Recent progress in syngas production via catalytic CO2 hydrogenation reaction

[Display omitted] •Recent advances in catalyst design for the RWGS reaction are studied.•CO adsorption energy in transition metals may affect their CO2 hydrogenation product selectivity.•Different reaction mechanisms for the RWGS reaction are proposed.•Electron density, catalyst structure, and the p...

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Vydáno v:	Applied catalysis. B, Environmental Ročník 295; s. 120319
Hlavní autoři:	Bahmanpour, Ali M., Signorile, Matteo, Kröcher, Oliver
Médium:	Journal Article
Jazyk:	angličtina
Vydáno:	Amsterdam Elsevier B.V 15.10.2021 Elsevier BV
Témata:	Carbon dioxide Catalyst design Catalysts CO2 hydrogenation Gas production High temperature Noble metals Oil and gas production Reaction mechanisms Reaction synthesis Reverse water-gas shift reaction Selectivity Stability Synthesis gas Catalyst design Synthesis gas Reverse water-gas shift reaction CO2 hydrogenation
ISSN:	0926-3373, 1873-3883
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Abstract	[Display omitted] •Recent advances in catalyst design for the RWGS reaction are studied.•CO adsorption energy in transition metals may affect their CO2 hydrogenation product selectivity.•Different reaction mechanisms for the RWGS reaction are proposed.•Electron density, catalyst structure, and the presence of hydroxyl groups are vital for catalyst design. Synthesis gas production through the catalytic reverse water-gas shift (RWGS) reaction is an attractive option for the conversion of CO2 to fuels. Many metal-based catalysts have been introduced for this reaction in order to provide high activity, CO selectivity, and stability. Recently, progress has been made in catalyst design and understanding of the reaction mechanism, which has shed light on the characteristics of the catalysts needed for this reaction. Accordingly, new noble and non-noble metal-based catalysts with remarkable performance have been introduced for this reaction. However, there is still much room for catalyst improvement specifically in regard to catalyst stability at the high temperatures required for this reaction. There are also controversial arguments regarding the active sites of the reaction. This review highlights the recent progress in catalyst design and understanding of the reaction mechanism for the RWGS reaction and derives proposals for further improvements of the process.
AbstractList	Synthesis gas production through the catalytic reverse water-gas shift (RWGS) reaction is an attractive option for the conversion of CO2 to fuels. Many metal-based catalysts have been introduced for this reaction in order to provide high activity, CO selectivity, and stability. Recently, progress has been made in catalyst design and understanding of the reaction mechanism, which has shed light on the characteristics of the catalysts needed for this reaction. Accordingly, new noble and non-noble metal-based catalysts with remarkable performance have been introduced for this reaction. However, there is still much room for catalyst improvement specifically in regard to catalyst stability at the high temperatures required for this reaction. There are also controversial arguments regarding the active sites of the reaction. This review highlights the recent progress in catalyst design and understanding of the reaction mechanism for the RWGS reaction and derives proposals for further improvements of the process. [Display omitted] •Recent advances in catalyst design for the RWGS reaction are studied.•CO adsorption energy in transition metals may affect their CO2 hydrogenation product selectivity.•Different reaction mechanisms for the RWGS reaction are proposed.•Electron density, catalyst structure, and the presence of hydroxyl groups are vital for catalyst design. Synthesis gas production through the catalytic reverse water-gas shift (RWGS) reaction is an attractive option for the conversion of CO2 to fuels. Many metal-based catalysts have been introduced for this reaction in order to provide high activity, CO selectivity, and stability. Recently, progress has been made in catalyst design and understanding of the reaction mechanism, which has shed light on the characteristics of the catalysts needed for this reaction. Accordingly, new noble and non-noble metal-based catalysts with remarkable performance have been introduced for this reaction. However, there is still much room for catalyst improvement specifically in regard to catalyst stability at the high temperatures required for this reaction. There are also controversial arguments regarding the active sites of the reaction. This review highlights the recent progress in catalyst design and understanding of the reaction mechanism for the RWGS reaction and derives proposals for further improvements of the process.
ArticleNumber	120319
Author	Kröcher, Oliver Signorile, Matteo Bahmanpour, Ali M.
Author_xml	– sequence: 1 givenname: Ali M. orcidid: 0000-0003-2092-9215 surname: Bahmanpour fullname: Bahmanpour, Ali M. organization: Institute of Chemical Sciences and Engineering, École Polytechnique Fédérale de Lausanne (EPFL), 1015, Lausanne, Switzerland – sequence: 2 givenname: Matteo surname: Signorile fullname: Signorile, Matteo organization: Department of Chemistry, NIS Centre and INSTM Reference Center, University of Turin, via P. Giuria 7, 10125, Turin, Italy – sequence: 3 givenname: Oliver orcidid: 0000-0002-7268-7257 surname: Kröcher fullname: Kröcher, Oliver email: oliver.kroecher@psi.ch organization: Institute of Chemical Sciences and Engineering, École Polytechnique Fédérale de Lausanne (EPFL), 1015, Lausanne, Switzerland
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Snippet	[Display omitted] •Recent advances in catalyst design for the RWGS reaction are studied.•CO adsorption energy in transition metals may affect their CO2... Synthesis gas production through the catalytic reverse water-gas shift (RWGS) reaction is an attractive option for the conversion of CO2 to fuels. Many...
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SubjectTerms	Carbon dioxide Catalyst design Catalysts CO2 hydrogenation Gas production High temperature Noble metals Oil and gas production Reaction mechanisms Reaction synthesis Reverse water-gas shift reaction Selectivity Stability Synthesis gas
Title	Recent progress in syngas production via catalytic CO2 hydrogenation reaction
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