Charge carrier trapping, recombination and transfer during TiO2 photocatalysis: An overview

[Display omitted] •Analytic methods to study the charge carrier dynamics are introduced.•The fates of charge carrier trapping and recombination are understood.•Various interfacial charge transfer processes are discussed case-by-case. Heterogeneous photocatalysis mediated by semiconducting TiO2 has a...

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Published in:	Catalysis today Vol. 335; pp. 78 - 90
Main Authors:	Qian, Ruifeng, Zong, Huixin, Schneider, Jenny, Zhou, Guanda, Zhao, Ting, Li, Yongli, Yang, Jing, Bahnemann, Detlef W., Pan, Jia Hong
Format:	Journal Article
Language:	English
Published:	Elsevier B.V 01.09.2019
Subjects:	Charge carrier dynamics Electron transfer EPR spectroscopy Semiconductor photocatalysis TiO2 Transient spectroscopy Electron transfer Semiconductor photocatalysis Charge carrier dynamics EPR spectroscopy TiO2 Transient spectroscopy
ISSN:	0920-5861, 1873-4308
Online Access:	Get full text
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Abstract	[Display omitted] •Analytic methods to study the charge carrier dynamics are introduced.•The fates of charge carrier trapping and recombination are understood.•Various interfacial charge transfer processes are discussed case-by-case. Heterogeneous photocatalysis mediated by semiconducting TiO2 has attracted continuous interest during the past decades and has shown great potentials in environmental remediation and solar energy conversion. Basically, photocatalysis is initiated by the TiO2 excitation. The generated charge carriers undergo trapping, recombination, and interfacial transfer before proceeding the redox reaction at TiO2 surface. Monitoring the charge carrier dynamics is of particulate importance for understanding the underlying mechanism and designing efficient photocatalysts. This review overviews the recent progress in characterization of charge carrier dynamics. We will present the analytic techniques for monitoring the fate of charge carriers at each elementary photocatalytic step, including charge carrier generation, trapping and recombination inside the photocatalyst, as well as the interfacial charge transfer. The charge carrier dynamics at TiO2/H2O interface, hole transfer reactions for O2 production, and photocatalytic oxidation of organic compounds and nitric oxides, and electron transfer reactions for photocatalytic reduction of viologens and metal ions are addressed, aiming at a deeper understanding of photocatalytic process.
AbstractList	[Display omitted] •Analytic methods to study the charge carrier dynamics are introduced.•The fates of charge carrier trapping and recombination are understood.•Various interfacial charge transfer processes are discussed case-by-case. Heterogeneous photocatalysis mediated by semiconducting TiO2 has attracted continuous interest during the past decades and has shown great potentials in environmental remediation and solar energy conversion. Basically, photocatalysis is initiated by the TiO2 excitation. The generated charge carriers undergo trapping, recombination, and interfacial transfer before proceeding the redox reaction at TiO2 surface. Monitoring the charge carrier dynamics is of particulate importance for understanding the underlying mechanism and designing efficient photocatalysts. This review overviews the recent progress in characterization of charge carrier dynamics. We will present the analytic techniques for monitoring the fate of charge carriers at each elementary photocatalytic step, including charge carrier generation, trapping and recombination inside the photocatalyst, as well as the interfacial charge transfer. The charge carrier dynamics at TiO2/H2O interface, hole transfer reactions for O2 production, and photocatalytic oxidation of organic compounds and nitric oxides, and electron transfer reactions for photocatalytic reduction of viologens and metal ions are addressed, aiming at a deeper understanding of photocatalytic process.
Author	Li, Yongli Schneider, Jenny Yang, Jing Zhao, Ting Qian, Ruifeng Pan, Jia Hong Zong, Huixin Zhou, Guanda Bahnemann, Detlef W.
Author_xml	– sequence: 1 givenname: Ruifeng surname: Qian fullname: Qian, Ruifeng organization: Beijing Key Laboratory of Energy Safety and Clean Utilization, School of Renewable Energy, North China Electric Power University, Beijing 102206, China – sequence: 2 givenname: Huixin surname: Zong fullname: Zong, Huixin organization: Beijing Key Laboratory of Energy Safety and Clean Utilization, School of Renewable Energy, North China Electric Power University, Beijing 102206, China – sequence: 3 givenname: Jenny surname: Schneider fullname: Schneider, Jenny organization: Department of Chemistry, University of North Carolina at Chapel Hill, Chapel Hill 27599, USA – sequence: 4 givenname: Guanda surname: Zhou fullname: Zhou, Guanda organization: Beijing Key Laboratory of Energy Safety and Clean Utilization, School of Renewable Energy, North China Electric Power University, Beijing 102206, China – sequence: 5 givenname: Ting surname: Zhao fullname: Zhao, Ting organization: Beijing Key Laboratory of Energy Safety and Clean Utilization, School of Renewable Energy, North China Electric Power University, Beijing 102206, China – sequence: 6 givenname: Yongli surname: Li fullname: Li, Yongli organization: School of Energy Power and Mechanical Engineering, North China Electric Power University, Beijing 102206, China – sequence: 7 givenname: Jing surname: Yang fullname: Yang, Jing email: yangjing@imre.a-star.edu.sg organization: Institute of Materials Research and Engineering, A⁎STAR (Agency for Science, Technology and Research), 2 Fusionopolis Way, Innovis, #08-03, 138634, Singapore – sequence: 8 givenname: Detlef W. surname: Bahnemann fullname: Bahnemann, Detlef W. email: bahnemann@iftc.uni-hannover.de organization: Institut für Technische Chemie, Leibniz Universität Hannover, Callinstrasse 3, D-30167, Hannover, Germany – sequence: 9 givenname: Jia Hong surname: Pan fullname: Pan, Jia Hong email: pan@ncepu.edu.cn organization: Beijing Key Laboratory of Energy Safety and Clean Utilization, School of Renewable Energy, North China Electric Power University, Beijing 102206, China
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Snippet	[Display omitted] •Analytic methods to study the charge carrier dynamics are introduced.•The fates of charge carrier trapping and recombination are...
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SubjectTerms	Charge carrier dynamics Electron transfer EPR spectroscopy Semiconductor photocatalysis TiO2 Transient spectroscopy
Title	Charge carrier trapping, recombination and transfer during TiO2 photocatalysis: An overview
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