In situ electro-generated Ni(OH)2 synergistic with Cu cathode to promote direct ammonia oxidation to nitrogen

To solve the problem of low removal rate and poor N2 selectivity in direct electrochemical ammonia oxidation (EAO), commercial Ni foam and Cu foam were used as anode and cathode of the EAO system, respectively. The coupling effect between the cathode and anode promoted nitrogen cycling during the re...

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Vydáno v:Water science and technology Ročník 90; číslo 1; s. 225 - 237
Hlavní autoři: Xue, Yuzhou, Wang, Xuanxuan, Liu, Qing, Feng, Mengru, Ding, Zimo, Chu, Jiayue, Zhu, Wenyan, Liu, Na, Li, Zhichun
Médium: Journal Article
Jazyk:angličtina
Vydáno: England IWA Publishing 01.07.2024
Témata:
Ammonia - chemistry
Copper - chemistry
coupling effect
direct electrochemical ammonia oxidation
Electrochemical Techniques - methods
Electrodes
goose-raising wastewater
Hydroxides - chemistry
n2 selectivity
Nickel - chemistry
Nitrogen - chemistry
nitrogen cycle
Oxidation-Reduction
Waste Disposal, Fluid - methods
Wastewater - chemistry
Water Pollutants, Chemical - chemistry
selectivity
coupling effect
direct electrochemical ammonia oxidation
nitrogen cycle
goose-raising wastewater
N
ISSN:0273-1223, 1996-9732
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Abstract To solve the problem of low removal rate and poor N2 selectivity in direct electrochemical ammonia oxidation (EAO), commercial Ni foam and Cu foam were used as anode and cathode of the EAO system, respectively. The coupling effect between the cathode and anode promoted nitrogen cycling during the reaction process, which improved N2 selectivity of the reaction system and promoted it to achieve a high ammonia removal rate. This study showed that the thin Ni(OH)2 with oxygen vacancy formed on the surface of Ni foam anode played an effective role in the dimerization of intermediate products in ammonia oxidation to form N2. This electrochemical system was used to treat real goose wastewater containing 422.5 mg/L NH4+-N and 94.5 mg/L total organic carbon (TOC). After treatment, this electrochemical system achieved good performance with an ammonia removal rate of 87%, N2 selectivity of 77%, and TOC removal rate of 72%. Therefore, this simple and efficient system with Ni foam anode and Cu foam cathode is a promising method for treating ammonia nitrogen wastewater.
AbstractList To solve the problem of low removal rate and poor N selectivity in direct electrochemical ammonia oxidation (EAO), commercial Ni foam and Cu foam were used as anode and cathode of the EAO system, respectively. The coupling effect between the cathode and anode promoted nitrogen cycling during the reaction process, which improved N selectivity of the reaction system and promoted it to achieve a high ammonia removal rate. This study showed that the thin Ni(OH) with oxygen vacancy formed on the surface of Ni foam anode played an effective role in the dimerization of intermediate products in ammonia oxidation to form N . This electrochemical system was used to treat real goose wastewater containing 422.5 mg/L NH -N and 94.5 mg/L total organic carbon (TOC). After treatment, this electrochemical system achieved good performance with an ammonia removal rate of 87%, N selectivity of 77%, and TOC removal rate of 72%. Therefore, this simple and efficient system with Ni foam anode and Cu foam cathode is a promising method for treating ammonia nitrogen wastewater.
To solve the problem of low removal rate and poor N2 selectivity in direct electrochemical ammonia oxidation (EAO), commercial Ni foam and Cu foam were used as anode and cathode of the EAO system, respectively. The coupling effect between the cathode and anode promoted nitrogen cycling during the reaction process, which improved N2 selectivity of the reaction system and promoted it to achieve a high ammonia removal rate. This study showed that the thin Ni(OH)2 with oxygen vacancy formed on the surface of Ni foam anode played an effective role in the dimerization of intermediate products in ammonia oxidation to form N2. This electrochemical system was used to treat real goose wastewater containing 422.5 mg/L NH4+-N and 94.5 mg/L total organic carbon (TOC). After treatment, this electrochemical system achieved good performance with an ammonia removal rate of 87%, N2 selectivity of 77%, and TOC removal rate of 72%. Therefore, this simple and efficient system with Ni foam anode and Cu foam cathode is a promising method for treating ammonia nitrogen wastewater. HIGHLIGHTS The use of commercial electrodes has increased the practicality of this system.; The anode was responsible for the ammonia oxidation.; The cathode was responsible for the reduction of nitrate.; The nitrogen cycle between the electrodes enabled this system to achieve high performance.; The electrochemical system had achieved significant results in practical goose wastewater treatment.;
To solve the problem of low removal rate and poor N2 selectivity in direct electrochemical ammonia oxidation (EAO), commercial Ni foam and Cu foam were used as anode and cathode of the EAO system, respectively. The coupling effect between the cathode and anode promoted nitrogen cycling during the reaction process, which improved N2 selectivity of the reaction system and promoted it to achieve a high ammonia removal rate. This study showed that the thin Ni(OH)2 with oxygen vacancy formed on the surface of Ni foam anode played an effective role in the dimerization of intermediate products in ammonia oxidation to form N2. This electrochemical system was used to treat real goose wastewater containing 422.5 mg/L NH4+-N and 94.5 mg/L total organic carbon (TOC). After treatment, this electrochemical system achieved good performance with an ammonia removal rate of 87%, N2 selectivity of 77%, and TOC removal rate of 72%. Therefore, this simple and efficient system with Ni foam anode and Cu foam cathode is a promising method for treating ammonia nitrogen wastewater.To solve the problem of low removal rate and poor N2 selectivity in direct electrochemical ammonia oxidation (EAO), commercial Ni foam and Cu foam were used as anode and cathode of the EAO system, respectively. The coupling effect between the cathode and anode promoted nitrogen cycling during the reaction process, which improved N2 selectivity of the reaction system and promoted it to achieve a high ammonia removal rate. This study showed that the thin Ni(OH)2 with oxygen vacancy formed on the surface of Ni foam anode played an effective role in the dimerization of intermediate products in ammonia oxidation to form N2. This electrochemical system was used to treat real goose wastewater containing 422.5 mg/L NH4+-N and 94.5 mg/L total organic carbon (TOC). After treatment, this electrochemical system achieved good performance with an ammonia removal rate of 87%, N2 selectivity of 77%, and TOC removal rate of 72%. Therefore, this simple and efficient system with Ni foam anode and Cu foam cathode is a promising method for treating ammonia nitrogen wastewater.
To solve the problem of low removal rate and poor N2 selectivity in direct electrochemical ammonia oxidation (EAO), commercial Ni foam and Cu foam were used as anode and cathode of the EAO system, respectively. The coupling effect between the cathode and anode promoted nitrogen cycling during the reaction process, which improved N2 selectivity of the reaction system and promoted it to achieve a high ammonia removal rate. This study showed that the thin Ni(OH)2 with oxygen vacancy formed on the surface of Ni foam anode played an effective role in the dimerization of intermediate products in ammonia oxidation to form N2. This electrochemical system was used to treat real goose wastewater containing 422.5 mg/L NH4+-N and 94.5 mg/L total organic carbon (TOC). After treatment, this electrochemical system achieved good performance with an ammonia removal rate of 87%, N2 selectivity of 77%, and TOC removal rate of 72%. Therefore, this simple and efficient system with Ni foam anode and Cu foam cathode is a promising method for treating ammonia nitrogen wastewater.
Author Wang, Xuanxuan
Liu, Na
Li, Zhichun
Chu, Jiayue
Zhu, Wenyan
Feng, Mengru
Liu, Qing
Ding, Zimo
Xue, Yuzhou
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CitedBy_id crossref_primary_10_1007_s10008_025_06213_4
crossref_primary_10_1016_j_jallcom_2024_177286
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Keywords selectivity
coupling effect
direct electrochemical ammonia oxidation
nitrogen cycle
goose-raising wastewater
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Snippet To solve the problem of low removal rate and poor N2 selectivity in direct electrochemical ammonia oxidation (EAO), commercial Ni foam and Cu foam were used as...
To solve the problem of low removal rate and poor N selectivity in direct electrochemical ammonia oxidation (EAO), commercial Ni foam and Cu foam were used as...
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SubjectTerms Ammonia - chemistry
Copper - chemistry
coupling effect
direct electrochemical ammonia oxidation
Electrochemical Techniques - methods
Electrodes
goose-raising wastewater
Hydroxides - chemistry
n2 selectivity
Nickel - chemistry
Nitrogen - chemistry
nitrogen cycle
Oxidation-Reduction
Waste Disposal, Fluid - methods
Wastewater - chemistry
Water Pollutants, Chemical - chemistry
Title In situ electro-generated Ni(OH)2 synergistic with Cu cathode to promote direct ammonia oxidation to nitrogen
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