All ‘green’ composites comprising flax fibres and humins' resins
The use of all “green” composite materials is a great environmental option for several applications such as construction or automotive. A new type of all green composites has been prepared by compression moulding flax fibres with humins as the matrix. Humins are macromolecular heterogeneous furanic...
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| Vydáno v: | Composites science and technology Ročník 171; s. 70 - 77 |
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| Hlavní autoři: | , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
| Vydáno: |
Barking
Elsevier Ltd
08.02.2019
Elsevier BV Elsevier |
| Témata: | |
| ISSN: | 0266-3538, 1879-1050 |
| On-line přístup: | Získat plný text |
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| Abstract | The use of all “green” composite materials is a great environmental option for several applications such as construction or automotive. A new type of all green composites has been prepared by compression moulding flax fibres with humins as the matrix. Humins are macromolecular heterogeneous furanic co-products from biorefinery operations. For the first time the potential of humins as a whole thermoset-like matrix in combination with natural fibres was studied. The raw industrial humins were cross-linked with and without catalyst. The effect of the process conditions on the final properties of the composites was studied. Good tensile properties were measured by tensile test and Dynamic Mechanical Analysis. Observations of the fracture surface were done by Scanning Electron Microscope, revealing a void-free morphology. The study finally focused on the water absorption behaviour, underlining the more hydrophobic nature of the humins' composites compared to the raw flax mat. The good adhesion between the fibre and the matrix was underlined. Humins interacts with the hydrophilic fibres thus creating a good interphase, leading to improved properties. The study demonstrated the possibility of using a biorefinery co-product as a thermoset matrix for preparing composites materials. |
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| AbstractList | The use of all “green” composite materials is a great environmental option for several applications such as construction or automotive. A new type of all green composites has been prepared by compression moulding flax fibres with humins as the matrix. Humins are macromolecular heterogeneous furanic co-products from biorefinery operations. For the first time the potential of humins as a whole thermoset-like matrix in combination with natural fibres was studied. The raw industrial humins were cross-linked with and without catalyst. The effect of the process conditions on the final properties of the composites was studied. Good tensile properties were measured by tensile test and Dynamic Mechanical Analysis. Observations of the fracture surface were done by Scanning Electron Microscope, revealing a void-free morphology. The study finally focused on the water absorption behaviour, underlining the more hydrophobic nature of the humins' composites compared to the raw flax mat. The good adhesion between the fibre and the matrix was underlined. Humins interacts with the hydrophilic fibres thus creating a good interphase, leading to improved properties. The study demonstrated the possibility of using a biorefinery co-product as a thermoset matrix for preparing composites materials. |
| Author | Sbirrazzuoli, Nicolas Sangregorio, Anna Guigo, Nathanael van der Waal, Jan C. |
| Author_xml | – sequence: 1 givenname: Anna surname: Sangregorio fullname: Sangregorio, Anna organization: Avantium Chemicals B.V., Zekeringstraat 29, 1014 BV, Amsterdam, the Netherlands – sequence: 2 givenname: Nathanael surname: Guigo fullname: Guigo, Nathanael email: nathanael.guigo@unice.fr organization: Université Côte d'Azur, Institut de Chimie de Nice, CNRS, UMR 7272, 06108, Nice, France – sequence: 3 givenname: Jan C. surname: van der Waal fullname: van der Waal, Jan C. organization: Avantium Chemicals B.V., Zekeringstraat 29, 1014 BV, Amsterdam, the Netherlands – sequence: 4 givenname: Nicolas surname: Sbirrazzuoli fullname: Sbirrazzuoli, Nicolas organization: Université Côte d'Azur, Institut de Chimie de Nice, CNRS, UMR 7272, 06108, Nice, France |
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| Keywords | Curing (B) Scanning electron microscopy (D) Fibres (A) Thermomechanical properties (B) Biocomposites |
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| SubjectTerms | Automobile industry Automotive engineering Biocomposites Chemical Sciences Composite materials Crosslinking Curing Curing (B) Dynamic mechanical analysis Fibers Fibres (A) Flax Fracture surfaces Material chemistry Mechanical properties Morphology Polymer matrix composites Pressure molding Refining Scanning electron microscopy Scanning electron microscopy (D) Tensile properties Tensile strength Tensile tests Thermomechanical properties (B) Thermosetting resins Water absorption |
| Title | All ‘green’ composites comprising flax fibres and humins' resins |
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