Influence of pH on heavy metal speciation and removal from wastewater using micellar-enhanced ultrafiltration

pH plays an important role in heavy metal removal during micellar-enhanced ultrafiltration (MEUF). In the present work, the influence of pH on heavy metal speciation and removal from wastewater by MEUF was investigated using an anionic surfactant (sodium dodecyl sulfate, SDS) and a hydrophilic membr...

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Vydané v:	Chemosphere (Oxford) Ročník 173; s. 199 - 206
Hlavní autori:	Huang, Jinhui, Yuan, Fang, Zeng, Guangming, Li, Xue, Gu, Yanling, Shi, Lixiu, Liu, Wenchu, Shi, Yahui
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	England Elsevier Ltd 01.04.2017
Predmet:	anionic surfactants cadmium Cadmium - isolation & purification copper Copper - isolation & purification Heavy metal speciation heavy metals Hydrogen-Ion Concentration hydrophilicity lead metal ions Metals, Heavy - isolation & purification Micellar-enhanced ultrafiltration Micelles Removal efficiency Sodium Dodecyl Sulfate Surface-Active Agents - chemistry ultrafiltration Ultrafiltration - methods wastewater Water Pollutants, Chemical - isolation & purification zinc Zinc - isolation & purification Heavy metal speciation pH Removal efficiency Micellar-enhanced ultrafiltration
ISSN:	0045-6535, 1879-1298
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Abstract	pH plays an important role in heavy metal removal during micellar-enhanced ultrafiltration (MEUF). In the present work, the influence of pH on heavy metal speciation and removal from wastewater by MEUF was investigated using an anionic surfactant (sodium dodecyl sulfate, SDS) and a hydrophilic membrane (polyether sulfone). Experiments were performed with pH values in the range of 1–12. Metal ion removal efficiency (R) was used to assess the effects of the MEUF process. Results showed that better removal rate of copper and cadmium was achieved at high pH values (pH > 3) with SDS feed concentration of 8 mM, while the optimal pH range was 3–10 for zinc and lead. The corresponding efficiencies for heavy metal removal decreased with the increasing feed concentration of metal ions under the pH conditions of 1–12. Furthermore, the heavy metal ion removal rate (50 mg/L) followed the order of Pb2+ > Cd2+ > Zn2+ > Cu2+. These results showed that pH is a key parameter in metal ion speciation and removal during MEUF. •Heavy metal speciation under different pH was simulated using Visual MINTEQ.•The effect of pH on heavy metal removal during MEUF was investigated.•A correlation for heavy metal ions speciation and removal efficiency was developed.
AbstractList	pH plays an important role in heavy metal removal during micellar-enhanced ultrafiltration (MEUF). In the present work, the influence of pH on heavy metal speciation and removal from wastewater by MEUF was investigated using an anionic surfactant (sodium dodecyl sulfate, SDS) and a hydrophilic membrane (polyether sulfone). Experiments were performed with pH values in the range of 1-12. Metal ion removal efficiency (R) was used to assess the effects of the MEUF process. Results showed that better removal rate of copper and cadmium was achieved at high pH values (pH > 3) with SDS feed concentration of 8 mM, while the optimal pH range was 3-10 for zinc and lead. The corresponding efficiencies for heavy metal removal decreased with the increasing feed concentration of metal ions under the pH conditions of 1-12. Furthermore, the heavy metal ion removal rate (50 mg/L) followed the order of Pb2+ > Cd2+ > Zn2+ > Cu2+. These results showed that pH is a key parameter in metal ion speciation and removal during MEUF. pH plays an important role in heavy metal removal during micellar-enhanced ultrafiltration (MEUF). In the present work, the influence of pH on heavy metal speciation and removal from wastewater by MEUF was investigated using an anionic surfactant (sodium dodecyl sulfate, SDS) and a hydrophilic membrane (polyether sulfone). Experiments were performed with pH values in the range of 1-12. Metal ion removal efficiency (R) was used to assess the effects of the MEUF process. Results showed that better removal rate of copper and cadmium was achieved at high pH values (pH > 3) with SDS feed concentration of 8 mM, while the optimal pH range was 3-10 for zinc and lead. The corresponding efficiencies for heavy metal removal decreased with the increasing feed concentration of metal ions under the pH conditions of 1-12. Furthermore, the heavy metal ion removal rate (50 mg/L) followed the order of Pb > Cd > Zn > Cu . These results showed that pH is a key parameter in metal ion speciation and removal during MEUF. pH plays an important role in heavy metal removal during micellar-enhanced ultrafiltration (MEUF). In the present work, the influence of pH on heavy metal speciation and removal from wastewater by MEUF was investigated using an anionic surfactant (sodium dodecyl sulfate, SDS) and a hydrophilic membrane (polyether sulfone). Experiments were performed with pH values in the range of 1–12. Metal ion removal efficiency (R) was used to assess the effects of the MEUF process. Results showed that better removal rate of copper and cadmium was achieved at high pH values (pH > 3) with SDS feed concentration of 8 mM, while the optimal pH range was 3–10 for zinc and lead. The corresponding efficiencies for heavy metal removal decreased with the increasing feed concentration of metal ions under the pH conditions of 1–12. Furthermore, the heavy metal ion removal rate (50 mg/L) followed the order of Pb2+ > Cd2+ > Zn2+ > Cu2+. These results showed that pH is a key parameter in metal ion speciation and removal during MEUF. •Heavy metal speciation under different pH was simulated using Visual MINTEQ.•The effect of pH on heavy metal removal during MEUF was investigated.•A correlation for heavy metal ions speciation and removal efficiency was developed.
Author	Zeng, Guangming Gu, Yanling Liu, Wenchu Li, Xue Shi, Yahui Yuan, Fang Huang, Jinhui Shi, Lixiu
Author_xml	– sequence: 1 givenname: Jinhui surname: Huang fullname: Huang, Jinhui email: huangjinhui_59@163.com organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 2 givenname: Fang surname: Yuan fullname: Yuan, Fang organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 3 givenname: Guangming surname: Zeng fullname: Zeng, Guangming email: zgming@hnu.edu.cn organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 4 givenname: Xue surname: Li fullname: Li, Xue organization: Department of Bioengineering and Environmental Science, Changsha University, Changsha 410003, China – sequence: 5 givenname: Yanling surname: Gu fullname: Gu, Yanling organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 6 givenname: Lixiu surname: Shi fullname: Shi, Lixiu organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 7 givenname: Wenchu surname: Liu fullname: Liu, Wenchu organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China – sequence: 8 givenname: Yahui surname: Shi fullname: Shi, Yahui organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, China
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Keywords	Heavy metal speciation pH Removal efficiency Micellar-enhanced ultrafiltration
Language	English
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Snippet	pH plays an important role in heavy metal removal during micellar-enhanced ultrafiltration (MEUF). In the present work, the influence of pH on heavy metal...
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SubjectTerms	anionic surfactants cadmium Cadmium - isolation & purification copper Copper - isolation & purification Heavy metal speciation heavy metals Hydrogen-Ion Concentration hydrophilicity lead metal ions Metals, Heavy - isolation & purification Micellar-enhanced ultrafiltration Micelles Removal efficiency Sodium Dodecyl Sulfate Surface-Active Agents - chemistry ultrafiltration Ultrafiltration - methods wastewater Water Pollutants, Chemical - isolation & purification zinc Zinc - isolation & purification
Title	Influence of pH on heavy metal speciation and removal from wastewater using micellar-enhanced ultrafiltration
URI	https://dx.doi.org/10.1016/j.chemosphere.2016.12.137 https://www.ncbi.nlm.nih.gov/pubmed/28110009 https://www.proquest.com/docview/1861589636 https://www.proquest.com/docview/2000333727
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