Self‐Assembly Growth of Twisted Bilayer Graphene on Liquid Cu
Twisted bilayer graphene (tBLG) possesses various novel physical properties. Most of tBLG are fabricated by using artificial methods of stacking or folding single‐layer graphene. Chemical vapor deposition (CVD) has been verified that it holds great potential for preparation of large‐size high‐qualit...
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| Vydané v: | Advanced materials interfaces Ročník 10; číslo 3 |
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| Hlavní autori: | , , , , , , |
| Médium: | Journal Article |
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Weinheim
John Wiley & Sons, Inc
01.01.2023
Wiley-VCH |
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| ISSN: | 2196-7350, 2196-7350 |
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| Abstract | Twisted bilayer graphene (tBLG) possesses various novel physical properties. Most of tBLG are fabricated by using artificial methods of stacking or folding single‐layer graphene. Chemical vapor deposition (CVD) has been verified that it holds great potential for preparation of large‐size high‐quality graphene. Therefore, it is significant for preparing tBLG in situ by using CVD technology. In this work, a novel approach is developed to directly prepare tBLGs on liquid Cu substrate. When the growth temperature exceeds a certain critical value, the state of aligned high‐quality single‐layer graphene domains grown on liquid Cu will be broken. Then, tBLG with twisted double‐layer regions is prepared in situ by rotating and intercalating between graphene domains. Experimental observations suggest that the liquid phase of Cu substrate and gas flow play a crucial role for the formation of tBLGs. These results demonstrate that the liquid Cu is an ideal potential substrate for preparing tBLGs with a full range of twisted angles and studying the formation mechanism of layer‐stacked materials.
Twisted bilayer graphene (tBLG) is prepared by chemical vapor deposition on liquid Cu. When the growth temperature exceeds a certain critical value, the state of aligned high‐quality single‐layer graphene domains grown on liquid Cu is broken. Then, tBLG with twisted double‐layer regions is obtained in situ by rotating and intercalating between graphene domains. |
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| AbstractList | Twisted bilayer graphene (tBLG) possesses various novel physical properties. Most of tBLG are fabricated by using artificial methods of stacking or folding single‐layer graphene. Chemical vapor deposition (CVD) has been verified that it holds great potential for preparation of large‐size high‐quality graphene. Therefore, it is significant for preparing tBLG in situ by using CVD technology. In this work, a novel approach is developed to directly prepare tBLGs on liquid Cu substrate. When the growth temperature exceeds a certain critical value, the state of aligned high‐quality single‐layer graphene domains grown on liquid Cu will be broken. Then, tBLG with twisted double‐layer regions is prepared in situ by rotating and intercalating between graphene domains. Experimental observations suggest that the liquid phase of Cu substrate and gas flow play a crucial role for the formation of tBLGs. These results demonstrate that the liquid Cu is an ideal potential substrate for preparing tBLGs with a full range of twisted angles and studying the formation mechanism of layer‐stacked materials.
Twisted bilayer graphene (tBLG) is prepared by chemical vapor deposition on liquid Cu. When the growth temperature exceeds a certain critical value, the state of aligned high‐quality single‐layer graphene domains grown on liquid Cu is broken. Then, tBLG with twisted double‐layer regions is obtained in situ by rotating and intercalating between graphene domains. Abstract Twisted bilayer graphene (tBLG) possesses various novel physical properties. Most of tBLG are fabricated by using artificial methods of stacking or folding single‐layer graphene. Chemical vapor deposition (CVD) has been verified that it holds great potential for preparation of large‐size high‐quality graphene. Therefore, it is significant for preparing tBLG in situ by using CVD technology. In this work, a novel approach is developed to directly prepare tBLGs on liquid Cu substrate. When the growth temperature exceeds a certain critical value, the state of aligned high‐quality single‐layer graphene domains grown on liquid Cu will be broken. Then, tBLG with twisted double‐layer regions is prepared in situ by rotating and intercalating between graphene domains. Experimental observations suggest that the liquid phase of Cu substrate and gas flow play a crucial role for the formation of tBLGs. These results demonstrate that the liquid Cu is an ideal potential substrate for preparing tBLGs with a full range of twisted angles and studying the formation mechanism of layer‐stacked materials. Twisted bilayer graphene (tBLG) possesses various novel physical properties. Most of tBLG are fabricated by using artificial methods of stacking or folding single‐layer graphene. Chemical vapor deposition (CVD) has been verified that it holds great potential for preparation of large‐size high‐quality graphene. Therefore, it is significant for preparing tBLG in situ by using CVD technology. In this work, a novel approach is developed to directly prepare tBLGs on liquid Cu substrate. When the growth temperature exceeds a certain critical value, the state of aligned high‐quality single‐layer graphene domains grown on liquid Cu will be broken. Then, tBLG with twisted double‐layer regions is prepared in situ by rotating and intercalating between graphene domains. Experimental observations suggest that the liquid phase of Cu substrate and gas flow play a crucial role for the formation of tBLGs. These results demonstrate that the liquid Cu is an ideal potential substrate for preparing tBLGs with a full range of twisted angles and studying the formation mechanism of layer‐stacked materials. |
| Author | Wang, Liping Li, Dong Yu, Gui Liu, Shan Liu, Mengya Xue, Xudong Zhou, Xiahong |
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| Snippet | Twisted bilayer graphene (tBLG) possesses various novel physical properties. Most of tBLG are fabricated by using artificial methods of stacking or folding... Abstract Twisted bilayer graphene (tBLG) possesses various novel physical properties. Most of tBLG are fabricated by using artificial methods of stacking or... |
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| SubjectTerms | Bilayers Chemical vapor deposition Domains Gas flow Graphene liquid Cu substrate Liquid phases Physical properties self‐intercalation Substrates twisted bilayer graphene |
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| Title | Self‐Assembly Growth of Twisted Bilayer Graphene on Liquid Cu |
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