Winter air pollution by and inhalation exposure to nitrated and oxygenated PAHs in rural Shanxi, north China

Polar polycyclic aromatic hydrocarbons (PAHs) derivatives like nitrated and oxygenated PAHs have higher toxic potentials than the parent one, and are receiving growing interests. In this study, we investigated household air pollution and personal exposure to nitro- and oxy-PAHs during a winter perio...

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Veröffentlicht in:Atmospheric environment (1994) Jg. 187; S. 210 - 217
Hauptverfasser: Du, Wei, Chen, Yuanchen, Shen, Guofeng, Wang, Wei, Zhuo, Shaojie, Huang, Ye, Pan, Xuelian, Tao, Shu
Format: Journal Article
Sprache:Englisch
Veröffentlicht: Elsevier Ltd 01.08.2018
Elsevier
Schlagworte:
air
Air pollution
atmospheric chemistry
burning
China
Continental interfaces, environment
cooking
Inhalation exposure
Nitrated PAHs
Ocean, Atmosphere
Oxygenated PAHs
particulates
polycyclic aromatic hydrocarbons
rural areas
Rural China
rural population
samplers
Sciences of the Universe
Size distribution
time-weighted average
toxicity
winter
wood
China
Air pollution
Size distribution
Inhalation exposure
Rural China
Nitrated PAHs
Oxygenated PAHs
ISSN:1352-2310, 1873-2844
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Zusammenfassung:Polar polycyclic aromatic hydrocarbons (PAHs) derivatives like nitrated and oxygenated PAHs have higher toxic potentials than the parent one, and are receiving growing interests. In this study, we investigated household air pollution and personal exposure to nitro- and oxy-PAHs during a winter period in rural Shanxi, northern China. The overall arithmetic means of 24-h average indoor nitro-PAHs and oxy-PAHs were 10.2 ± 3.6 and 76.8 ± 51.8 ng/m3, respectively, that were much higher than the 7.98 ± 4.30 and 54.7 ± 45.4 ng/m3 in the outdoor air. Nearly 90% of particulate PAHs derivatives were enriched in fine PM2.5 and even finer PM1.0 fraction. Daily inhalation exposure to nitro- and oxy-PAHs for the rural population were 8.41 ± 3.08 and 68.5 ± 79.7 ng/m3, respectively. Residents burning briquette for cooking were found to have lower household air pollution and exposure levels compared with those burning wood. The calculated time-weighted average concentration overestimated, though correlated positively, the daily inhalation exposure compared to the that from personal carried samplers. [Display omitted] •Nitrated and oxygenated PAHs in paired indoor-outdoor rural households.•Inhalation exposure to PAHs derivatives using portable samplers.•Enrichment in fine and sub-micron particle fractions.•Substantial discrepancy between the time-weighted average concentration and directly measured exposure.•Lower pollution in homes burning briquettes for cooking compared to the use of wood combustion.
Bibliographie:ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
ISSN:1352-2310
1873-2844
DOI:10.1016/j.atmosenv.2018.06.004