Design of the local spin polarization at the organic–ferromagnetic interface

By means of ab initio calculations and spin-polarized scanning tunneling microscopy experiments the creation of a complex energy dependent magnetic structure with a tailored spin-polarized interface is demonstrated. We show this novel effect by adsorbing organic molecules containing π(p(z)) electron...

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Vydáno v:Physical review letters Ročník 105; číslo 6; s. 066601
Hlavní autoři: Atodiresei, Nicolae, Brede, Jens, Lazić, Predrag, Caciuc, Vasile, Hoffmann, Germar, Wiesendanger, Roland, Blügel, Stefan
Médium: Journal Article
Jazyk:angličtina
Vydáno: United States 04.08.2010
ISSN:0031-9007, 1079-7114, 1079-7114
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Popis
Shrnutí:By means of ab initio calculations and spin-polarized scanning tunneling microscopy experiments the creation of a complex energy dependent magnetic structure with a tailored spin-polarized interface is demonstrated. We show this novel effect by adsorbing organic molecules containing π(p(z)) electrons onto a magnetic surface. The hybridization of the out-of-plane p(z) atomic-type orbitals with the d states of the metal leads to the inversion of the spin polarization at the organic site due to a p(z)-d Zener exchange-type mechanism. As a key result, we demonstrate the possibility to selectively and efficiently inject spin-up and spin-down electrons from a ferromagnetic-organic interface, an effect which can be exploited in future spintronic devices.
Bibliografie:ObjectType-Article-1
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ISSN:0031-9007
1079-7114
1079-7114
DOI:10.1103/PhysRevLett.105.066601