Transient photoinduced ‘hidden’ phase in a manganite

The control over phase transitions in complex oxides offers the possibility to control their electronic and structural properties. The discovery of a new route to ultrafast photoswitching of manganites via high-energy ‘hidden’ excited states offers the possibility of phase transitions free from ther...

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Published in:	Nature materials Vol. 10; no. 2; pp. 101 - 105
Main Authors:	Ichikawa, Hirohiko, Nozawa, Shunsuke, Sato, Tokushi, Tomita, Ayana, Ichiyanagi, Kouhei, Chollet, Matthieu, Guerin, Laurent, Dean, Nicky, Cavalleri, Andrea, Adachi, Shin-ichi, Arima, Taka-hisa, Sawa, Hiroshi, Ogimoto, Yasushi, Nakamura, Masao, Tamaki, Ryo, Miyano, Kenjiro, Koshihara, Shin-ya
Format:	Journal Article
Language:	English
Published:	London Nature Publishing Group UK 01.02.2011 Nature Publishing Group
Subjects:	Biomaterials Chemistry and Materials Science Condensed Matter Physics Diffraction Electronics letter Materials Science Nanotechnology Optical and Electronic Materials Particle physics Phase transitions Physics Thin films X-ray diffraction
ISSN:	1476-1122, 1476-4660, 1476-4660
Online Access:	Get full text
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Abstract	The control over phase transitions in complex oxides offers the possibility to control their electronic and structural properties. The discovery of a new route to ultrafast photoswitching of manganites via high-energy ‘hidden’ excited states offers the possibility of phase transitions free from thermal effects. Photoinduced phase transitions are of special interest in condensed matter physics 1 , 2 because they can be used to change complex macroscopic material properties on the ultrafast timescale. Cooperative interactions between microscopic degrees of freedom greatly enhance the number and nature of accessible states, making it possible to switch electronic, magnetic or structural properties in new ways 2 , 3 , 4 , 5 , 6 , 7 , 8 , 9 . Photons with high energies, of the order of electron volts, in particular are able to access electronic states that may differ greatly from states produced with stimuli close to equilibrium 10 . In this study we report the photoinduced change in the lattice structure of a charge and orbitally ordered Nd 0.5 Sr 0.5 MnO 3 thin film using picosecond time-resolved X-ray diffraction. The photoinduced state is structurally ordered, homogeneous, metastable and has crystallographic parameters different from any thermodynamically accessible state. A femtosecond time-resolved spectroscopic study shows the formation of an electronic gap in this state. In addition, the threshold-like behaviour and high efficiency in photo-generation yield of this gapped state highlight the important role of cooperative interactions in the formation process. These combined observations point towards a ‘hidden insulating phase’ distinct from that found in the hitherto known phase diagram.
AbstractList	The control over phase transitions in complex oxides offers the possibility to control their electronic and structural properties. The discovery of a new route to ultrafast photoswitching of manganites via high-energy ‘hidden’ excited states offers the possibility of phase transitions free from thermal effects. Photoinduced phase transitions are of special interest in condensed matter physics 1 , 2 because they can be used to change complex macroscopic material properties on the ultrafast timescale. Cooperative interactions between microscopic degrees of freedom greatly enhance the number and nature of accessible states, making it possible to switch electronic, magnetic or structural properties in new ways 2 , 3 , 4 , 5 , 6 , 7 , 8 , 9 . Photons with high energies, of the order of electron volts, in particular are able to access electronic states that may differ greatly from states produced with stimuli close to equilibrium 10 . In this study we report the photoinduced change in the lattice structure of a charge and orbitally ordered Nd 0.5 Sr 0.5 MnO 3 thin film using picosecond time-resolved X-ray diffraction. The photoinduced state is structurally ordered, homogeneous, metastable and has crystallographic parameters different from any thermodynamically accessible state. A femtosecond time-resolved spectroscopic study shows the formation of an electronic gap in this state. In addition, the threshold-like behaviour and high efficiency in photo-generation yield of this gapped state highlight the important role of cooperative interactions in the formation process. These combined observations point towards a ‘hidden insulating phase’ distinct from that found in the hitherto known phase diagram. Photoinduced phase transitions are of special interest in condensed matter physics because they can be used to change complex macroscopic material properties on the ultrafast timescale. Cooperative interactions between microscopic degrees of freedom greatly enhance the number and nature of accessible states, making it possible to switch electronic, magnetic or structural properties in new ways. Photons with high energies, of the order of electron volts, in particular are able to access electronic states that may differ greatly from states produced with stimuli close to equilibrium. In this study we report the photoinduced change in the lattice structure of a charge and orbitally ordered Nd(0.5)Sr(0.5)MnO(3) thin film using picosecond time-resolved X-ray diffraction. The photoinduced state is structurally ordered, homogeneous, metastable and has crystallographic parameters different from any thermodynamically accessible state. A femtosecond time-resolved spectroscopic study shows the formation of an electronic gap in this state. In addition, the threshold-like behaviour and high efficiency in photo-generation yield of this gapped state highlight the important role of cooperative interactions in the formation process. These combined observations point towards a 'hidden insulating phase' distinct from that found in the hitherto known phase diagram.Photoinduced phase transitions are of special interest in condensed matter physics because they can be used to change complex macroscopic material properties on the ultrafast timescale. Cooperative interactions between microscopic degrees of freedom greatly enhance the number and nature of accessible states, making it possible to switch electronic, magnetic or structural properties in new ways. Photons with high energies, of the order of electron volts, in particular are able to access electronic states that may differ greatly from states produced with stimuli close to equilibrium. In this study we report the photoinduced change in the lattice structure of a charge and orbitally ordered Nd(0.5)Sr(0.5)MnO(3) thin film using picosecond time-resolved X-ray diffraction. The photoinduced state is structurally ordered, homogeneous, metastable and has crystallographic parameters different from any thermodynamically accessible state. A femtosecond time-resolved spectroscopic study shows the formation of an electronic gap in this state. In addition, the threshold-like behaviour and high efficiency in photo-generation yield of this gapped state highlight the important role of cooperative interactions in the formation process. These combined observations point towards a 'hidden insulating phase' distinct from that found in the hitherto known phase diagram. Photoinduced phase transitions are of special interest in condensed matter physics because they can be used to change complex macroscopic material properties on the ultrafast timescale. Cooperative interactions between microscopic degrees of freedom greatly enhance the number and nature of accessible states, making it possible to switch electronic, magnetic or structural properties in new ways. Photons with high energies, of the order of electron volts, in particular are able to access electronic states that may differ greatly from states produced with stimuli close to equilibrium. In this study we report the photoinduced change in the lattice structure of a charge and orbitally ordered Nd(0.5)Sr(0.5)MnO(3) thin film using picosecond time-resolved X-ray diffraction. The photoinduced state is structurally ordered, homogeneous, metastable and has crystallographic parameters different from any thermodynamically accessible state. A femtosecond time-resolved spectroscopic study shows the formation of an electronic gap in this state. In addition, the threshold-like behaviour and high efficiency in photo-generation yield of this gapped state highlight the important role of cooperative interactions in the formation process. These combined observations point towards a 'hidden insulating phase' distinct from that found in the hitherto known phase diagram. Photoinduced phase transitions are of special interest in condensed matter physics because they can be used to change complex macroscopic material properties on the ultrafast timescale. Cooperative interactions between microscopic degrees of freedom greatly enhance the number and nature of accessible states, making it possible to switch electronic, magnetic or structural properties in new ways. Photons with high energies, of the order of electron volts, in particular are able to access electronic states that may differ greatly from states produced with stimuli close to equilibrium. In this study we report the photoinduced change in the lattice structure of a charge and orbitally ordered Nd0.5Sr0.5MnO3 thin film using picosecond time-resolved X-ray diffraction. The photoinduced state is structurally ordered, homogeneous, metastable and has crystallographic parameters different from any thermodynamically accessible state. A femtosecond time-resolved spectroscopic study shows the formation of an electronic gap in this state. In addition, the threshold-like behaviour and high efficiency in photo-generation yield of this gapped state highlight the important role of cooperative interactions in the formation process. These combined observations point towards a "hidden insulating phase" distinct from that found in the hitherto known phase diagram. [PUBLICATION ABSTRACT]
Author	Chollet, Matthieu Tamaki, Ryo Adachi, Shin-ichi Dean, Nicky Arima, Taka-hisa Guerin, Laurent Sato, Tokushi Ichiyanagi, Kouhei Miyano, Kenjiro Nakamura, Masao Koshihara, Shin-ya Sawa, Hiroshi Tomita, Ayana Ichikawa, Hirohiko Nozawa, Shunsuke Ogimoto, Yasushi Cavalleri, Andrea
Author_xml	– sequence: 1 givenname: Hirohiko surname: Ichikawa fullname: Ichikawa, Hirohiko organization: JST, ERATO – sequence: 2 givenname: Shunsuke surname: Nozawa fullname: Nozawa, Shunsuke organization: JST, ERATO, Photon Factory, Institute of Materials Structure Science, High Energy Accelerator Research Organization – sequence: 3 givenname: Tokushi surname: Sato fullname: Sato, Tokushi organization: JST, ERATO, Photon Factory, Institute of Materials Structure Science, High Energy Accelerator Research Organization, CREST & Department of Materials Science, JST, Tokyo Institute of Technology – sequence: 4 givenname: Ayana surname: Tomita fullname: Tomita, Ayana organization: JST, ERATO, CREST & Department of Materials Science, JST, Tokyo Institute of Technology – sequence: 5 givenname: Kouhei surname: Ichiyanagi fullname: Ichiyanagi, Kouhei organization: JST, ERATO, Present addresses: #609(7A2) Kiban Bldg., 5-1-5 Kashiwanoha, Kashiwa City, 277-8561, Chiba, Japan (K.I.); X-ray Science Division, Argonne National Lab., Argonne, Illinois 60439, USA (M.C.); European Synchrotron Radiation Facility (ESRF), 6 rue Jules Horowitz, BP220, 38043 Grenoble, France (L.G.); Department of Applied Physics, Nagoya University, Nagoya 464-8603, Japan (H.S.); Cross-Correlated Materials Research Group (CMRG), ASI, RIKEN, Wako, Saitama 351-0198, Japan (M.N.) – sequence: 6 givenname: Matthieu surname: Chollet fullname: Chollet, Matthieu organization: CREST & Department of Materials Science, JST, Tokyo Institute of Technology, Present addresses: #609(7A2) Kiban Bldg., 5-1-5 Kashiwanoha, Kashiwa City, 277-8561, Chiba, Japan (K.I.); X-ray Science Division, Argonne National Lab., Argonne, Illinois 60439, USA (M.C.); European Synchrotron Radiation Facility (ESRF), 6 rue Jules Horowitz, BP220, 38043 Grenoble, France (L.G.); Department of Applied Physics, Nagoya University, Nagoya 464-8603, Japan (H.S.); Cross-Correlated Materials Research Group (CMRG), ASI, RIKEN, Wako, Saitama 351-0198, Japan (M.N.) – sequence: 7 givenname: Laurent surname: Guerin fullname: Guerin, Laurent organization: JST, ERATO, Present addresses: #609(7A2) Kiban Bldg., 5-1-5 Kashiwanoha, Kashiwa City, 277-8561, Chiba, Japan (K.I.); X-ray Science Division, Argonne National Lab., Argonne, Illinois 60439, USA (M.C.); European Synchrotron Radiation Facility (ESRF), 6 rue Jules Horowitz, BP220, 38043 Grenoble, France (L.G.); Department of Applied Physics, Nagoya University, Nagoya 464-8603, Japan (H.S.); Cross-Correlated Materials Research Group (CMRG), ASI, RIKEN, Wako, Saitama 351-0198, Japan (M.N.) – sequence: 8 givenname: Nicky surname: Dean fullname: Dean, Nicky organization: Department of Physics, University of Oxford, Clarendon Laboratory – sequence: 9 givenname: Andrea surname: Cavalleri fullname: Cavalleri, Andrea organization: Department of Physics, University of Oxford, Clarendon Laboratory, Max Planck Research Group for Structural Dynamics, University of Hamburg, Center For Free Electron Laser Science – sequence: 10 givenname: Shin-ichi surname: Adachi fullname: Adachi, Shin-ichi organization: JST, ERATO, Photon Factory, Institute of Materials Structure Science, High Energy Accelerator Research Organization – sequence: 11 givenname: Taka-hisa surname: Arima fullname: Arima, Taka-hisa organization: Institute of Multidisciplinary Research for Advanced Materials, Tohoku University – sequence: 12 givenname: Hiroshi surname: Sawa fullname: Sawa, Hiroshi organization: Photon Factory, Institute of Materials Structure Science, High Energy Accelerator Research Organization, Present addresses: #609(7A2) Kiban Bldg., 5-1-5 Kashiwanoha, Kashiwa City, 277-8561, Chiba, Japan (K.I.); X-ray Science Division, Argonne National Lab., Argonne, Illinois 60439, USA (M.C.); European Synchrotron Radiation Facility (ESRF), 6 rue Jules Horowitz, BP220, 38043 Grenoble, France (L.G.); Department of Applied Physics, Nagoya University, Nagoya 464-8603, Japan (H.S.); Cross-Correlated Materials Research Group (CMRG), ASI, RIKEN, Wako, Saitama 351-0198, Japan (M.N.) – sequence: 13 givenname: Yasushi surname: Ogimoto fullname: Ogimoto, Yasushi organization: JST, CREST & Research Center for Advanced Science and Technology, University of Tokyo – sequence: 14 givenname: Masao surname: Nakamura fullname: Nakamura, Masao organization: JST, CREST & Research Center for Advanced Science and Technology, University of Tokyo, Present addresses: #609(7A2) Kiban Bldg., 5-1-5 Kashiwanoha, Kashiwa City, 277-8561, Chiba, Japan (K.I.); X-ray Science Division, Argonne National Lab., Argonne, Illinois 60439, USA (M.C.); European Synchrotron Radiation Facility (ESRF), 6 rue Jules Horowitz, BP220, 38043 Grenoble, France (L.G.); Department of Applied Physics, Nagoya University, Nagoya 464-8603, Japan (H.S.); Cross-Correlated Materials Research Group (CMRG), ASI, RIKEN, Wako, Saitama 351-0198, Japan (M.N.) – sequence: 15 givenname: Ryo surname: Tamaki fullname: Tamaki, Ryo organization: JST, CREST & Research Center for Advanced Science and Technology, University of Tokyo – sequence: 16 givenname: Kenjiro surname: Miyano fullname: Miyano, Kenjiro organization: JST, CREST & Research Center for Advanced Science and Technology, University of Tokyo – sequence: 17 givenname: Shin-ya surname: Koshihara fullname: Koshihara, Shin-ya email: skoshi@cms.titech.ac.jp organization: JST, ERATO, CREST & Department of Materials Science, JST, Tokyo Institute of Technology
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/21240287$$D View this record in MEDLINE/PubMed
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ContentType	Journal Article
Copyright	Springer Nature Limited 2010 Copyright Nature Publishing Group Feb 2011
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Snippet	The control over phase transitions in complex oxides offers the possibility to control their electronic and structural properties. The discovery of a new route... Photoinduced phase transitions are of special interest in condensed matter physics because they can be used to change complex macroscopic material properties...
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SubjectTerms	Biomaterials Chemistry and Materials Science Condensed Matter Physics Diffraction Electronics letter Materials Science Nanotechnology Optical and Electronic Materials Particle physics Phase transitions Physics Thin films X-ray diffraction
Title	Transient photoinduced ‘hidden’ phase in a manganite
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