Flexible polydimethylsiloxane/multi-walled carbon nanotubes membranous metacomposites with negative permittivity

Metacomposites with negative electromagnetic parameters can be promising substitute for periodic metamaterials. In this paper, we devoted to fabricating flexible metacomposite films, which have great potential applications in the field of wearable cloaks, sensing, perfect absorption and stretchable...

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Vydáno v:	Polymer (Guilford) Ročník 125; s. 50 - 57
Hlavní autoři:	Sun, Kai, Xie, Peitao, Wang, Zhongyang, Su, Tongming, Shao, Qian, Ryu, JongEun, Zhang, Xihua, Guo, Jiang, Shankar, Akash, Li, Jianfeng, Fan, Runhua, Cao, Dapeng, Guo, Zhanhu
Médium:	Journal Article
Jazyk:	angličtina
Vydáno:	Kidlington Elsevier Ltd 08.09.2017 Elsevier BV
Témata:	Carbon Complex permittivity Conduction Conductivity Dielectric loss Dielectrics Electric dipoles Electronic devices Electronic equipment Flexible metamaterials Metacomposites Metamaterials Multi wall carbon nanotubes Nanocomposites Nanotechnology Nanotubes Negative permittivity Particulate composites Permittivity Polydimethylsiloxane Polymerization Silicone resins Transportation networks Wearable technology Negative permittivity Flexible metamaterials Metacomposites
ISSN:	0032-3861, 1873-2291
On-line přístup:	Získat plný text
Tagy:	Přidat tag Žádné tagy, Buďte první, kdo vytvoří štítek k tomuto záznamu!

Abstract	Metacomposites with negative electromagnetic parameters can be promising substitute for periodic metamaterials. In this paper, we devoted to fabricating flexible metacomposite films, which have great potential applications in the field of wearable cloaks, sensing, perfect absorption and stretchable electronic devices. The conductivity and the complex permittivity were investigated in flexible polydimethylsiloxane (PDMS)/multi-walled carbon nanotubes (MWCNTs) membranous nanocomposites, which were fabricated via in-situ polymerization process. With the increase of conductive one-dimension carbon nanotubes concentration, there was a percolation transition observed in conduction due to the formation of continuous networks. The dielectric dispersion behavior was also analyzed in the spectra of complex permittivity. It is indicated that the conduction and polarization make a combined effect on the dielectric loss in flexible PDMS/MWCNTs composites. The negative permittivity with a dielectric resonance was obtained, and was attributed to the induced electric dipoles. [Display omitted] •Flexible conductive polydimethylsiloxane metacomposites were prepared.•Negative permittivity was observed in the nanocomposites.•Induced electric dipoles attributed to the negative permittivity.
AbstractList	Metacomposites with negative electromagnetic parameters can be promising substitute for periodic metamaterials. In this paper, we devoted to fabricating flexible metacomposite films, which have great potential applications in the field of wearable cloaks, sensing, perfect absorption and stretchable electronic devices. The conductivity and the complex permittivity were investigated in flexible polydimethylsiloxane (PDMS)/multi-walled carbon nanotubes (MWCNTs) membranous nanocomposites, which were fabricated via in-situ polymerization process. With the increase of conductive one-dimension carbon nanotubes concentration, there was a percolation transition observed in conduction due to the formation of continuous networks. The dielectric dispersion behavior was also analyzed in the spectra of complex permittivity. It is indicated that the conduction and polarization make a combined effect on the dielectric loss in flexible PDMS/MWCNTs composites. The negative permittivity with a dielectric resonance was obtained, and was attributed to the induced electric dipoles. [Display omitted] •Flexible conductive polydimethylsiloxane metacomposites were prepared.•Negative permittivity was observed in the nanocomposites.•Induced electric dipoles attributed to the negative permittivity. Metacomposites with negative electromagnetic parameters can be promising substitute for periodic metamaterials. In this paper, we devoted to fabricating flexible metacomposite films, which have great potential applications in the field of wearable cloaks, sensing, perfect absorption and stretchable electronic devices. The conductivity and the complex permittivity were investigated in flexible polydimethylsiloxane (PDMS)/multi-walled carbon nanotubes (MWCNTs) membranous nanocomposites, which were fabricated via in-situ polymerization process. With the increase of conductive one-dimension carbon nanotubes concentration, there was a percolation transition observed in conduction due to the formation of continuous networks. The dielectric dispersion behavior was also analyzed in the spectra of complex permittivity. It is indicated that the conduction and polarization make a combined effect on the dielectric loss in flexible PDMS/MWCNTs composites. The negative permittivity with a dielectric resonance was obtained, and was attributed to the induced electric dipoles.
Author	Fan, Runhua Xie, Peitao Su, Tongming Zhang, Xihua Shankar, Akash Ryu, JongEun Li, Jianfeng Wang, Zhongyang Sun, Kai Cao, Dapeng Shao, Qian Guo, Zhanhu Guo, Jiang
Author_xml	– sequence: 1 givenname: Kai surname: Sun fullname: Sun, Kai organization: College of Ocean Science and Engineering, Shanghai Maritime University, Shanghai 201306, PR China – sequence: 2 givenname: Peitao surname: Xie fullname: Xie, Peitao organization: School of Materials Science and Engineering, Shandong University, Jinan, 250061, PR China – sequence: 3 givenname: Zhongyang surname: Wang fullname: Wang, Zhongyang organization: School of Materials Science and Engineering, Shandong University, Jinan, 250061, PR China – sequence: 4 givenname: Tongming surname: Su fullname: Su, Tongming organization: Integrated Composites Laboratory (ICL), Department of Chemical & Biomolecular Engineering, University of Tennessee, Knoxville, TN 37996, USA – sequence: 5 givenname: Qian surname: Shao fullname: Shao, Qian organization: College of Chemical and Environmental Engineering, Shandong University of Science and Technology, Qingdao 266590, PR China – sequence: 6 givenname: JongEun surname: Ryu fullname: Ryu, JongEun organization: Department of Mechanical Engineering, Indiana University-Purdue University Indianapolis, Indianapolis, IN 46202, USA – sequence: 7 givenname: Xihua surname: Zhang fullname: Zhang, Xihua organization: School of Materials Science and Engineering, Shandong University, Jinan, 250061, PR China – sequence: 8 givenname: Jiang surname: Guo fullname: Guo, Jiang organization: Integrated Composites Laboratory (ICL), Department of Chemical & Biomolecular Engineering, University of Tennessee, Knoxville, TN 37996, USA – sequence: 9 givenname: Akash surname: Shankar fullname: Shankar, Akash organization: Department of Mechanical Engineering, Indiana University-Purdue University Indianapolis, Indianapolis, IN 46202, USA – sequence: 10 givenname: Jianfeng surname: Li fullname: Li, Jianfeng organization: College of Chemical and Environmental Engineering, Shandong University of Science and Technology, Qingdao 266590, PR China – sequence: 11 givenname: Runhua surname: Fan fullname: Fan, Runhua email: rhfan@shmtu.edu.cn organization: College of Ocean Science and Engineering, Shanghai Maritime University, Shanghai 201306, PR China – sequence: 12 givenname: Dapeng surname: Cao fullname: Cao, Dapeng email: caodp@mail.buct.edu.cn organization: State Key Laboratory of Organic–Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029, China – sequence: 13 givenname: Zhanhu surname: Guo fullname: Guo, Zhanhu email: zguo10@utk.edu organization: Integrated Composites Laboratory (ICL), Department of Chemical & Biomolecular Engineering, University of Tennessee, Knoxville, TN 37996, USA
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Snippet	Metacomposites with negative electromagnetic parameters can be promising substitute for periodic metamaterials. In this paper, we devoted to fabricating...
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SubjectTerms	Carbon Complex permittivity Conduction Conductivity Dielectric loss Dielectrics Electric dipoles Electronic devices Electronic equipment Flexible metamaterials Metacomposites Metamaterials Multi wall carbon nanotubes Nanocomposites Nanotechnology Nanotubes Negative permittivity Particulate composites Permittivity Polydimethylsiloxane Polymerization Silicone resins Transportation networks Wearable technology
Title	Flexible polydimethylsiloxane/multi-walled carbon nanotubes membranous metacomposites with negative permittivity
URI	https://dx.doi.org/10.1016/j.polymer.2017.07.083 https://www.proquest.com/docview/1956486229
Volume	125
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