CNT/PDMS composite membranes for H2 and CH4 gas separation
Polydimethylsiloxane (PDMS) composites with different weight amounts of multi-walled carbon nanotubes (MWCNT) were synthesised as membranes to evaluate their gas separation properties. The selectivity of the membranes was investigated for the separation of H2 from CH4 gas species. Membranes with MWC...
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| Vydáno v: | International journal of hydrogen energy Ročník 38; číslo 25; s. 10494 - 10501 |
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| Hlavní autoři: | , , , , , , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
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Kidlington
Elsevier Ltd
21.08.2013
Elsevier |
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| ISSN: | 0360-3199, 1879-3487 |
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| Abstract | Polydimethylsiloxane (PDMS) composites with different weight amounts of multi-walled carbon nanotubes (MWCNT) were synthesised as membranes to evaluate their gas separation properties. The selectivity of the membranes was investigated for the separation of H2 from CH4 gas species. Membranes with MWCNT concentrations of 1% increased the selectivity to H2 gas by 94.8%. Furthermore, CH4 permeation was almost totally blocked through membranes with MWCNT concentrations greater than 5%. Vibrational spectroscopy and X-ray photoelectron spectroscopy techniques revealed that upon the incorporation of MWCNT a decrease in the number of available Si–CH3 and Si–O bonds as well as an increase in the formation of Si–C bonds occurred that initiated the reduction in CH4 permeation. As a result, the developed membranes can be an efficient and low cost solution for separating H2 from larger gas molecules such as CH4.
•PDMS nanocomposite membranes of different MWCNT concentrations were synthesized.•The membranes were investigated for separating H2 and CH4 gas molecules.•Si–CH3, Si–O, and Si–C bonds played important roles in the membranes' performance.•More than 1wt% of MWCNT in membranes selectively attenuated the permeation of CH4.•MWCNT emerged as an effective additive for tuning H2/CH4 membranes' selectivity. |
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| AbstractList | Polydimethylsiloxane (PDMS) composites with different weight amounts of multi-walled carbon nanotubes (MWCNT) were synthesised as membranes to evaluate their gas separation properties. The selectivity of the membranes was investigated for the separation of H2 from CH4 gas species. Membranes with MWCNT concentrations of 1% increased the selectivity to H2 gas by 94.8%. Furthermore, CH4 permeation was almost totally blocked through membranes with MWCNT concentrations greater than 5%. Vibrational spectroscopy and X-ray photoelectron spectroscopy techniques revealed that upon the incorporation of MWCNT a decrease in the number of available Si–CH3 and Si–O bonds as well as an increase in the formation of Si–C bonds occurred that initiated the reduction in CH4 permeation. As a result, the developed membranes can be an efficient and low cost solution for separating H2 from larger gas molecules such as CH4.
•PDMS nanocomposite membranes of different MWCNT concentrations were synthesized.•The membranes were investigated for separating H2 and CH4 gas molecules.•Si–CH3, Si–O, and Si–C bonds played important roles in the membranes' performance.•More than 1wt% of MWCNT in membranes selectively attenuated the permeation of CH4.•MWCNT emerged as an effective additive for tuning H2/CH4 membranes' selectivity. Polydimethylsiloxane (PDMS) composites with different weight amounts of multi-walled carbon nanotubes (MWCNT) were synthesised as membranes to evaluate their gas separation properties. The selectivity of the membranes was investigated for the separation of H2 from CH4 gas species. Membranes with MWCNT concentrations of 1% increased the selectivity to H2 gas by 94.8%. Furthermore, CH4 permeation was almost totally blocked through membranes with MWCNT concentrations greater than 5%. Vibrational spectroscopy and X-ray photoelectron spectroscopy techniques revealed that upon the incorporation of MWCNT a decrease in the number of available SiaCH3 and SiaO bonds as well as an increase in the formation of SiaC bonds occurred that initiated the reduction in CH4 permeation. As a result, the developed membranes can be an efficient and low cost solution for separating H2 from larger gas molecules such as CH4. |
| Author | Kalantar-zadeh, Kourosh Du Plessis, Johan Nour, Majid Berean, Kyle Sriram, Sharath McSweeney, Chris Balendhran, Sivacarendran Ou, Jian Zhen Bhaskaran, Madhu |
| Author_xml | – sequence: 1 givenname: Majid surname: Nour fullname: Nour, Majid email: nour.mk@gmail.com organization: School of Electrical and Computer Engineering, RMIT University, Melbourne, Australia – sequence: 2 givenname: Kyle surname: Berean fullname: Berean, Kyle email: kyleberean@gmail.com organization: School of Electrical and Computer Engineering, RMIT University, Melbourne, Australia – sequence: 3 givenname: Sivacarendran surname: Balendhran fullname: Balendhran, Sivacarendran organization: School of Electrical and Computer Engineering, RMIT University, Melbourne, Australia – sequence: 4 givenname: Jian Zhen surname: Ou fullname: Ou, Jian Zhen organization: School of Electrical and Computer Engineering, RMIT University, Melbourne, Australia – sequence: 5 givenname: Johan surname: Du Plessis fullname: Du Plessis, Johan organization: School of Applied Sciences, RMIT University, Melbourne, Australia – sequence: 6 givenname: Chris surname: McSweeney fullname: McSweeney, Chris organization: CSIRO Livestock Industries, Queensland BioScience Precinct, St Lucia, Australia – sequence: 7 givenname: Madhu surname: Bhaskaran fullname: Bhaskaran, Madhu organization: School of Electrical and Computer Engineering, RMIT University, Melbourne, Australia – sequence: 8 givenname: Sharath surname: Sriram fullname: Sriram, Sharath organization: School of Electrical and Computer Engineering, RMIT University, Melbourne, Australia – sequence: 9 givenname: Kourosh surname: Kalantar-zadeh fullname: Kalantar-zadeh, Kourosh email: kourosh.kalantar@rmit.edu.au organization: School of Electrical and Computer Engineering, RMIT University, Melbourne, Australia |
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| Keywords | Carbon nanotube Membrane Gas separation H2 Polydimethylsiloxane CH4 Hydrogen CH Carbon nanotubes H |
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| Snippet | Polydimethylsiloxane (PDMS) composites with different weight amounts of multi-walled carbon nanotubes (MWCNT) were synthesised as membranes to evaluate their... |
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| SubjectTerms | Alternative fuels. Production and utilization Applied sciences Carbon nanotube CH4 Energy Exact sciences and technology Fuels Gas separation Hydrogen Hydrogen-based energy Membrane Membranes Multi wall carbon nanotubes Penetration Permeation Polydimethylsiloxane Selectivity Silicone resins |
| Title | CNT/PDMS composite membranes for H2 and CH4 gas separation |
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