Experimental study of aging-induced cementation effect on permeability property of bentonites
In geological disposal for high-level radioactive waste, bentonites are planned to be used as the buffer material surrounding radioactive waste in Japan. Bentonite-based buffer material requires low water permeation for delaying contact between groundwater and the waste. Because of the extremely lon...
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| Vydané v: | IOP conference series. Earth and environmental science Ročník 1124; číslo 1; s. 12118 - 12125 |
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| Hlavní autori: | , , |
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01.01.2023
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| Abstract | In geological disposal for high-level radioactive waste, bentonites are planned to be used as the buffer material surrounding radioactive waste in Japan. Bentonite-based buffer material requires low water permeation for delaying contact between groundwater and the waste. Because of the extremely long half-lives of radionuclides of the waste, several barriers including the buffer material are designed to maintain workability of the geological disposal facility for tens of thousands of years. However, in the disposal circumstances with high water pressure, high temperature and various groundwater chemistries, occurrence of cementation and consequently property changes of the bentonite in the buffer are concerned. Few studies are available to understand the effect of cementation on bentonite properties because of the difficulties of simulating long-term alteration process experimentally. From the viewpoint of natural analogues, cementation process of the buffer may be regarded as part of formation process of bentonite ore. Thus, in this study, permeability tests were conducted on three kinds of Na-type bentonite ores with different geological ages from respectively, Japan, USA, and China to see the influence of cementation on permeability of bentonites. For comparison, undisturbed and reconstituted specimens were prepared. The results show that difference of hydraulic conductivities of the undisturbed and reconstituted specimens for each ore is less than one order, and this difference seems not to correlate with the geological age of the ores. From these results, the influence of cementation on the hydraulic properties of bentonite buffer seems small. It may also be a counteracted result by cementation effects in terms of restriction of the swelling of montmorillonite and blockage of water flow paths. |
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| AbstractList | In geological disposal for high-level radioactive waste, bentonites are planned to be used as the buffer material surrounding radioactive waste in Japan. Bentonite-based buffer material requires low water permeation for delaying contact between groundwater and the waste. Because of the extremely long half-lives of radionuclides of the waste, several barriers including the buffer material are designed to maintain workability of the geological disposal facility for tens of thousands of years. However, in the disposal circumstances with high water pressure, high temperature and various groundwater chemistries, occurrence of cementation and consequently property changes of the bentonite in the buffer are concerned. Few studies are available to understand the effect of cementation on bentonite properties because of the difficulties of simulating long-term alteration process experimentally. From the viewpoint of natural analogues, cementation process of the buffer may be regarded as part of formation process of bentonite ore. Thus, in this study, permeability tests were conducted on three kinds of Na-type bentonite ores with different geological ages from respectively, Japan, USA, and China to see the influence of cementation on permeability of bentonites. For comparison, undisturbed and reconstituted specimens were prepared. The results show that difference of hydraulic conductivities of the undisturbed and reconstituted specimens for each ore is less than one order, and this difference seems not to correlate with the geological age of the ores. From these results, the influence of cementation on the hydraulic properties of bentonite buffer seems small. It may also be a counteracted result by cementation effects in terms of restriction of the swelling of montmorillonite and blockage of water flow paths. |
| Author | Komine, H. Wang, H. Ito, D. |
| Author_xml | – sequence: 1 givenname: D. surname: Ito fullname: Ito, D. organization: Waseda University Research associate, , Japan – sequence: 2 givenname: H. surname: Wang fullname: Wang, H. organization: Waseda University Associate professor, , Japan – sequence: 3 givenname: H. surname: Komine fullname: Komine, H. organization: Waseda University Professor, , Japan |
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| Cites_doi | 10.1346/CCMN.1971.0190303 10.1180/claymin.1992.027.3.08 10.1139/t99-052 10.1016/j.enggeo.2013.06.013 10.1139/t04-016 10.1680/jgeot.19.P.088 10.1061/(ASCE)1090-0241(2008)134:4(497) 10.1007/s00015-015-0187-y 10.1016/j.pce.2008.10.024 10.3327/jnuce.5.103 10.1016/j.sandf.2022.101210 10.1139/t99-057 |
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| References | Pusch (EES_1124_1_012118bib1) 1992; 27 Karnland (EES_1124_1_012118bib7) 2008; 33 Abichou (EES_1124_1_012118bib10) 2004; 41 Alexander (EES_1124_1_012118bib14) 2015; 108 (EES_1124_1_012118bib22) 2018 EES_1124_1_012118bib4 Ito (EES_1124_1_012118bib20) Wang (EES_1124_1_012118bib21) 2021 Dixon (EES_1124_1_012118bib6) 1999; 36 Chen (EES_1124_1_012118bib12) 2021; 71 Komine (EES_1124_1_012118bib11) 2008; 134 Ogata (EES_1124_1_012118bib3) 1999; 5 Ito (EES_1124_1_012118bib23) 2020; 76 Mesri (EES_1124_1_012118bib5) 1971; 19 Ito (EES_1124_1_012118bib19) 2021 Tomita (EES_1124_1_012118bib18) 1990; 23 Ito (EES_1124_1_012118bib16) 1999; 38 Achari (EES_1124_1_012118bib9) 1999; 36 Ito (EES_1124_1_012118bib24) 2022 Wang (EES_1124_1_012118bib8) 2013; 164 Michell (EES_1124_1_012118bib13) 2005 Bremer (EES_1124_1_012118bib17) 2016 Pusch (EES_1124_1_012118bib15) 1983; TR83-16 (EES_1124_1_012118bib2) 1999 |
| References_xml | – volume: 19 start-page: 151 year: 1971 ident: EES_1124_1_012118bib5 article-title: Mechanisms controlling the permeability of clays publication-title: Clays and Clay Minerals doi: 10.1346/CCMN.1971.0190303 – volume: 76 start-page: 295 year: 2020 ident: EES_1124_1_012118bib23 article-title: Evaluating influience of cementation on swelling properties of bentonite buffer material based on the results of bentonite ores publication-title: Journal of Japan Society of Civil Engineers – volume: 27 start-page: 353 year: 1992 ident: EES_1124_1_012118bib1 article-title: Use of bentonite for isolation of radioactive waste products publication-title: Clay Minerals doi: 10.1180/claymin.1992.027.3.08 – volume: 36 start-page: 783 year: 1999 ident: EES_1124_1_012118bib9 article-title: Prediction of the hydraulic conductivity of clays using the electric double layer theory publication-title: Canadian Geotechnical Journal doi: 10.1139/t99-052 – volume: 164 start-page: 67 year: 2013 ident: EES_1124_1_012118bib8 article-title: Hydraulic conductivity and microstructure changes of compacted bentonite/sand mixture during hydration publication-title: Engineering Geology doi: 10.1016/j.enggeo.2013.06.013 – volume: 41 start-page: 698 year: 2004 ident: EES_1124_1_012118bib10 article-title: Network model for hydraulic conductivity of sand-bentonite mixtures publication-title: Canadian Geotechnical Journal doi: 10.1139/t04-016 – year: 2022 ident: EES_1124_1_012118bib24 article-title: Experimental study to elucidate cementation effect on swelling pressure and montmorillonite basal spacing of bentonite ore – volume: 71 start-page: 1071 year: 2021 ident: EES_1124_1_012118bib12 article-title: A model for hydraulic conductivity of compacted bentonite – inclusion of microstructure effects under confined wetting publication-title: Géotechnique doi: 10.1680/jgeot.19.P.088 – volume: 134 start-page: 497 year: 2008 ident: EES_1124_1_012118bib11 article-title: Theoretical equations on hydraulic conductivities of bentonite-based buffer and backfill for underground disposal of radioactive wastes publication-title: Journal of Geotechnical and Geoenvironmental Engineering doi: 10.1061/(ASCE)1090-0241(2008)134:4(497) – volume: 38 start-page: 181 year: 1999 ident: EES_1124_1_012118bib16 article-title: The study of genesis and formation condition of bentonite publication-title: Journal of the Clay Science Society of Japan – start-page: 99 year: 1999 ident: EES_1124_1_012118bib2 article-title: H12: project to establish the scientific and technical basis for HLW disposal in Japan -project overview report-JNC TN1400 – volume: 108 start-page: 75 year: 2015 ident: EES_1124_1_012118bib14 article-title: Natural analogues: studies of geological processes relevant to radioactive waste disposal in deep geological repositries publication-title: Swiss J Geosci doi: 10.1007/s00015-015-0187-y – volume: 33 start-page: S472 year: 2008 ident: EES_1124_1_012118bib7 article-title: Sealing ability of Wyoming bentonite pellets foreseen as buffer material – Laboratory results publication-title: Physics and Chemistry of the Earth doi: 10.1016/j.pce.2008.10.024 – volume: 5 start-page: 103 year: 1999 ident: EES_1124_1_012118bib3 article-title: Execution techniques for high level radioactive waste disposal: IV design and manufacturing procedure of engineered barriers publication-title: J. 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| Snippet | In geological disposal for high-level radioactive waste, bentonites are planned to be used as the buffer material surrounding radioactive waste in Japan.... |
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| SubjectTerms | Aging Aging (artificial) Aging (natural) Bentonite Buffers Cementation Flow paths Geology Groundwater High level radioactive wastes High temperature Hydraulic properties Minerals Montmorillonite Ores Permeability Permeability tests Radioactive waste disposal Radioactive wastes Radioisotopes Water flow Water pressure Workability |
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| Title | Experimental study of aging-induced cementation effect on permeability property of bentonites |
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