All ‘green’ composites comprising flax fibres and humins' resins

The use of all “green” composite materials is a great environmental option for several applications such as construction or automotive. A new type of all green composites has been prepared by compression moulding flax fibres with humins as the matrix. Humins are macromolecular heterogeneous furanic...

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Vydané v:	Composites science and technology Ročník 171; s. 70 - 77
Hlavní autori:	Sangregorio, Anna, Guigo, Nathanael, van der Waal, Jan C., Sbirrazzuoli, Nicolas
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	Barking Elsevier Ltd 08.02.2019 Elsevier BV Elsevier
Predmet:	Automobile industry Automotive engineering Biocomposites Chemical Sciences Composite materials Crosslinking Curing Curing (B) Dynamic mechanical analysis Fibers Fibres (A) Flax Fracture surfaces Material chemistry Mechanical properties Morphology Polymer matrix composites Pressure molding Refining Scanning electron microscopy Scanning electron microscopy (D) Tensile properties Tensile strength Tensile tests Thermomechanical properties (B) Thermosetting resins Water absorption Curing (B) Scanning electron microscopy (D) Fibres (A) Thermomechanical properties (B) Biocomposites
ISSN:	0266-3538, 1879-1050
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Abstract	The use of all “green” composite materials is a great environmental option for several applications such as construction or automotive. A new type of all green composites has been prepared by compression moulding flax fibres with humins as the matrix. Humins are macromolecular heterogeneous furanic co-products from biorefinery operations. For the first time the potential of humins as a whole thermoset-like matrix in combination with natural fibres was studied. The raw industrial humins were cross-linked with and without catalyst. The effect of the process conditions on the final properties of the composites was studied. Good tensile properties were measured by tensile test and Dynamic Mechanical Analysis. Observations of the fracture surface were done by Scanning Electron Microscope, revealing a void-free morphology. The study finally focused on the water absorption behaviour, underlining the more hydrophobic nature of the humins' composites compared to the raw flax mat. The good adhesion between the fibre and the matrix was underlined. Humins interacts with the hydrophilic fibres thus creating a good interphase, leading to improved properties. The study demonstrated the possibility of using a biorefinery co-product as a thermoset matrix for preparing composites materials.
AbstractList	The use of all “green” composite materials is a great environmental option for several applications such as construction or automotive. A new type of all green composites has been prepared by compression moulding flax fibres with humins as the matrix. Humins are macromolecular heterogeneous furanic co-products from biorefinery operations. For the first time the potential of humins as a whole thermoset-like matrix in combination with natural fibres was studied. The raw industrial humins were cross-linked with and without catalyst. The effect of the process conditions on the final properties of the composites was studied. Good tensile properties were measured by tensile test and Dynamic Mechanical Analysis. Observations of the fracture surface were done by Scanning Electron Microscope, revealing a void-free morphology. The study finally focused on the water absorption behaviour, underlining the more hydrophobic nature of the humins' composites compared to the raw flax mat. The good adhesion between the fibre and the matrix was underlined. Humins interacts with the hydrophilic fibres thus creating a good interphase, leading to improved properties. The study demonstrated the possibility of using a biorefinery co-product as a thermoset matrix for preparing composites materials.
Author	Sbirrazzuoli, Nicolas Sangregorio, Anna Guigo, Nathanael van der Waal, Jan C.
Author_xml	– sequence: 1 givenname: Anna surname: Sangregorio fullname: Sangregorio, Anna organization: Avantium Chemicals B.V., Zekeringstraat 29, 1014 BV, Amsterdam, the Netherlands – sequence: 2 givenname: Nathanael surname: Guigo fullname: Guigo, Nathanael email: nathanael.guigo@unice.fr organization: Université Côte d'Azur, Institut de Chimie de Nice, CNRS, UMR 7272, 06108, Nice, France – sequence: 3 givenname: Jan C. surname: van der Waal fullname: van der Waal, Jan C. organization: Avantium Chemicals B.V., Zekeringstraat 29, 1014 BV, Amsterdam, the Netherlands – sequence: 4 givenname: Nicolas surname: Sbirrazzuoli fullname: Sbirrazzuoli, Nicolas organization: Université Côte d'Azur, Institut de Chimie de Nice, CNRS, UMR 7272, 06108, Nice, France
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Snippet	The use of all “green” composite materials is a great environmental option for several applications such as construction or automotive. A new type of all green... The use of all "green" composite materials is a great environmental option for several applications such as construction or automotive. A new type of all green...
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SubjectTerms	Automobile industry Automotive engineering Biocomposites Chemical Sciences Composite materials Crosslinking Curing Curing (B) Dynamic mechanical analysis Fibers Fibres (A) Flax Fracture surfaces Material chemistry Mechanical properties Morphology Polymer matrix composites Pressure molding Refining Scanning electron microscopy Scanning electron microscopy (D) Tensile properties Tensile strength Tensile tests Thermomechanical properties (B) Thermosetting resins Water absorption
Title	All ‘green’ composites comprising flax fibres and humins' resins
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