Techno‐Economic Analysis of Methane Pyrolysis in Molten Metals: Decarbonizing Natural Gas

Methane pyrolysis using a molten metal process to produce hydrogen is compared to steam methane reforming (SMR) for the industrial production of hydrogen. Capital and operating cost models for pyrolysis and SMR were used to generate cash‐flow and production costs for several different molten pyrolys...

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Veröffentlicht in:	Chemical engineering & technology Jg. 40; H. 6; S. 1022 - 1030
Hauptverfasser:	Parkinson, Brett, Matthews, Joshua W., McConnaughy, Thomas B., Upham, D. Chester, McFarland, Eric W.
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Frankfurt Wiley Subscription Services, Inc 01.06.2017 Wiley Blackwell (John Wiley & Sons)
Schlagworte:	Carbon Carbon dioxide Carbon tax Catalysis Cost engineering Economic analysis Hydrogen production Industrial engineering Liquid metals Manufacturing engineering Methane Methane pyrolysis Natural gas Natural gas conversion Production costs Pyrolysis Reforming Steam methane reforming Taxes
ISSN:	0930-7516, 1521-4125
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Abstract	Methane pyrolysis using a molten metal process to produce hydrogen is compared to steam methane reforming (SMR) for the industrial production of hydrogen. Capital and operating cost models for pyrolysis and SMR were used to generate cash‐flow and production costs for several different molten pyrolysis systems. The economics were most sensitive to the methane conversion and the value obtained for the solid carbon by‐product. The pyrolysis system at 1500 °C is competitive with a carbon tax of $78 t−1; however, if a catalytic process at 1000 °C were developed using a conventional fired heater, it would be competitive with SMR without a carbon dioxide cost penalty. Several pyrolysis alternatives become competitive with increasing carbon dioxide taxes. Methane pyrolysis using a molten metal‐based process to produce carbon and hydrogen is compared to steam methane reforming for the industrial production of hydrogen. Capital and operating cost models for pyrolysis and steam methane reforming were applied to generate cash‐flow and production costs for several different pyrolysis systems making use of molten metals.
AbstractList	Methane pyrolysis using a molten metal process to produce hydrogen is compared to steam methane reforming (SMR) for the industrial production of hydrogen. Capital and operating cost models for pyrolysis and SMR were used to generate cash‐flow and production costs for several different molten pyrolysis systems. The economics were most sensitive to the methane conversion and the value obtained for the solid carbon by‐product. The pyrolysis system at 1500 °C is competitive with a carbon tax of $78 t −1 ; however, if a catalytic process at 1000 °C were developed using a conventional fired heater, it would be competitive with SMR without a carbon dioxide cost penalty. Several pyrolysis alternatives become competitive with increasing carbon dioxide taxes. Methane pyrolysis using a molten metal process to produce hydrogen is compared to steam methane reforming (SMR) for the industrial production of hydrogen. Capital and operating cost models for pyrolysis and SMR were used to generate cash‐flow and production costs for several different molten pyrolysis systems. The economics were most sensitive to the methane conversion and the value obtained for the solid carbon by‐product. The pyrolysis system at 1500 °C is competitive with a carbon tax of $78 t−1; however, if a catalytic process at 1000 °C were developed using a conventional fired heater, it would be competitive with SMR without a carbon dioxide cost penalty. Several pyrolysis alternatives become competitive with increasing carbon dioxide taxes. Methane pyrolysis using a molten metal‐based process to produce carbon and hydrogen is compared to steam methane reforming for the industrial production of hydrogen. Capital and operating cost models for pyrolysis and steam methane reforming were applied to generate cash‐flow and production costs for several different pyrolysis systems making use of molten metals. Methane pyrolysis using a molten metal process to produce hydrogen is compared to steam methane reforming (SMR) for the industrial production of hydrogen. Capital and operating cost models for pyrolysis and SMR were used to generate cash-flow and production costs for several different molten pyrolysis systems. The economics were most sensitive to the methane conversion and the value obtained for the solid carbon by-product. The pyrolysis system at 1500°C is competitive with a carbon tax of $78t-1; however, if a catalytic process at 1000°C were developed using a conventional fired heater, it would be competitive with SMR without a carbon dioxide cost penalty. Several pyrolysis alternatives become competitive with increasing carbon dioxide taxes.
Author	Matthews, Joshua W. Upham, D. Chester McFarland, Eric W. Parkinson, Brett McConnaughy, Thomas B.
Author_xml	– sequence: 1 givenname: Brett surname: Parkinson fullname: Parkinson, Brett organization: University of Queensland – sequence: 2 givenname: Joshua W. surname: Matthews fullname: Matthews, Joshua W. organization: Loughborough University – sequence: 3 givenname: Thomas B. surname: McConnaughy fullname: McConnaughy, Thomas B. organization: University of Queensland – sequence: 4 givenname: D. Chester surname: Upham fullname: Upham, D. Chester organization: University of California – sequence: 5 givenname: Eric W. surname: McFarland fullname: McFarland, Eric W. email: ewmcfar@engineering.ucsb.edu organization: University of California
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Snippet	Methane pyrolysis using a molten metal process to produce hydrogen is compared to steam methane reforming (SMR) for the industrial production of hydrogen....
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SubjectTerms	Carbon Carbon dioxide Carbon tax Catalysis Cost engineering Economic analysis Hydrogen production Industrial engineering Liquid metals Manufacturing engineering Methane Methane pyrolysis Natural gas Natural gas conversion Production costs Pyrolysis Reforming Steam methane reforming Taxes
Title	Techno‐Economic Analysis of Methane Pyrolysis in Molten Metals: Decarbonizing Natural Gas
URI	https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fceat.201600414 https://www.proquest.com/docview/1920460129 https://www.osti.gov/biblio/1400609
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