Zeolitic Materials with Hierarchical Porous Structures

During the past several years, different kinds of hierarchical structured zeolitic materials have been synthesized due to their highly attractive properties, such as superior mass/heat transfer characteristics, lower restriction of the diffusion of reactants in the mesopores, and low pressure drop....

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Vydáno v:	Advanced materials (Weinheim) Ročník 23; číslo 22-23; s. 2602 - 2615
Hlavní autoři:	Lopez-Orozco, Sofia, Inayat, Amer, Schwab, Andreas, Selvam, Thangaraj, Schwieger, Wilhelm
Médium:	Journal Article
Jazyk:	angličtina
Vydáno:	Weinheim WILEY-VCH Verlag 17.06.2011 WILEY‐VCH Verlag
Témata:	Alkenes - chemistry Benzene - chemistry Catalysis Catalyst Foams Hierarchical zeolites Methanol - chemistry Phenol - chemistry Porosity Pressure Structured composites Zeolites - chemistry
ISSN:	0935-9648, 1521-4095, 1521-4095
On-line přístup:	Získat plný text
Tagy:	Přidat tag Žádné tagy, Buďte první, kdo vytvoří štítek k tomuto záznamu!

Abstract	During the past several years, different kinds of hierarchical structured zeolitic materials have been synthesized due to their highly attractive properties, such as superior mass/heat transfer characteristics, lower restriction of the diffusion of reactants in the mesopores, and low pressure drop. Our contribution provides general information regarding types and preparation methods of hierarchical zeolitic materials and their relative advantages and disadvantages. Thereafter, recent advances in the preparation and characterization of hierarchical zeolitic structures within the crystallites by post‐synthetic treatment methods, such as dealumination or desilication; and structured devices by in situ and ex situ zeolite coatings on open‐cellular ceramic foams as (non‐reactive as well as reactive) supports are highlighted. Specific advantages of using hierarchical zeolitic catalysts/structures in selected catalytic reactions, such as benzene to phenol (BTOP) and methanol to olefins (MTO) are presented. Hierarchical zeolitic materials have attractive properties, such as superior mass/heat transfer characteristics, lower restriction of the diffusion of the reactants in the mesopores, and low pressure drop. Our Progress Report provides general information about the recent advances in the preparation and characterization of hierarchical zeolitic structures combining two (e.g., micro–meso, micro–macro) or even three (micro–meso–macro) levels of porosity.
AbstractList	During the past several years, different kinds of hierarchical structured zeolitic materials have been synthesized due to their highly attractive properties, such as superior mass/heat transfer characteristics, lower restriction of the diffusion of reactants in the mesopores, and low pressure drop. Our contribution provides general information regarding types and preparation methods of hierarchical zeolitic materials and their relative advantages and disadvantages. Thereafter, recent advances in the preparation and characterization of hierarchical zeolitic structures within the crystallites by post‐synthetic treatment methods, such as dealumination or desilication; and structured devices by in situ and ex situ zeolite coatings on open‐cellular ceramic foams as (non‐reactive as well as reactive) supports are highlighted. Specific advantages of using hierarchical zeolitic catalysts/structures in selected catalytic reactions, such as benzene to phenol (BTOP) and methanol to olefins (MTO) are presented. During the past several years, different kinds of hierarchical structured zeolitic materials have been synthesized due to their highly attractive properties, such as superior mass/heat transfer characteristics, lower restriction of the diffusion of reactants in the mesopores, and low pressure drop. Our contribution provides general information regarding types and preparation methods of hierarchical zeolitic materials and their relative advantages and disadvantages. Thereafter, recent advances in the preparation and characterization of hierarchical zeolitic structures within the crystallites by post‐synthetic treatment methods, such as dealumination or desilication; and structured devices by in situ and ex situ zeolite coatings on open‐cellular ceramic foams as (non‐reactive as well as reactive) supports are highlighted. Specific advantages of using hierarchical zeolitic catalysts/structures in selected catalytic reactions, such as benzene to phenol (BTOP) and methanol to olefins (MTO) are presented. Hierarchical zeolitic materials have attractive properties, such as superior mass/heat transfer characteristics, lower restriction of the diffusion of the reactants in the mesopores, and low pressure drop. Our Progress Report provides general information about the recent advances in the preparation and characterization of hierarchical zeolitic structures combining two (e.g., micro–meso, micro–macro) or even three (micro–meso–macro) levels of porosity. During the past several years, different kinds of hierarchical structured zeolitic materials have been synthesized due to their highly attractive properties, such as superior mass/heat transfer characteristics, lower restriction of the diffusion of reactants in the mesopores, and low pressure drop. Our contribution provides general information regarding types and preparation methods of hierarchical zeolitic materials and their relative advantages and disadvantages. Thereafter, recent advances in the preparation and characterization of hierarchical zeolitic structures within the crystallites by post-synthetic treatment methods, such as dealumination or desilication; and structured devices by in situ and ex situ zeolite coatings on open-cellular ceramic foams as (non-reactive as well as reactive) supports are highlighted. Specific advantages of using hierarchical zeolitic catalysts/structures in selected catalytic reactions, such as benzene to phenol (BTOP) and methanol to olefins (MTO) are presented.During the past several years, different kinds of hierarchical structured zeolitic materials have been synthesized due to their highly attractive properties, such as superior mass/heat transfer characteristics, lower restriction of the diffusion of reactants in the mesopores, and low pressure drop. Our contribution provides general information regarding types and preparation methods of hierarchical zeolitic materials and their relative advantages and disadvantages. Thereafter, recent advances in the preparation and characterization of hierarchical zeolitic structures within the crystallites by post-synthetic treatment methods, such as dealumination or desilication; and structured devices by in situ and ex situ zeolite coatings on open-cellular ceramic foams as (non-reactive as well as reactive) supports are highlighted. Specific advantages of using hierarchical zeolitic catalysts/structures in selected catalytic reactions, such as benzene to phenol (BTOP) and methanol to olefins (MTO) are presented.
Author	Lopez-Orozco, Sofia Inayat, Amer Schwab, Andreas Selvam, Thangaraj Schwieger, Wilhelm
Author_xml	– sequence: 1 givenname: Sofia surname: Lopez-Orozco fullname: Lopez-Orozco, Sofia organization: Friedrich-Alexander-Universität Erlangen-Nürnberg, CRT, Egerlandstraße 3, 91058 Erlangen, Germany – sequence: 2 givenname: Amer surname: Inayat fullname: Inayat, Amer organization: Friedrich-Alexander-Universität Erlangen-Nürnberg, CRT, Egerlandstraße 3, 91058 Erlangen, Germany – sequence: 3 givenname: Andreas surname: Schwab fullname: Schwab, Andreas organization: Friedrich-Alexander-Universität Erlangen-Nürnberg, CRT, Egerlandstraße 3, 91058 Erlangen, Germany – sequence: 4 givenname: Thangaraj surname: Selvam fullname: Selvam, Thangaraj organization: Friedrich-Alexander-Universität Erlangen-Nürnberg, CRT, Egerlandstraße 3, 91058 Erlangen, Germany – sequence: 5 givenname: Wilhelm surname: Schwieger fullname: Schwieger, Wilhelm email: Wilhelm.Schwieger@crt.cbi.uni-erlangen.de organization: Friedrich-Alexander-Universität Erlangen-Nürnberg, CRT, Egerlandstraße 3, 91058 Erlangen, Germany
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/21495091$$D View this record in MEDLINE/PubMed
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Snippet	During the past several years, different kinds of hierarchical structured zeolitic materials have been synthesized due to their highly attractive properties,...
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SubjectTerms	Alkenes - chemistry Benzene - chemistry Catalysis Catalyst Foams Hierarchical zeolites Methanol - chemistry Phenol - chemistry Porosity Pressure Structured composites Zeolites - chemistry
Title	Zeolitic Materials with Hierarchical Porous Structures
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