 8–12% on average over the fire regions and 16% in the fire plume. Analysis related to the impact of particle mixing state and BC distribution on SSA shows results similar to AOD. The impact of the mixing state on SSA can reach −8.5% over the fire regions and it is higher than the impact of the BC representation, which is lower than 2%. At the location of fires, water absorbed by inorganics and organics is shown to influence the AOD by about 2%, which is in the lower range of the influence of water on AOD over the region (between 0 and 40%). This low influence of water on AOD during fire is due to assumptions made in the modelling, where most of secondary organic aerosols formed during fires are assumed to be hydrophobic. •Water absorbed by inorganics and organics enhances optical properties.•Mixing-state representation matters more than black-carbon distribution in particles.•The mixing state of dust needs to be considered separately from other compounds. The impact of mixing state of particles from biomass burning on aerosoloptical properties (aerosol optical depth (AOD) and single-scattering albedo(SSA)) is studied over the Euro-Mediterranean region during the severe fireevent in the Balkans between 20 and 31 July 2007, also characterized by high dust concentrations. When the mixing state is resolved in chemistry-transport models, chemical compounds are grouped for computational rea-sons, and internal mixing is assumed within each group. Up to six groupsare de ned here (dust, black carbon, two inorganic groups and two organicgroups). The influence of different grouping assumptions is studied hereand compared to the influence of the distribution of black carbon (BC) in particles (“pure homogeneous” representation and “core-shell” one), and theinfluence of modeling the water absorbed by both inorganic and organiccompounds. The comparisons of simulated AODs to observations from thesurface network AERONET show that AOD is slightly underestimatedwhen aerosol compounds are assumed to be externally mixed and slightly overestimated when they are assumed to be internally mixed. The mixing state of dust with other compounds, as well as the distribution of BC inparticles, strongly influence the optical properties. The impact of themixing state on AOD is higher than the impact of the distribution ofBC in particles, reaching 8-12% on average over the fire regions and16% in the fire plume. Analysis related to the impact of particle mixing state and BC distribution on SSA shows results similar to AOD. Theimpact of the mixing state on SSA can reach -8.5% over the fire regionsand it is higher than the impact of the BC representation, which is lowerthan 2%. At the location of fires, water ab sorbed by inorganics and organics is shown to influence the AOD by about 2%, which is in the lowerrange of the influence of water on AOD over the region (between 0 and40%). This low influence of water on AOD during fire is due toassumptions made in the modelling, where most of secondary organicaerosols formed during fires are assumed to be hydrophobic
ArticleNumber	117042
Author	Turquety, Solene Kim, Youngseob Majdi, Marwa Sartelet, Karine
Author_xml	– sequence: 1 givenname: Marwa surname: Majdi fullname: Majdi, Marwa organization: CEREA: Joint Laboratory École des Ponts ParisTech, EdF R&D, Université Paris-Est, 77455, Champs sur Marne, France – sequence: 2 givenname: Youngseob surname: Kim fullname: Kim, Youngseob organization: CEREA: Joint Laboratory École des Ponts ParisTech, EdF R&D, Université Paris-Est, 77455, Champs sur Marne, France – sequence: 3 givenname: Solene surname: Turquety fullname: Turquety, Solene organization: Laboratoire de Métérologie Dynamique (LMD)-IPSL, Sorbonne Université, CNRS UMR 8539, École Polytechnique, Paris, France – sequence: 4 givenname: Karine orcidid: 0000-0002-8165-2128 surname: Sartelet fullname: Sartelet, Karine email: karine.sartelet@enpc.fr organization: CEREA: Joint Laboratory École des Ponts ParisTech, EdF R&D, Université Paris-Est, 77455, Champs sur Marne, France
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Keywords	Hydrophilic Mixing state Aerosol optical properties Black carbon Core-shell Hydrophobic hydrophilic hydrophobic black carbon mixing state core-shell
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Snippet	The impact of mixing state of particles from biomass burning on aerosol optical properties (aerosol optical depth (AOD) and single-scattering albedo (SSA)) is... The impact of mixing state of particles from biomass burning on aerosoloptical properties (aerosol optical depth (AOD) and single-scattering albedo(SSA)) is...
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SubjectTerms	Aerosol optical properties aerosols Balkans biomass burning Black carbon carbon Core-shell dust Environmental Engineering Environmental Sciences governmental programs and projects Hydrophilic Hydrophobic hydrophobicity Mediterranean region Mixing state optical properties organic compounds particulates wildfires
Title	Impact of mixing state on aerosol optical properties during severe wildfires over the Euro-Mediterranean region
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