Nonfullerene Tandem Organic Solar Cells with High Performance of 14.11

Fabricating solar cells with tandem structure is an efficient way to broaden the photon response range without further increasing the thermalization loss in the system. In this work, a tandem organic solar cell (TOSC) based on highly efficient nonfullerene acceptors (NFAs) with series connection typ...

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Veröffentlicht in:	Advanced materials (Weinheim) Jg. 30; H. 18; S. e1707508 - n/a
Hauptverfasser:	Zhang, Yamin, Kan, Bin, Sun, Yanna, Wang, Yanbo, Xia, Ruoxi, Ke, Xin, Yi, Yuan‐Qiu‐Qiang, Li, Chenxi, Yip, Hin‐Lap, Wan, Xiangjian, Cao, Yong, Chen, Yongsheng
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Germany Wiley Subscription Services, Inc 03.05.2018
Schlagworte:	Energy conversion efficiency Energy gap high efficiency Materials science nonfullerene acceptors Photovoltaic cells Polymers Solar cells tandem organic solar cells Thermalization (energy absorption) Thickness high efficiency nonfullerene acceptors tandem organic solar cells
ISSN:	0935-9648, 1521-4095, 1521-4095
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Abstract	Fabricating solar cells with tandem structure is an efficient way to broaden the photon response range without further increasing the thermalization loss in the system. In this work, a tandem organic solar cell (TOSC) based on highly efficient nonfullerene acceptors (NFAs) with series connection type is demonstrated. To meet the different demands of front and rear sub‐cells, two NFAs named F‐M and NOBDT with a whole absorption range from 300 to 900 nm are designed, when blended with wide bandgap polymer poly[(2,6‐(4,8‐bis(5‐(2‐ethylhexyl)thiophen‐2‐yl)‐benzo[1,2‐b:4,5‐b′]dithiophene))‐alt‐(5,5‐(1′,3′‐di‐2‐thienyl‐5′,7′‐bis(2‐ethylhexyl)benzo[1′,2′‐c:4′,5′‐c′]dithiophene‐4,8‐dione))] (PBDB‐T) and narrow bandgap polymer PTB7‐Th, respectively, the PBDB‐T: F‐M system exhibits a high Voc of 0.98 V and the PTB7‐Th: NOBDT system shows a remarkable Jsc of 19.16 mA cm−2, which demonstrate their potential in the TOSCs. With the guidance of optical simulation, by systematically optimizing the thickness of each layer in the TOSC, an outstanding power conversion efficiency of 14.11%, with a Voc of 1.71 V, a Jsc of 11.72 mA cm−2, and a satisfactory fill factor of 0.70 is achieved; this result is one of the top efficiencies reported to date in the field of organic solar cells. A non‐fullerene tandem organic solar cell (OSC) with high efficiency is fabricated. Two non‐fullerene acceptors named F‐M and NOBDT with a whole absorption range from 300–900 nm are designed for the front and rear sub‐cell respectively; the tandem cell based on them demonstrates an outstanding PCE of 14.11%, which is among the top PCEs in the field of OSCs.
AbstractList	Fabricating solar cells with tandem structure is an efficient way to broaden the photon response range without further increasing the thermalization loss in the system. In this work, a tandem organic solar cell (TOSC) based on highly efficient nonfullerene acceptors (NFAs) with series connection type is demonstrated. To meet the different demands of front and rear sub‐cells, two NFAs named F‐M and NOBDT with a whole absorption range from 300 to 900 nm are designed, when blended with wide bandgap polymer poly[(2,6‐(4,8‐bis(5‐(2‐ethylhexyl)thiophen‐2‐yl)‐benzo[1,2‐b:4,5‐b′]dithiophene))‐alt‐(5,5‐(1′,3′‐di‐2‐thienyl‐5′,7′‐bis(2‐ethylhexyl)benzo[1′,2′‐c:4′,5′‐c′]dithiophene‐4,8‐dione))] (PBDB‐T) and narrow bandgap polymer PTB7‐Th, respectively, the PBDB‐T: F‐M system exhibits a high Voc of 0.98 V and the PTB7‐Th: NOBDT system shows a remarkable Jsc of 19.16 mA cm−2, which demonstrate their potential in the TOSCs. With the guidance of optical simulation, by systematically optimizing the thickness of each layer in the TOSC, an outstanding power conversion efficiency of 14.11%, with a Voc of 1.71 V, a Jsc of 11.72 mA cm−2, and a satisfactory fill factor of 0.70 is achieved; this result is one of the top efficiencies reported to date in the field of organic solar cells. Fabricating solar cells with tandem structure is an efficient way to broaden the photon response range without further increasing the thermalization loss in the system. In this work, a tandem organic solar cell (TOSC) based on highly efficient nonfullerene acceptors (NFAs) with series connection type is demonstrated. To meet the different demands of front and rear sub‐cells, two NFAs named F‐M and NOBDT with a whole absorption range from 300 to 900 nm are designed, when blended with wide bandgap polymer poly[(2,6‐(4,8‐bis(5‐(2‐ethylhexyl)thiophen‐2‐yl)‐benzo[1,2‐b:4,5‐b′]dithiophene))‐ alt ‐(5,5‐(1′,3′‐di‐2‐thienyl‐5′,7′‐bis(2‐ethylhexyl)benzo[1′,2′‐c:4′,5′‐c′]dithiophene‐4,8‐dione))] (PBDB‐T) and narrow bandgap polymer PTB7‐Th, respectively, the PBDB‐T: F‐M system exhibits a high V oc of 0.98 V and the PTB7‐Th: NOBDT system shows a remarkable J sc of 19.16 mA cm −2 , which demonstrate their potential in the TOSCs. With the guidance of optical simulation, by systematically optimizing the thickness of each layer in the TOSC, an outstanding power conversion efficiency of 14.11%, with a V oc of 1.71 V, a J sc of 11.72 mA cm −2 , and a satisfactory fill factor of 0.70 is achieved; this result is one of the top efficiencies reported to date in the field of organic solar cells. Fabricating solar cells with tandem structure is an efficient way to broaden the photon response range without further increasing the thermalization loss in the system. In this work, a tandem organic solar cell (TOSC) based on highly efficient nonfullerene acceptors (NFAs) with series connection type is demonstrated. To meet the different demands of front and rear sub-cells, two NFAs named F-M and NOBDT with a whole absorption range from 300 to 900 nm are designed, when blended with wide bandgap polymer poly[(2,6-(4,8-bis(5-(2-ethylhexyl)thiophen-2-yl)-benzo[1,2-b:4,5-b']dithiophene))-alt-(5,5-(1',3'-di-2-thienyl-5',7'-bis(2-ethylhexyl)benzo[1',2'-c:4',5'-c']dithiophene-4,8-dione))] (PBDB-T) and narrow bandgap polymer PTB7-Th, respectively, the PBDB-T: F-M system exhibits a high V of 0.98 V and the PTB7-Th: NOBDT system shows a remarkable J of 19.16 mA cm , which demonstrate their potential in the TOSCs. With the guidance of optical simulation, by systematically optimizing the thickness of each layer in the TOSC, an outstanding power conversion efficiency of 14.11%, with a V of 1.71 V, a J of 11.72 mA cm , and a satisfactory fill factor of 0.70 is achieved; this result is one of the top efficiencies reported to date in the field of organic solar cells. Fabricating solar cells with tandem structure is an efficient way to broaden the photon response range without further increasing the thermalization loss in the system. In this work, a tandem organic solar cell (TOSC) based on highly efficient nonfullerene acceptors (NFAs) with series connection type is demonstrated. To meet the different demands of front and rear sub-cells, two NFAs named F-M and NOBDT with a whole absorption range from 300 to 900 nm are designed, when blended with wide bandgap polymer poly[(2,6-(4,8-bis(5-(2-ethylhexyl)thiophen-2-yl)-benzo[1,2-b:4,5-b']dithiophene))-alt-(5,5-(1',3'-di-2-thienyl-5',7'-bis(2-ethylhexyl)benzo[1',2'-c:4',5'-c']dithiophene-4,8-dione))] (PBDB-T) and narrow bandgap polymer PTB7-Th, respectively, the PBDB-T: F-M system exhibits a high Voc of 0.98 V and the PTB7-Th: NOBDT system shows a remarkable Jsc of 19.16 mA cm-2 , which demonstrate their potential in the TOSCs. With the guidance of optical simulation, by systematically optimizing the thickness of each layer in the TOSC, an outstanding power conversion efficiency of 14.11%, with a Voc of 1.71 V, a Jsc of 11.72 mA cm-2 , and a satisfactory fill factor of 0.70 is achieved; this result is one of the top efficiencies reported to date in the field of organic solar cells.Fabricating solar cells with tandem structure is an efficient way to broaden the photon response range without further increasing the thermalization loss in the system. In this work, a tandem organic solar cell (TOSC) based on highly efficient nonfullerene acceptors (NFAs) with series connection type is demonstrated. To meet the different demands of front and rear sub-cells, two NFAs named F-M and NOBDT with a whole absorption range from 300 to 900 nm are designed, when blended with wide bandgap polymer poly[(2,6-(4,8-bis(5-(2-ethylhexyl)thiophen-2-yl)-benzo[1,2-b:4,5-b']dithiophene))-alt-(5,5-(1',3'-di-2-thienyl-5',7'-bis(2-ethylhexyl)benzo[1',2'-c:4',5'-c']dithiophene-4,8-dione))] (PBDB-T) and narrow bandgap polymer PTB7-Th, respectively, the PBDB-T: F-M system exhibits a high Voc of 0.98 V and the PTB7-Th: NOBDT system shows a remarkable Jsc of 19.16 mA cm-2 , which demonstrate their potential in the TOSCs. With the guidance of optical simulation, by systematically optimizing the thickness of each layer in the TOSC, an outstanding power conversion efficiency of 14.11%, with a Voc of 1.71 V, a Jsc of 11.72 mA cm-2 , and a satisfactory fill factor of 0.70 is achieved; this result is one of the top efficiencies reported to date in the field of organic solar cells. Fabricating solar cells with tandem structure is an efficient way to broaden the photon response range without further increasing the thermalization loss in the system. In this work, a tandem organic solar cell (TOSC) based on highly efficient nonfullerene acceptors (NFAs) with series connection type is demonstrated. To meet the different demands of front and rear sub‐cells, two NFAs named F‐M and NOBDT with a whole absorption range from 300 to 900 nm are designed, when blended with wide bandgap polymer poly[(2,6‐(4,8‐bis(5‐(2‐ethylhexyl)thiophen‐2‐yl)‐benzo[1,2‐b:4,5‐b′]dithiophene))‐alt‐(5,5‐(1′,3′‐di‐2‐thienyl‐5′,7′‐bis(2‐ethylhexyl)benzo[1′,2′‐c:4′,5′‐c′]dithiophene‐4,8‐dione))] (PBDB‐T) and narrow bandgap polymer PTB7‐Th, respectively, the PBDB‐T: F‐M system exhibits a high Voc of 0.98 V and the PTB7‐Th: NOBDT system shows a remarkable Jsc of 19.16 mA cm−2, which demonstrate their potential in the TOSCs. With the guidance of optical simulation, by systematically optimizing the thickness of each layer in the TOSC, an outstanding power conversion efficiency of 14.11%, with a Voc of 1.71 V, a Jsc of 11.72 mA cm−2, and a satisfactory fill factor of 0.70 is achieved; this result is one of the top efficiencies reported to date in the field of organic solar cells. A non‐fullerene tandem organic solar cell (OSC) with high efficiency is fabricated. Two non‐fullerene acceptors named F‐M and NOBDT with a whole absorption range from 300–900 nm are designed for the front and rear sub‐cell respectively; the tandem cell based on them demonstrates an outstanding PCE of 14.11%, which is among the top PCEs in the field of OSCs.
Author	Sun, Yanna Wang, Yanbo Xia, Ruoxi Cao, Yong Chen, Yongsheng Ke, Xin Zhang, Yamin Li, Chenxi Wan, Xiangjian Yip, Hin‐Lap Kan, Bin Yi, Yuan‐Qiu‐Qiang
Author_xml	– sequence: 1 givenname: Yamin surname: Zhang fullname: Zhang, Yamin organization: Nankai University – sequence: 2 givenname: Bin surname: Kan fullname: Kan, Bin organization: Nankai University – sequence: 3 givenname: Yanna surname: Sun fullname: Sun, Yanna organization: Nankai University – sequence: 4 givenname: Yanbo surname: Wang fullname: Wang, Yanbo organization: Nankai University – sequence: 5 givenname: Ruoxi surname: Xia fullname: Xia, Ruoxi organization: South China University of Technology – sequence: 6 givenname: Xin surname: Ke fullname: Ke, Xin organization: Nankai University – sequence: 7 givenname: Yuan‐Qiu‐Qiang surname: Yi fullname: Yi, Yuan‐Qiu‐Qiang organization: Nankai University – sequence: 8 givenname: Chenxi surname: Li fullname: Li, Chenxi organization: Nankai University – sequence: 9 givenname: Hin‐Lap surname: Yip fullname: Yip, Hin‐Lap organization: South China University of Technology – sequence: 10 givenname: Xiangjian surname: Wan fullname: Wan, Xiangjian organization: Nankai University – sequence: 11 givenname: Yong surname: Cao fullname: Cao, Yong organization: South China University of Technology – sequence: 12 givenname: Yongsheng orcidid: 0000-0003-1448-8177 surname: Chen fullname: Chen, Yongsheng email: yschen99@nankai.edu.cn organization: Nankai University
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/29575107$$D View this record in MEDLINE/PubMed
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Copyright	2018 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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Snippet	Fabricating solar cells with tandem structure is an efficient way to broaden the photon response range without further increasing the thermalization loss in...
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SubjectTerms	Energy conversion efficiency Energy gap high efficiency Materials science nonfullerene acceptors Photovoltaic cells Polymers Solar cells tandem organic solar cells Thermalization (energy absorption) Thickness
Title	Nonfullerene Tandem Organic Solar Cells with High Performance of 14.11
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