Improving the strength of polyethylene solids by simple controlling of the molecular weight distribution

We prepared model polyethylene (PE) samples that contain the controlled-amounts of the high-molecular-weight component by blending a monodispersed PE into a polydispersed PE, to elucidate the influence of the high-molecular-weight component of a polymer on its mechanical properties. The strength and...

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Published in:	Polymer (Guilford) Vol. 218; p. 123526
Main Authors:	Kida, Takumitsu, Tanaka, Ryo, Hiejima, Yusuke, Nitta, Koh-hei, Shiono, Takeshi
Format:	Journal Article
Language:	English
Published:	Kidlington Elsevier Ltd 18.03.2021 Elsevier BV
Subjects:	Clusters Mechanical properties Molecular weight Molecular weight distribution Polyethylene Polyethylenes Polymers Strain Strain hardening Tie molecules Transmitters Tie molecules Mechanical properties Polyethylene Molecular weight distribution
ISSN:	0032-3861, 1873-2291
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Abstract	We prepared model polyethylene (PE) samples that contain the controlled-amounts of the high-molecular-weight component by blending a monodispersed PE into a polydispersed PE, to elucidate the influence of the high-molecular-weight component of a polymer on its mechanical properties. The strength and strain-hardening modulus were significantly enhanced by the addition of a monodispersed PE of sufficiently high molecular weight, and the critical value of Mw was determined to be ~3.0 × 105. The improved strength and strain-hardening modulus are attributed to higher amounts of inter-cluster links that bridge adjacent lamellar cluster units because these links act as stress transmitters between these units. [Display omitted] •Model polyethylene (PE) samples with different shapes of molecular weight distribution were prepared by blending mono- and polydispersed PEs.•The strength and strain-hardening modulus were enhanced by adding a high-molecular-weight component with Mw > 3.0 × 105.•The improvement of tensile properties is attributed to larger amounts of inter-cluster links, which act as stress transmitters between lamellar cluster units.
AbstractList	We prepared model polyethylene (PE) samples that contain the controlled-amounts of the high-molecular-weight component by blending a monodispersed PE into a polydispersed PE, to elucidate the influence of the high-molecular-weight component of a polymer on its mechanical properties. The strength and strain-hardening modulus were significantly enhanced by the addition of a monodispersed PE of sufficiently high molecular weight, and the critical value of Mw was determined to be ~3.0 × 105. The improved strength and strain-hardening modulus are attributed to higher amounts of inter-cluster links that bridge adjacent lamellar cluster units because these links act as stress transmitters between these units. We prepared model polyethylene (PE) samples that contain the controlled-amounts of the high-molecular-weight component by blending a monodispersed PE into a polydispersed PE, to elucidate the influence of the high-molecular-weight component of a polymer on its mechanical properties. The strength and strain-hardening modulus were significantly enhanced by the addition of a monodispersed PE of sufficiently high molecular weight, and the critical value of Mw was determined to be ~3.0 × 105. The improved strength and strain-hardening modulus are attributed to higher amounts of inter-cluster links that bridge adjacent lamellar cluster units because these links act as stress transmitters between these units. [Display omitted] •Model polyethylene (PE) samples with different shapes of molecular weight distribution were prepared by blending mono- and polydispersed PEs.•The strength and strain-hardening modulus were enhanced by adding a high-molecular-weight component with Mw > 3.0 × 105.•The improvement of tensile properties is attributed to larger amounts of inter-cluster links, which act as stress transmitters between lamellar cluster units.
ArticleNumber	123526
Author	Kida, Takumitsu Shiono, Takeshi Tanaka, Ryo Nitta, Koh-hei Hiejima, Yusuke
Author_xml	– sequence: 1 givenname: Takumitsu orcidid: 0000-0002-9494-3004 surname: Kida fullname: Kida, Takumitsu organization: Graduate School of Advanced Science and Engineering, Hiroshima University, Higashi-Hiroshima, 739-8527, Japan – sequence: 2 givenname: Ryo surname: Tanaka fullname: Tanaka, Ryo organization: Graduate School of Advanced Science and Engineering, Hiroshima University, Higashi-Hiroshima, 739-8527, Japan – sequence: 3 givenname: Yusuke surname: Hiejima fullname: Hiejima, Yusuke organization: Department of Chemical and Materials Science, Kanazawa University, Kakuma Campus, Kanazawa, 920-1192, Japan – sequence: 4 givenname: Koh-hei surname: Nitta fullname: Nitta, Koh-hei organization: Department of Chemical and Materials Science, Kanazawa University, Kakuma Campus, Kanazawa, 920-1192, Japan – sequence: 5 givenname: Takeshi surname: Shiono fullname: Shiono, Takeshi email: tshiono@hiroshima-u.ac.jp organization: Graduate School of Advanced Science and Engineering, Hiroshima University, Higashi-Hiroshima, 739-8527, Japan
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Snippet	We prepared model polyethylene (PE) samples that contain the controlled-amounts of the high-molecular-weight component by blending a monodispersed PE into a...
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SubjectTerms	Clusters Mechanical properties Molecular weight Molecular weight distribution Polyethylene Polyethylenes Polymers Strain Strain hardening Tie molecules Transmitters
Title	Improving the strength of polyethylene solids by simple controlling of the molecular weight distribution
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