Selective Adsorption and Separation of Xylene Isomers and Ethylbenzene with the Microporous Vanadium(IV) Terephthalate MIL-47

A breakthrough result: The microporous metal–organic framework MIL‐47 is an excellent adsorbent for the separation of C8 alkylaromatic compounds, such as ethylbenzene, meta‐xylene, and para‐xylene. The potential of MIL‐47, with its high uptake capacity and its hydrophobic nature, for real separation...

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Vydáno v:	Angewandte Chemie International Edition Ročník 46; číslo 23; s. 4293 - 4297
Hlavní autoři:	Alaerts, Luc, Kirschhock, Christine E. A., Maes, Michael, van der Veen, Monique A., Finsy, Vincent, Depla, Anouschka, Martens, Johan A., Baron, Gino V., Jacobs, Pierre A., Denayer, Joeri F. M., De Vos, Dirk E.
Médium:	Journal Article
Jazyk:	angličtina
Vydáno:	Weinheim WILEY-VCH Verlag 01.01.2007 WILEY‐VCH Verlag
Témata:	Adsorption Benzene Derivatives - chemistry host-guest systems Isomerism liquid chromatography metal-organic frameworks microporous materials Organometallic Compounds - chemistry Porosity Surface Properties Xylenes - chemistry
ISSN:	1433-7851, 1521-3773
On-line přístup:	Získat plný text
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Abstract	A breakthrough result: The microporous metal–organic framework MIL‐47 is an excellent adsorbent for the separation of C8 alkylaromatic compounds, such as ethylbenzene, meta‐xylene, and para‐xylene. The potential of MIL‐47, with its high uptake capacity and its hydrophobic nature, for real separations of the C8 alkylaromatic compounds was demonstrated by breakthrough and chromatographic experiments (see picture).
AbstractList	A breakthrough result: The microporous metal–organic framework MIL‐47 is an excellent adsorbent for the separation of C8 alkylaromatic compounds, such as ethylbenzene, meta‐xylene, and para‐xylene. The potential of MIL‐47, with its high uptake capacity and its hydrophobic nature, for real separations of the C8 alkylaromatic compounds was demonstrated by breakthrough and chromatographic experiments (see picture).
Author	Kirschhock, Christine E. A. Denayer, Joeri F. M. van der Veen, Monique A. Depla, Anouschka Finsy, Vincent Maes, Michael Baron, Gino V. Alaerts, Luc Martens, Johan A. Jacobs, Pierre A. De Vos, Dirk E.
Author_xml	– sequence: 1 givenname: Luc surname: Alaerts fullname: Alaerts, Luc organization: Centre for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Leuven, Belgium, Fax: (+32) 16-321-998 – sequence: 2 givenname: Christine E. A. surname: Kirschhock fullname: Kirschhock, Christine E. A. organization: Centre for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Leuven, Belgium, Fax: (+32) 16-321-998 – sequence: 3 givenname: Michael surname: Maes fullname: Maes, Michael organization: Centre for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Leuven, Belgium, Fax: (+32) 16-321-998 – sequence: 4 givenname: Monique A. surname: van der Veen fullname: van der Veen, Monique A. organization: Centre for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Leuven, Belgium, Fax: (+32) 16-321-998 – sequence: 5 givenname: Vincent surname: Finsy fullname: Finsy, Vincent organization: Department of Chemical Engineering, Vrije Universiteit Brussel, Pleinlaan 2, 1050 Brussel, Belgium – sequence: 6 givenname: Anouschka surname: Depla fullname: Depla, Anouschka organization: Centre for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Leuven, Belgium, Fax: (+32) 16-321-998 – sequence: 7 givenname: Johan A. surname: Martens fullname: Martens, Johan A. organization: Centre for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Leuven, Belgium, Fax: (+32) 16-321-998 – sequence: 8 givenname: Gino V. surname: Baron fullname: Baron, Gino V. organization: Department of Chemical Engineering, Vrije Universiteit Brussel, Pleinlaan 2, 1050 Brussel, Belgium – sequence: 9 givenname: Pierre A. surname: Jacobs fullname: Jacobs, Pierre A. organization: Centre for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Leuven, Belgium, Fax: (+32) 16-321-998 – sequence: 10 givenname: Joeri F. M. surname: Denayer fullname: Denayer, Joeri F. M. organization: Department of Chemical Engineering, Vrije Universiteit Brussel, Pleinlaan 2, 1050 Brussel, Belgium – sequence: 11 givenname: Dirk E. surname: De Vos fullname: De Vos, Dirk E. email: dirk.devos@biw.kuleuven.be organization: Centre for Surface Chemistry and Catalysis, Katholieke Universiteit Leuven, Kasteelpark Arenberg 23, 3001 Leuven, Belgium, Fax: (+32) 16-321-998
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Notes	istex:74902D24FAC9F9CC07AFE0EB563E5FDFCAC6B16C ark:/67375/WNG-ZZFFFJNC-T L.A. and J.D. are grateful to F.W.O.-Vlaanderen (Research Foundation-Flanders) for positions as a research assistant and post-doctoral researcher, respectively. This work was performed in the frame of the IAP Functional Supramolecular Systems of the Belgian Federal Government. Belgian Federal Government ArticleID:ANIE200700056 L.A. and J.D. are grateful to F.W.O.‐Vlaanderen (Research Foundation—Flanders) for positions as a research assistant and post‐doctoral researcher, respectively. This work was performed in the frame of the IAP Functional Supramolecular Systems of the Belgian Federal Government. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23
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Snippet	A breakthrough result: The microporous metal–organic framework MIL‐47 is an excellent adsorbent for the separation of C8 alkylaromatic compounds, such as...
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SubjectTerms	Adsorption Benzene Derivatives - chemistry host-guest systems Isomerism liquid chromatography metal-organic frameworks microporous materials Organometallic Compounds - chemistry Porosity Surface Properties Xylenes - chemistry
Title	Selective Adsorption and Separation of Xylene Isomers and Ethylbenzene with the Microporous Vanadium(IV) Terephthalate MIL-47
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