Probing the Spin Dimensionality in Single‐Layer CrSBr Van Der Waals Heterostructures by Magneto‐Transport Measurements

2D magnetic materials offer unprecedented opportunities for fundamental and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI3 and Cr2Ge2Te6, the field has expanded to 2D antiferromagnets exhibiting different spin anisotropies and textures. Of particular interest...

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Veröffentlicht in:	Advanced materials (Weinheim) Jg. 34; H. 41; S. e2204940 - n/a
Hauptverfasser:	Boix‐Constant, Carla, Mañas‐Valero, Samuel, Ruiz, Alberto M., Rybakov, Andrey, Konieczny, Krzysztof Aleksander, Pillet, Sébastien, Baldoví, José J., Coronado, Eugenio
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Weinheim Wiley Subscription Services, Inc 01.10.2022 Wiley-VCH Verlag
Schlagworte:	2D magnets 2D materials Anisotropy Antiferromagnetism Bilayers Condensed Matter DFT calculations electrical properties Ferromagnetism Heterostructures Ising model Magnetic materials Magnetic properties Magnetoresistance Magnetoresistivity Magnets Materials science Monolayers Multilayers Physics quantum materials Spintronics Strongly Correlated Electrons Transport properties van der Waals heterostructures van der Waals heterostructures quantum materials 2D magnets electrical properties DFT calculations 2D materials
ISSN:	0935-9648, 1521-4095, 1521-4095
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Abstract	2D magnetic materials offer unprecedented opportunities for fundamental and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI3 and Cr2Ge2Te6, the field has expanded to 2D antiferromagnets exhibiting different spin anisotropies and textures. Of particular interest is the layered metamagnet CrSBr, a relatively air‐stable semiconductor formed by antiferromagnetically‐coupled ferromagnetic layers (Tc∼150 K) that can be exfoliated down to the single‐layer. It presents a complex magnetic behavior with a dynamic magnetic crossover, exhibiting a low‐temperature hidden‐order below T∼40 K. Here, the magneto‐transport properties of CrSBr vertical heterostructures in the 2D limit are inspected. The results demonstrate the marked low‐dimensional character of the ferromagnetic monolayer, with short‐range correlations above Tc and an Ising‐type in‐plane anisotropy, being the spins spontaneously aligned along the easy axis b below Tc. By applying moderate magnetic fields along a and c axes, a spin‐reorientation occurs, leading to a magnetoresistance enhancement below T. In multilayers, a spin‐valve behavior is observed, with negative magnetoresistance strongly enhanced along the three directions below T*. These results show that CrSBr monolayer/bilayer provides an ideal platform for studying and controlling field‐induced phenomena in two‐dimensions, offering new insights regarding 2D magnets and their integration into vertical spintronic devices. The magneto‐transport properties of 2D CrSBr vertical van der Waals heterostructures are inspected, revealing a spontaneous spin alignment along the b‐axis together with spin‐reorientation and field‐induced phases. In multilayers, a spin‐valve behavior is observed with large negative magnetoresistance. This makes CrSBr of high interest not only as a new 2D magnetic model but also as a potential spintronic component.
AbstractList	2D magnetic materials offer unprecedented opportunities for fundamental and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI3 and Cr2Ge2Te6, the field has expanded to 2D antiferromagnets exhibiting different spin anisotropies and textures. Of particular interest is the layered metamagnet CrSBr, a relatively air‐stable semiconductor formed by antiferromagnetically‐coupled ferromagnetic layers (Tc∼150 K) that can be exfoliated down to the single‐layer. It presents a complex magnetic behavior with a dynamic magnetic crossover, exhibiting a low‐temperature hidden‐order below T∼40 K. Here, the magneto‐transport properties of CrSBr vertical heterostructures in the 2D limit are inspected. The results demonstrate the marked low‐dimensional character of the ferromagnetic monolayer, with short‐range correlations above Tc and an Ising‐type in‐plane anisotropy, being the spins spontaneously aligned along the easy axis b below Tc. By applying moderate magnetic fields along a and c axes, a spin‐reorientation occurs, leading to a magnetoresistance enhancement below T. In multilayers, a spin‐valve behavior is observed, with negative magnetoresistance strongly enhanced along the three directions below T. These results show that CrSBr monolayer/bilayer provides an ideal platform for studying and controlling field‐induced phenomena in two‐dimensions, offering new insights regarding 2D magnets and their integration into vertical spintronic devices. The magneto‐transport properties of 2D CrSBr vertical van der Waals heterostructures are inspected, revealing a spontaneous spin alignment along the b‐axis together with spin‐reorientation and field‐induced phases. In multilayers, a spin‐valve behavior is observed with large negative magnetoresistance. This makes CrSBr of high interest not only as a new 2D magnetic model but also as a potential spintronic component. 2D magnetic materials offer unprecedented opportunities for fundamental and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI 3 and Cr 2 Ge 2 Te 6 , the field has expanded to 2D antiferromagnets exhibiting different spin anisotropies and textures. Of particular interest is the layered metamagnet CrSBr, a relatively air‐stable semiconductor formed by antiferromagnetically‐coupled ferromagnetic layers ( T c ∼150 K) that can be exfoliated down to the single‐layer. It presents a complex magnetic behavior with a dynamic magnetic crossover, exhibiting a low‐temperature hidden‐order below T ∼40 K. Here, the magneto‐transport properties of CrSBr vertical heterostructures in the 2D limit are inspected. The results demonstrate the marked low‐dimensional character of the ferromagnetic monolayer, with short‐range correlations above T c and an Ising‐type in‐plane anisotropy, being the spins spontaneously aligned along the easy axis b below T c . By applying moderate magnetic fields along a and c axes, a spin‐reorientation occurs, leading to a magnetoresistance enhancement below T . In multilayers, a spin‐valve behavior is observed, with negative magnetoresistance strongly enhanced along the three directions below T . These results show that CrSBr monolayer/bilayer provides an ideal platform for studying and controlling field‐induced phenomena in two‐dimensions, offering new insights regarding 2D magnets and their integration into vertical spintronic devices. 2D magnetic materials offer unprecedented opportunities for fundamental and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI3 and Cr2 Ge2 Te6 , the field has expanded to 2D antiferromagnets exhibiting different spin anisotropies and textures. Of particular interest is the layered metamagnet CrSBr, a relatively air-stable semiconductor formed by antiferromagnetically-coupled ferromagnetic layers (Tc ∼150 K) that can be exfoliated down to the single-layer. It presents a complex magnetic behavior with a dynamic magnetic crossover, exhibiting a low-temperature hidden-order below T∼40 K. Here, the magneto-transport properties of CrSBr vertical heterostructures in the 2D limit are inspected. The results demonstrate the marked low-dimensional character of the ferromagnetic monolayer, with short-range correlations above Tc and an Ising-type in-plane anisotropy, being the spins spontaneously aligned along the easy axis b below Tc . By applying moderate magnetic fields along a and c axes, a spin-reorientation occurs, leading to a magnetoresistance enhancement below T. In multilayers, a spin-valve behavior is observed, with negative magnetoresistance strongly enhanced along the three directions below T. These results show that CrSBr monolayer/bilayer provides an ideal platform for studying and controlling field-induced phenomena in two-dimensions, offering new insights regarding 2D magnets and their integration into vertical spintronic devices.2D magnetic materials offer unprecedented opportunities for fundamental and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI3 and Cr2 Ge2 Te6 , the field has expanded to 2D antiferromagnets exhibiting different spin anisotropies and textures. Of particular interest is the layered metamagnet CrSBr, a relatively air-stable semiconductor formed by antiferromagnetically-coupled ferromagnetic layers (Tc ∼150 K) that can be exfoliated down to the single-layer. It presents a complex magnetic behavior with a dynamic magnetic crossover, exhibiting a low-temperature hidden-order below T∼40 K. Here, the magneto-transport properties of CrSBr vertical heterostructures in the 2D limit are inspected. The results demonstrate the marked low-dimensional character of the ferromagnetic monolayer, with short-range correlations above Tc and an Ising-type in-plane anisotropy, being the spins spontaneously aligned along the easy axis b below Tc . By applying moderate magnetic fields along a and c axes, a spin-reorientation occurs, leading to a magnetoresistance enhancement below T. In multilayers, a spin-valve behavior is observed, with negative magnetoresistance strongly enhanced along the three directions below T. These results show that CrSBr monolayer/bilayer provides an ideal platform for studying and controlling field-induced phenomena in two-dimensions, offering new insights regarding 2D magnets and their integration into vertical spintronic devices. 2D magnetic materials offer unprecedented opportunities for fundamental and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D CrI3 and Cr2Ge2Te6, the field has expanded to 2D antiferromagnets exhibiting different spin anisotropies and textures. Of particular interest is the layered metamagnet CrSBr, a relatively air‐stable semiconductor formed by antiferromagnetically‐coupled ferromagnetic layers (Tc∼150 K) that can be exfoliated down to the single‐layer. It presents a complex magnetic behavior with a dynamic magnetic crossover, exhibiting a low‐temperature hidden‐order below T∼40 K. Here, the magneto‐transport properties of CrSBr vertical heterostructures in the 2D limit are inspected. The results demonstrate the marked low‐dimensional character of the ferromagnetic monolayer, with short‐range correlations above Tc and an Ising‐type in‐plane anisotropy, being the spins spontaneously aligned along the easy axis b below Tc. By applying moderate magnetic fields along a and c axes, a spin‐reorientation occurs, leading to a magnetoresistance enhancement below T. In multilayers, a spin‐valve behavior is observed, with negative magnetoresistance strongly enhanced along the three directions below T*. These results show that CrSBr monolayer/bilayer provides an ideal platform for studying and controlling field‐induced phenomena in two‐dimensions, offering new insights regarding 2D magnets and their integration into vertical spintronic devices.
Author	Mañas‐Valero, Samuel Boix‐Constant, Carla Ruiz, Alberto M. Coronado, Eugenio Baldoví, José J. Rybakov, Andrey Pillet, Sébastien Konieczny, Krzysztof Aleksander
Author_xml	– sequence: 1 givenname: Carla orcidid: 0000-0003-3213-5906 surname: Boix‐Constant fullname: Boix‐Constant, Carla organization: Universitat de València – sequence: 2 givenname: Samuel orcidid: 0000-0001-6319-9238 surname: Mañas‐Valero fullname: Mañas‐Valero, Samuel email: samuel.manas@uv.es organization: Universitat de València – sequence: 3 givenname: Alberto M. orcidid: 0000-0002-5351-7711 surname: Ruiz fullname: Ruiz, Alberto M. organization: Universitat de València – sequence: 4 givenname: Andrey orcidid: 0000-0002-9924-3576 surname: Rybakov fullname: Rybakov, Andrey organization: Universitat de València – sequence: 5 givenname: Krzysztof Aleksander orcidid: 0000-0003-4618-5154 surname: Konieczny fullname: Konieczny, Krzysztof Aleksander organization: CRM2 – sequence: 6 givenname: Sébastien orcidid: 0000-0003-0530-5244 surname: Pillet fullname: Pillet, Sébastien organization: CRM2 – sequence: 7 givenname: José J. orcidid: 0000-0002-2277-3974 surname: Baldoví fullname: Baldoví, José J. organization: Universitat de València – sequence: 8 givenname: Eugenio orcidid: 0000-0002-1848-8791 surname: Coronado fullname: Coronado, Eugenio email: eugenio.coronado@uv.es organization: Universitat de València
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Snippet	2D magnetic materials offer unprecedented opportunities for fundamental and applied research in spintronics and magnonics. Beyond the pioneering studies on 2D...
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SubjectTerms	2D magnets 2D materials Anisotropy Antiferromagnetism Bilayers Condensed Matter DFT calculations electrical properties Ferromagnetism Heterostructures Ising model Magnetic materials Magnetic properties Magnetoresistance Magnetoresistivity Magnets Materials science Monolayers Multilayers Physics quantum materials Spintronics Strongly Correlated Electrons Transport properties van der Waals heterostructures
Title	Probing the Spin Dimensionality in Single‐Layer CrSBr Van Der Waals Heterostructures by Magneto‐Transport Measurements
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