Hydrogen-induced transgranular to intergranular fracture transition in bi-crystalline nickel

It is known that hydrogen can influence the dislocation plasticity and fracture mode transition of metallic materials, however, the nanoscale interaction mechanism between hydrogen and grain boundary largely remains illusive. By uniaxial straining of bi-crystalline Ni with a Σ5(210)[001] grain bound...

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Vydané v:Scripta materialia Ročník 204; s. 114122
Hlavní autori: Ding, Yu, Yu, Haiyang, Zhao, Kai, Lin, Meichao, Xiao, Senbo, Ortiz, Michael, He, Jianying, Zhang, Zhiliang
Médium: Journal Article
Jazyk:English
Vydavateľské údaje: Elsevier Ltd 01.11.2021
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ISSN:1359-6462, 1872-8456, 1872-8456
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Abstract It is known that hydrogen can influence the dislocation plasticity and fracture mode transition of metallic materials, however, the nanoscale interaction mechanism between hydrogen and grain boundary largely remains illusive. By uniaxial straining of bi-crystalline Ni with a Σ5(210)[001] grain boundary, a transgranular to intergranular fracture transition facilitated by hydrogen is elucidated by atomistic modeling, and a specific hydrogen-controlled plasticity mechanism is revealed. Hydrogen is found to form a local atmosphere in the vicinity of grain boundary, which induces a local stress concentration and inhibits the subsequent stress relaxation at the grain boundary during deformation. It is this local stress concentration that promotes earlier dislocation emission, twinning evolution, and generation of more vacancies that facilitate nanovoiding. The nucleation and growth of nanovoids finally leads to intergranular fracture at the grain boundary, in contrast to the transgranular fracture of hydrogen-free sample. [Display omitted]
AbstractList It is known that hydrogen can influence the dislocation plasticity and fracture mode transition of metallic materials, however, the nanoscale interaction mechanism between hydrogen and grain boundary largely remains illusive. By uniaxial straining of bi-crystalline Ni with a Σ5(210)[001] grain boundary, a transgranular to intergranular fracture transition facilitated by hydrogen is elucidated by atomistic modeling, and a specific hydrogen-controlled plasticity mechanism is revealed. Hydrogen is found to form a local atmosphere in the vicinity of grain boundary, which induces a local stress concentration and inhibits the subsequent stress relaxation at the grain boundary during deformation. It is this local stress concentration that promotes earlier dislocation emission, twinning evolution, and generation of more vacancies that facilitate nanovoiding. The nucleation and growth of nanovoids finally leads to intergranular fracture at the grain boundary, in contrast to the transgranular fracture of hydrogen-free sample.
It is known that hydrogen can influence the dislocation plasticity and fracture mode transition of metallic materials, however, the nanoscale interaction mechanism between hydrogen and grain boundary largely remains illusive. By uniaxial straining of bi-crystalline Ni with a Σ5(210)[001] grain boundary, a transgranular to intergranular fracture transition facilitated by hydrogen is elucidated by atomistic modeling, and a specific hydrogen-controlled plasticity mechanism is revealed. Hydrogen is found to form a local atmosphere in the vicinity of grain boundary, which induces a local stress concentration and inhibits the subsequent stress relaxation at the grain boundary during deformation. It is this local stress concentration that promotes earlier dislocation emission, twinning evolution, and generation of more vacancies that facilitate nanovoiding. The nucleation and growth of nanovoids finally leads to intergranular fracture at the grain boundary, in contrast to the transgranular fracture of hydrogen-free sample. [Display omitted]
ArticleNumber 114122
Author Yu, Haiyang
He, Jianying
Zhao, Kai
Zhang, Zhiliang
Ding, Yu
Xiao, Senbo
Lin, Meichao
Ortiz, Michael
Author_xml – sequence: 1
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  surname: Ding
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  organization: Department of Structural Engineering, Norwegian University of Science and Technology (NTNU), Trondheim 7491, Norway
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  givenname: Haiyang
  orcidid: 0000-0002-2419-6736
  surname: Yu
  fullname: Yu, Haiyang
  organization: Division of Applied Mechanics, Department of Materials Science and Engineering, Uppsala University, Uppsala SE-75121, Sweden
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  givenname: Kai
  orcidid: 0000-0003-2645-7917
  surname: Zhao
  fullname: Zhao, Kai
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  givenname: Meichao
  surname: Lin
  fullname: Lin, Meichao
  organization: Department of Structural Engineering, Norwegian University of Science and Technology (NTNU), Trondheim 7491, Norway
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  givenname: Senbo
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  surname: Ortiz
  fullname: Ortiz, Michael
  organization: Graduate Aerospace Laboratories, California Institute of Technology, 1200 E. California Blvd., Pasadena, CA 91125, United States
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  givenname: Jianying
  surname: He
  fullname: He, Jianying
  organization: Department of Structural Engineering, Norwegian University of Science and Technology (NTNU), Trondheim 7491, Norway
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  givenname: Zhiliang
  surname: Zhang
  fullname: Zhang, Zhiliang
  email: zhiliang.zhang@ntnu.no
  organization: Department of Structural Engineering, Norwegian University of Science and Technology (NTNU), Trondheim 7491, Norway
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Keywords Molecular dynamics (MD)
Fracture
Hydrogen embrittlement
Grain boundary
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Snippet It is known that hydrogen can influence the dislocation plasticity and fracture mode transition of metallic materials, however, the nanoscale interaction...
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StartPage 114122
SubjectTerms Engineering Science with specialization in Solid Mechanics
Fracture
Grain boundary
Hydrogen embrittlement
Molecular dynamics (MD)
Teknisk fysik med inriktning mot hållfasthetslära
Title Hydrogen-induced transgranular to intergranular fracture transition in bi-crystalline nickel
URI https://dx.doi.org/10.1016/j.scriptamat.2021.114122
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