Solution‐Processable Pure Green Thermally Activated Delayed Fluorescence Emitter Based on the Multiple Resonance Effect

Thermally activated delayed fluorescence (TADF) materials based on the multiple resonance (MR) effect are applied in organic light‐emitting diodes (OLEDs), combining high color purity and efficiency. However, they are not fabricated via solution‐processing, which is an economical approach toward the...

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Vydáno v:	Advanced materials (Weinheim) Ročník 32; číslo 40; s. e2004072 - n/a
Hlavní autoři:	Ikeda, Naoya, Oda, Susumu, Matsumoto, Ryuji, Yoshioka, Mayu, Fukushima, Daisuke, Yoshiura, Kazuki, Yasuda, Nobuhiro, Hatakeyama, Takuji
Médium:	Journal Article
Jazyk:	angličtina
Vydáno:	Weinheim Wiley Subscription Services, Inc 01.10.2020
Témata:	Boron Efficiency Electroluminescence Emitters Energy gap Fluorescence Interlayers Ionization potentials Mass production Materials science Molecular orbitals multiple resonance effect Organic light emitting diodes Oxygen atoms Photoluminescence Polymers pure green Quantum efficiency Resonance solution‐processable Synthesis thermally activated delayed fluorescence
ISSN:	0935-9648, 1521-4095, 1521-4095
On-line přístup:	Získat plný text
Tagy:	Přidat tag Žádné tagy, Buďte první, kdo vytvoří štítek k tomuto záznamu!

Abstract	Thermally activated delayed fluorescence (TADF) materials based on the multiple resonance (MR) effect are applied in organic light‐emitting diodes (OLEDs), combining high color purity and efficiency. However, they are not fabricated via solution‐processing, which is an economical approach toward the mass production of OLED displays. Here, a solution‐processable MR‐TADF material (OAB‐ABP‐1), with an extended π‐skeleton and bulky substituents, is designed. OAB‐ABP‐1 is synthesized from commercially available starting materials via a four‐step process involving one‐shot double borylation. OAB‐ABP‐1 presents attractive photophysical properties, a narrow emission band, a high photoluminescence quantum yield, a small energy gap between S1 and T1, and low activation energy for reverse intersystem crossing. These properties are attributed to the alternating localization of the highest occupied and lowest unoccupied molecular orbitals induced by the boron, nitrogen, and oxygen atoms. Furthermore, to facilitate charge recombination, two novel semiconducting polymers with similar ionization potentials to that of OAB‐ABP‐1 are synthesized for use as interlayer and emissive layer materials. A solution‐processed OLED device is fabricated using OAB‐ABP‐1 and the aforementioned polymers; it exhibits pure green electroluminescence with a small full‐width at half‐maximum and a high external quantum efficiency with minimum efficiency roll‐off. A thermally activated delayed fluorescence material featuring a multiple resonance effect of boron, nitrogen, and oxygen atoms (OAB‐ABP‐1) is synthesized by one‐shot double borylation. A solution‐processed organic light‐emitting diode (OLED) device using OAB‐ABP‐1 exhibits pure green electroluminescence with a small full‐width at half‐maximum, and a high external quantum efficiency with minimum efficiency roll‐off.
AbstractList	Thermally activated delayed fluorescence (TADF) materials based on the multiple resonance (MR) effect are applied in organic light-emitting diodes (OLEDs), combining high color purity and efficiency. However, they are not fabricated via solution-processing, which is an economical approach toward the mass production of OLED displays. Here, a solution-processable MR-TADF material (OAB-ABP-1), with an extended π-skeleton and bulky substituents, is designed. OAB-ABP-1 is synthesized from commercially available starting materials via a four-step process involving one-shot double borylation. OAB-ABP-1 presents attractive photophysical properties, a narrow emission band, a high photoluminescence quantum yield, a small energy gap between S1 and T1 , and low activation energy for reverse intersystem crossing. These properties are attributed to the alternating localization of the highest occupied and lowest unoccupied molecular orbitals induced by the boron, nitrogen, and oxygen atoms. Furthermore, to facilitate charge recombination, two novel semiconducting polymers with similar ionization potentials to that of OAB-ABP-1 are synthesized for use as interlayer and emissive layer materials. A solution-processed OLED device is fabricated using OAB-ABP-1 and the aforementioned polymers; it exhibits pure green electroluminescence with a small full-width at half-maximum and a high external quantum efficiency with minimum efficiency roll-off.Thermally activated delayed fluorescence (TADF) materials based on the multiple resonance (MR) effect are applied in organic light-emitting diodes (OLEDs), combining high color purity and efficiency. However, they are not fabricated via solution-processing, which is an economical approach toward the mass production of OLED displays. Here, a solution-processable MR-TADF material (OAB-ABP-1), with an extended π-skeleton and bulky substituents, is designed. OAB-ABP-1 is synthesized from commercially available starting materials via a four-step process involving one-shot double borylation. OAB-ABP-1 presents attractive photophysical properties, a narrow emission band, a high photoluminescence quantum yield, a small energy gap between S1 and T1 , and low activation energy for reverse intersystem crossing. These properties are attributed to the alternating localization of the highest occupied and lowest unoccupied molecular orbitals induced by the boron, nitrogen, and oxygen atoms. Furthermore, to facilitate charge recombination, two novel semiconducting polymers with similar ionization potentials to that of OAB-ABP-1 are synthesized for use as interlayer and emissive layer materials. A solution-processed OLED device is fabricated using OAB-ABP-1 and the aforementioned polymers; it exhibits pure green electroluminescence with a small full-width at half-maximum and a high external quantum efficiency with minimum efficiency roll-off. Thermally activated delayed fluorescence (TADF) materials based on the multiple resonance (MR) effect are applied in organic light‐emitting diodes (OLEDs), combining high color purity and efficiency. However, they are not fabricated via solution‐processing, which is an economical approach toward the mass production of OLED displays. Here, a solution‐processable MR‐TADF material (OAB‐ABP‐1), with an extended π‐skeleton and bulky substituents, is designed. OAB‐ABP‐1 is synthesized from commercially available starting materials via a four‐step process involving one‐shot double borylation. OAB‐ABP‐1 presents attractive photophysical properties, a narrow emission band, a high photoluminescence quantum yield, a small energy gap between S1 and T1, and low activation energy for reverse intersystem crossing. These properties are attributed to the alternating localization of the highest occupied and lowest unoccupied molecular orbitals induced by the boron, nitrogen, and oxygen atoms. Furthermore, to facilitate charge recombination, two novel semiconducting polymers with similar ionization potentials to that of OAB‐ABP‐1 are synthesized for use as interlayer and emissive layer materials. A solution‐processed OLED device is fabricated using OAB‐ABP‐1 and the aforementioned polymers; it exhibits pure green electroluminescence with a small full‐width at half‐maximum and a high external quantum efficiency with minimum efficiency roll‐off. A thermally activated delayed fluorescence material featuring a multiple resonance effect of boron, nitrogen, and oxygen atoms (OAB‐ABP‐1) is synthesized by one‐shot double borylation. A solution‐processed organic light‐emitting diode (OLED) device using OAB‐ABP‐1 exhibits pure green electroluminescence with a small full‐width at half‐maximum, and a high external quantum efficiency with minimum efficiency roll‐off. Thermally activated delayed fluorescence (TADF) materials based on the multiple resonance (MR) effect are applied in organic light‐emitting diodes (OLEDs), combining high color purity and efficiency. However, they are not fabricated via solution‐processing, which is an economical approach toward the mass production of OLED displays. Here, a solution‐processable MR‐TADF material (OAB‐ABP‐1), with an extended π‐skeleton and bulky substituents, is designed. OAB‐ABP‐1 is synthesized from commercially available starting materials via a four‐step process involving one‐shot double borylation. OAB‐ABP‐1 presents attractive photophysical properties, a narrow emission band, a high photoluminescence quantum yield, a small energy gap between S1 and T1, and low activation energy for reverse intersystem crossing. These properties are attributed to the alternating localization of the highest occupied and lowest unoccupied molecular orbitals induced by the boron, nitrogen, and oxygen atoms. Furthermore, to facilitate charge recombination, two novel semiconducting polymers with similar ionization potentials to that of OAB‐ABP‐1 are synthesized for use as interlayer and emissive layer materials. A solution‐processed OLED device is fabricated using OAB‐ABP‐1 and the aforementioned polymers; it exhibits pure green electroluminescence with a small full‐width at half‐maximum and a high external quantum efficiency with minimum efficiency roll‐off. Thermally activated delayed fluorescence (TADF) materials based on the multiple resonance (MR) effect are applied in organic light‐emitting diodes (OLEDs), combining high color purity and efficiency. However, they are not fabricated via solution‐processing, which is an economical approach toward the mass production of OLED displays. Here, a solution‐processable MR‐TADF material (OAB‐ABP‐1), with an extended π‐skeleton and bulky substituents, is designed. OAB‐ABP‐1 is synthesized from commercially available starting materials via a four‐step process involving one‐shot double borylation. OAB‐ABP‐1 presents attractive photophysical properties, a narrow emission band, a high photoluminescence quantum yield, a small energy gap between S 1 and T 1 , and low activation energy for reverse intersystem crossing. These properties are attributed to the alternating localization of the highest occupied and lowest unoccupied molecular orbitals induced by the boron, nitrogen, and oxygen atoms. Furthermore, to facilitate charge recombination, two novel semiconducting polymers with similar ionization potentials to that of OAB‐ABP‐1 are synthesized for use as interlayer and emissive layer materials. A solution‐processed OLED device is fabricated using OAB‐ABP‐1 and the aforementioned polymers; it exhibits pure green electroluminescence with a small full‐width at half‐maximum and a high external quantum efficiency with minimum efficiency roll‐off.
Author	Fukushima, Daisuke Hatakeyama, Takuji Yoshioka, Mayu Yoshiura, Kazuki Oda, Susumu Ikeda, Naoya Matsumoto, Ryuji Yasuda, Nobuhiro
Author_xml	– sequence: 1 givenname: Naoya surname: Ikeda fullname: Ikeda, Naoya organization: Kwansei Gakuin University – sequence: 2 givenname: Susumu orcidid: 0000-0003-1088-1932 surname: Oda fullname: Oda, Susumu organization: Kwansei Gakuin University – sequence: 3 givenname: Ryuji surname: Matsumoto fullname: Matsumoto, Ryuji organization: Sumitomo Chemical Co., Ltd – sequence: 4 givenname: Mayu surname: Yoshioka fullname: Yoshioka, Mayu organization: Sumitomo Chemical Co., Ltd – sequence: 5 givenname: Daisuke surname: Fukushima fullname: Fukushima, Daisuke organization: Sumitomo Chemical Co., Ltd – sequence: 6 givenname: Kazuki surname: Yoshiura fullname: Yoshiura, Kazuki organization: Kwansei Gakuin University – sequence: 7 givenname: Nobuhiro surname: Yasuda fullname: Yasuda, Nobuhiro organization: Japan Synchrotron Radiation Research Institute (JASRI) – sequence: 8 givenname: Takuji orcidid: 0000-0002-7483-9525 surname: Hatakeyama fullname: Hatakeyama, Takuji email: hatake@kwansei.ac.jp organization: Kwansei Gakuin University
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Snippet	Thermally activated delayed fluorescence (TADF) materials based on the multiple resonance (MR) effect are applied in organic light‐emitting diodes (OLEDs),... Thermally activated delayed fluorescence (TADF) materials based on the multiple resonance (MR) effect are applied in organic light-emitting diodes (OLEDs),...
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SubjectTerms	Boron Efficiency Electroluminescence Emitters Energy gap Fluorescence Interlayers Ionization potentials Mass production Materials science Molecular orbitals multiple resonance effect Organic light emitting diodes Oxygen atoms Photoluminescence Polymers pure green Quantum efficiency Resonance solution‐processable Synthesis thermally activated delayed fluorescence
Title	Solution‐Processable Pure Green Thermally Activated Delayed Fluorescence Emitter Based on the Multiple Resonance Effect
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