Improving the strength of polyethylene solids by simple controlling of the molecular weight distribution
We prepared model polyethylene (PE) samples that contain the controlled-amounts of the high-molecular-weight component by blending a monodispersed PE into a polydispersed PE, to elucidate the influence of the high-molecular-weight component of a polymer on its mechanical properties. The strength and...
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| Vydané v: | Polymer (Guilford) Ročník 218; s. 123526 |
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| Hlavní autori: | , , , , |
| Médium: | Journal Article |
| Jazyk: | English |
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Elsevier Ltd
18.03.2021
Elsevier BV |
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| ISSN: | 0032-3861, 1873-2291 |
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| Abstract | We prepared model polyethylene (PE) samples that contain the controlled-amounts of the high-molecular-weight component by blending a monodispersed PE into a polydispersed PE, to elucidate the influence of the high-molecular-weight component of a polymer on its mechanical properties. The strength and strain-hardening modulus were significantly enhanced by the addition of a monodispersed PE of sufficiently high molecular weight, and the critical value of Mw was determined to be ~3.0 × 105. The improved strength and strain-hardening modulus are attributed to higher amounts of inter-cluster links that bridge adjacent lamellar cluster units because these links act as stress transmitters between these units.
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•Model polyethylene (PE) samples with different shapes of molecular weight distribution were prepared by blending mono- and polydispersed PEs.•The strength and strain-hardening modulus were enhanced by adding a high-molecular-weight component with Mw > 3.0 × 105.•The improvement of tensile properties is attributed to larger amounts of inter-cluster links, which act as stress transmitters between lamellar cluster units. |
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| AbstractList | We prepared model polyethylene (PE) samples that contain the controlled-amounts of the high-molecular-weight component by blending a monodispersed PE into a polydispersed PE, to elucidate the influence of the high-molecular-weight component of a polymer on its mechanical properties. The strength and strain-hardening modulus were significantly enhanced by the addition of a monodispersed PE of sufficiently high molecular weight, and the critical value of Mw was determined to be ~3.0 × 105. The improved strength and strain-hardening modulus are attributed to higher amounts of inter-cluster links that bridge adjacent lamellar cluster units because these links act as stress transmitters between these units. We prepared model polyethylene (PE) samples that contain the controlled-amounts of the high-molecular-weight component by blending a monodispersed PE into a polydispersed PE, to elucidate the influence of the high-molecular-weight component of a polymer on its mechanical properties. The strength and strain-hardening modulus were significantly enhanced by the addition of a monodispersed PE of sufficiently high molecular weight, and the critical value of Mw was determined to be ~3.0 × 105. The improved strength and strain-hardening modulus are attributed to higher amounts of inter-cluster links that bridge adjacent lamellar cluster units because these links act as stress transmitters between these units. [Display omitted] •Model polyethylene (PE) samples with different shapes of molecular weight distribution were prepared by blending mono- and polydispersed PEs.•The strength and strain-hardening modulus were enhanced by adding a high-molecular-weight component with Mw > 3.0 × 105.•The improvement of tensile properties is attributed to larger amounts of inter-cluster links, which act as stress transmitters between lamellar cluster units. |
| ArticleNumber | 123526 |
| Author | Kida, Takumitsu Shiono, Takeshi Tanaka, Ryo Nitta, Koh-hei Hiejima, Yusuke |
| Author_xml | – sequence: 1 givenname: Takumitsu orcidid: 0000-0002-9494-3004 surname: Kida fullname: Kida, Takumitsu organization: Graduate School of Advanced Science and Engineering, Hiroshima University, Higashi-Hiroshima, 739-8527, Japan – sequence: 2 givenname: Ryo surname: Tanaka fullname: Tanaka, Ryo organization: Graduate School of Advanced Science and Engineering, Hiroshima University, Higashi-Hiroshima, 739-8527, Japan – sequence: 3 givenname: Yusuke surname: Hiejima fullname: Hiejima, Yusuke organization: Department of Chemical and Materials Science, Kanazawa University, Kakuma Campus, Kanazawa, 920-1192, Japan – sequence: 4 givenname: Koh-hei surname: Nitta fullname: Nitta, Koh-hei organization: Department of Chemical and Materials Science, Kanazawa University, Kakuma Campus, Kanazawa, 920-1192, Japan – sequence: 5 givenname: Takeshi surname: Shiono fullname: Shiono, Takeshi email: tshiono@hiroshima-u.ac.jp organization: Graduate School of Advanced Science and Engineering, Hiroshima University, Higashi-Hiroshima, 739-8527, Japan |
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| SubjectTerms | Clusters Mechanical properties Molecular weight Molecular weight distribution Polyethylene Polyethylenes Polymers Strain Strain hardening Tie molecules Transmitters |
| Title | Improving the strength of polyethylene solids by simple controlling of the molecular weight distribution |
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