On the interplay between charge, spin and structural dynamics in transition metal complexes
This perspective presents some recent results concerning ultrafast intramolecular relaxation processes in metal-based molecular complexes. Ultrafast electronic/vibrational relaxation at sub-vibrational time scales, ultrafast intersystem crossing processes and ultrafast structure changes are discusse...
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| Veröffentlicht in: | Dalton transactions : an international journal of inorganic chemistry Jg. 41; H. 42; S. 13022 |
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| 1. Verfasser: | |
| Format: | Journal Article |
| Sprache: | Englisch |
| Veröffentlicht: |
England
14.11.2012
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| ISSN: | 1477-9234, 1477-9234 |
| Online-Zugang: | Weitere Angaben |
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| Zusammenfassung: | This perspective presents some recent results concerning ultrafast intramolecular relaxation processes in metal-based molecular complexes. Ultrafast electronic/vibrational relaxation at sub-vibrational time scales, ultrafast intersystem crossing processes and ultrafast structure changes are discussed, stressing the questions that still need to be solved in order to arrive at a rationale that describes these processes. We will also discuss some new techniques, based on core-level spectroscopies that can provide new insights into the ultrafast intramolecular relaxation in these systems. |
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| Bibliographie: | ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
| ISSN: | 1477-9234 1477-9234 |
| DOI: | 10.1039/c2dt30764b |