Enhanced water flux through graphitic carbon nitride nanosheets membrane by incorporating polyacrylic acid

Membranes assembled from two‐dimensional (2‐D) layered materials have shown potential use in water purification. Recently, a 2‐D graphitic carbon nitride (g‐C3N4) nanosheets membrane exhibits considerable separation performance in water purification. In this study, to further improve this water sepa...

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Vydané v:	AIChE journal Ročník 64; číslo 6; s. 2181 - 2188
Hlavní autori:	Wang, Yanjie, Liu, Lingfei, Xue, Jian, Hou, Jiamin, Ding, Li, Wang, Haihui
Médium:	Journal Article
Jazyk:	English
Vydavateľské údaje:	New York American Institute of Chemical Engineers 01.06.2018
Predmet:	Antifouling Antifouling substances Carbon Carbon nitride Composite structures g‐C3N4 nanosheets Layered materials membrane Membranes modification Nanoparticles Nanosheets Polyacrylic acid Purification Rejection rate Separation Ultrafiltration Water purification
ISSN:	0001-1541, 1547-5905
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Abstract	Membranes assembled from two‐dimensional (2‐D) layered materials have shown potential use in water purification. Recently, a 2‐D graphitic carbon nitride (g‐C3N4) nanosheets membrane exhibits considerable separation performance in water purification. In this study, to further improve this water separation performance, polyacrylic acid (PAA) was introduced to tune the nanochannels formed between the g‐C3N4 nanosheets. The fabricated g‐C3N4‐PAA hybrid membranes possessed higher water flux without sacrificing much rejection rate compared with that of the g‐C3N4 membrane; however, noticeable fouling was observed upon addition of the PAA into the membrane composite structure. In addition, the effect of PAA on the morphology, surface hydrophilicity, separation performance, and antifouling properties of the g‐C3N4 membrane were examined in detail. Overall, incorporating PAA into the g‐C3N4 nanosheets membrane was an effective and convenient method to improve the water separation performance, which could promote the application of the 2‐D g‐C3N4 nanosheets membrane in practical ultrafiltration processes. © 2018 American Institute of Chemical Engineers AIChE J, 64: 2181–2188, 2018
AbstractList	Membranes assembled from two‐dimensional (2‐D) layered materials have shown potential use in water purification. Recently, a 2‐D graphitic carbon nitride (g‐C3N4) nanosheets membrane exhibits considerable separation performance in water purification. In this study, to further improve this water separation performance, polyacrylic acid (PAA) was introduced to tune the nanochannels formed between the g‐C3N4 nanosheets. The fabricated g‐C3N4‐PAA hybrid membranes possessed higher water flux without sacrificing much rejection rate compared with that of the g‐C3N4 membrane; however, noticeable fouling was observed upon addition of the PAA into the membrane composite structure. In addition, the effect of PAA on the morphology, surface hydrophilicity, separation performance, and antifouling properties of the g‐C3N4 membrane were examined in detail. Overall, incorporating PAA into the g‐C3N4 nanosheets membrane was an effective and convenient method to improve the water separation performance, which could promote the application of the 2‐D g‐C3N4 nanosheets membrane in practical ultrafiltration processes. © 2018 American Institute of Chemical Engineers AIChE J, 64: 2181–2188, 2018 Membranes assembled from two‐dimensional (2‐D) layered materials have shown potential use in water purification. Recently, a 2‐D graphitic carbon nitride (g‐C 3 N 4 ) nanosheets membrane exhibits considerable separation performance in water purification. In this study, to further improve this water separation performance, polyacrylic acid (PAA) was introduced to tune the nanochannels formed between the g‐C 3 N 4 nanosheets. The fabricated g‐C 3 N 4 ‐PAA hybrid membranes possessed higher water flux without sacrificing much rejection rate compared with that of the g‐C 3 N 4 membrane; however, noticeable fouling was observed upon addition of the PAA into the membrane composite structure. In addition, the effect of PAA on the morphology, surface hydrophilicity, separation performance, and antifouling properties of the g‐C 3 N 4 membrane were examined in detail. Overall, incorporating PAA into the g‐C 3 N 4 nanosheets membrane was an effective and convenient method to improve the water separation performance, which could promote the application of the 2‐D g‐C 3 N 4 nanosheets membrane in practical ultrafiltration processes. © 2018 American Institute of Chemical Engineers AIChE J , 64: 2181–2188, 2018
Author	Liu, Lingfei Xue, Jian Hou, Jiamin Wang, Yanjie Ding, Li Wang, Haihui
Author_xml	– sequence: 1 givenname: Yanjie surname: Wang fullname: Wang, Yanjie organization: South China University of Technology – sequence: 2 givenname: Lingfei surname: Liu fullname: Liu, Lingfei organization: South China University of Technology – sequence: 3 givenname: Jian surname: Xue fullname: Xue, Jian email: xuejian@scut.edu.cn organization: South China University of Technology – sequence: 4 givenname: Jiamin surname: Hou fullname: Hou, Jiamin organization: South China University of Technology – sequence: 5 givenname: Li surname: Ding fullname: Ding, Li organization: South China University of Technology – sequence: 6 givenname: Haihui orcidid: 0000-0002-2917-4739 surname: Wang fullname: Wang, Haihui email: hhwang@scut.edu.cn organization: South China University of Technology
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Snippet	Membranes assembled from two‐dimensional (2‐D) layered materials have shown potential use in water purification. Recently, a 2‐D graphitic carbon nitride... Membranes assembled from two‐dimensional (2‐D) layered materials have shown potential use in water purification. Recently, a 2‐D graphitic carbon nitride (g‐C...
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SubjectTerms	Antifouling Antifouling substances Carbon Carbon nitride Composite structures g‐C3N4 nanosheets Layered materials membrane Membranes modification Nanoparticles Nanosheets Polyacrylic acid Purification Rejection rate Separation Ultrafiltration Water purification
Title	Enhanced water flux through graphitic carbon nitride nanosheets membrane by incorporating polyacrylic acid
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