Room‐Temperature Magnetic Skyrmions and Large Topological Hall Effect in Chromium Telluride Engineered by Self‐Intercalation

Room‐temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano‐spintronic devices. However, such skyrmion‐hosting materials are rare in nature. In this study, a self‐intercalated transition metal dichalcogenide Cr1+xTe2 with a layered crystal...

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Published in:Advanced materials (Weinheim) Vol. 35; no. 1; pp. e2205967 - n/a
Main Authors: Zhang, Chenhui, Liu, Chen, Zhang, Junwei, Yuan, Youyou, Wen, Yan, Li, Yan, Zheng, Dongxing, Zhang, Qiang, Hou, Zhipeng, Yin, Gen, Liu, Kai, Peng, Yong, Zhang, Xi‐Xiang
Format: Journal Article
Language:English
Published: Germany Wiley Subscription Services, Inc 01.01.2023
Subjects:
Chromium
chromium telluride
Crystal structure
Curie temperature
Electromagnetism
Hall effect
Hypothetical particles
Intercalation
layered materials
Low temperature
Magnetic anisotropy
magnetic skyrmions
Magnetism
Materials science
Particle theory
self‐intercalation
Tellurides
Temperature
topological Hall effect
Topology
Transition metal compounds
chromium telluride
topological Hall effect
layered materials
self-intercalation
magnetic skyrmions
ISSN:0935-9648, 1521-4095, 1521-4095
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Abstract Room‐temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano‐spintronic devices. However, such skyrmion‐hosting materials are rare in nature. In this study, a self‐intercalated transition metal dichalcogenide Cr1+xTe2 with a layered crystal structure that hosts room‐temperature skyrmions and exhibits large THE is reported. By tuning the self‐intercalate concentration, a monotonic control of Curie temperature from 169 to 333 K and a magnetic anisotropy transition from out‐of‐plane to the in‐plane configuration are achieved. Based on the intercalation engineering, room‐temperature skyrmions are successfully created in Cr1.53Te2 with a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy. Remarkably, a skyrmion‐induced topological Hall resistivity as large as ≈106 nΩ cm is observed at 290 K. Moreover, a sign reversal of THE is also found at low temperatures, which can be ascribed to other topological spin textures having an opposite topological charge to that of the skyrmions. Therefore, chromium telluride can be a new paradigm of the skyrmion material family with promising prospects for future device applications. Magnetic skyrmions and large topological Hall effect are demonstrated in chromium telluride. The Curie temperature and magnetic anisotropy in Cr1+xTe2 can be controlled by the self‐intercalate concentration x. In Cr1.53Te2, which has a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy, room‐temperature skyrmions and topological Hall resistivity as large as ≈106 nΩ cm are observed.
AbstractList Room-temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano-spintronic devices. However, such skyrmion-hosting materials are rare in nature. In this study, a self-intercalated transition metal dichalcogenide Cr1+ x Te2 with a layered crystal structure that hosts room-temperature skyrmions and exhibits large THE is reported. By tuning the self-intercalate concentration, a monotonic control of Curie temperature from 169 to 333 K and a magnetic anisotropy transition from out-of-plane to the in-plane configuration are achieved. Based on the intercalation engineering, room-temperature skyrmions are successfully created in Cr1.53 Te2 with a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy. Remarkably, a skyrmion-induced topological Hall resistivity as large as ≈106 nΩ cm is observed at 290 K. Moreover, a sign reversal of THE is also found at low temperatures, which can be ascribed to other topological spin textures having an opposite topological charge to that of the skyrmions. Therefore, chromium telluride can be a new paradigm of the skyrmion material family with promising prospects for future device applications.Room-temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano-spintronic devices. However, such skyrmion-hosting materials are rare in nature. In this study, a self-intercalated transition metal dichalcogenide Cr1+ x Te2 with a layered crystal structure that hosts room-temperature skyrmions and exhibits large THE is reported. By tuning the self-intercalate concentration, a monotonic control of Curie temperature from 169 to 333 K and a magnetic anisotropy transition from out-of-plane to the in-plane configuration are achieved. Based on the intercalation engineering, room-temperature skyrmions are successfully created in Cr1.53 Te2 with a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy. Remarkably, a skyrmion-induced topological Hall resistivity as large as ≈106 nΩ cm is observed at 290 K. Moreover, a sign reversal of THE is also found at low temperatures, which can be ascribed to other topological spin textures having an opposite topological charge to that of the skyrmions. Therefore, chromium telluride can be a new paradigm of the skyrmion material family with promising prospects for future device applications.
Room-temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano-spintronic devices. However, such skyrmion-hosting materials are rare in nature. In this study, a self-intercalated transition metal dichalcogenide Cr Te with a layered crystal structure that hosts room-temperature skyrmions and exhibits large THE is reported. By tuning the self-intercalate concentration, a monotonic control of Curie temperature from 169 to 333 K and a magnetic anisotropy transition from out-of-plane to the in-plane configuration are achieved. Based on the intercalation engineering, room-temperature skyrmions are successfully created in Cr Te with a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy. Remarkably, a skyrmion-induced topological Hall resistivity as large as ≈106 nΩ cm is observed at 290 K. Moreover, a sign reversal of THE is also found at low temperatures, which can be ascribed to other topological spin textures having an opposite topological charge to that of the skyrmions. Therefore, chromium telluride can be a new paradigm of the skyrmion material family with promising prospects for future device applications.
Room‐temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano‐spintronic devices. However, such skyrmion‐hosting materials are rare in nature. In this study, a self‐intercalated transition metal dichalcogenide Cr1+xTe2 with a layered crystal structure that hosts room‐temperature skyrmions and exhibits large THE is reported. By tuning the self‐intercalate concentration, a monotonic control of Curie temperature from 169 to 333 K and a magnetic anisotropy transition from out‐of‐plane to the in‐plane configuration are achieved. Based on the intercalation engineering, room‐temperature skyrmions are successfully created in Cr1.53Te2 with a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy. Remarkably, a skyrmion‐induced topological Hall resistivity as large as ≈106 nΩ cm is observed at 290 K. Moreover, a sign reversal of THE is also found at low temperatures, which can be ascribed to other topological spin textures having an opposite topological charge to that of the skyrmions. Therefore, chromium telluride can be a new paradigm of the skyrmion material family with promising prospects for future device applications. Magnetic skyrmions and large topological Hall effect are demonstrated in chromium telluride. The Curie temperature and magnetic anisotropy in Cr1+xTe2 can be controlled by the self‐intercalate concentration x. In Cr1.53Te2, which has a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy, room‐temperature skyrmions and topological Hall resistivity as large as ≈106 nΩ cm are observed.
Room‐temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano‐spintronic devices. However, such skyrmion‐hosting materials are rare in nature. In this study, a self‐intercalated transition metal dichalcogenide Cr1+xTe2 with a layered crystal structure that hosts room‐temperature skyrmions and exhibits large THE is reported. By tuning the self‐intercalate concentration, a monotonic control of Curie temperature from 169 to 333 K and a magnetic anisotropy transition from out‐of‐plane to the in‐plane configuration are achieved. Based on the intercalation engineering, room‐temperature skyrmions are successfully created in Cr1.53Te2 with a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy. Remarkably, a skyrmion‐induced topological Hall resistivity as large as ≈106 nΩ cm is observed at 290 K. Moreover, a sign reversal of THE is also found at low temperatures, which can be ascribed to other topological spin textures having an opposite topological charge to that of the skyrmions. Therefore, chromium telluride can be a new paradigm of the skyrmion material family with promising prospects for future device applications.
Room‐temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano‐spintronic devices. However, such skyrmion‐hosting materials are rare in nature. In this study, a self‐intercalated transition metal dichalcogenide Cr 1+ x Te 2 with a layered crystal structure that hosts room‐temperature skyrmions and exhibits large THE is reported. By tuning the self‐intercalate concentration, a monotonic control of Curie temperature from 169 to 333 K and a magnetic anisotropy transition from out‐of‐plane to the in‐plane configuration are achieved. Based on the intercalation engineering, room‐temperature skyrmions are successfully created in Cr 1.53 Te 2 with a Curie temperature of 295 K and a relatively weak perpendicular magnetic anisotropy. Remarkably, a skyrmion‐induced topological Hall resistivity as large as ≈106 nΩ cm is observed at 290 K. Moreover, a sign reversal of THE is also found at low temperatures, which can be ascribed to other topological spin textures having an opposite topological charge to that of the skyrmions. Therefore, chromium telluride can be a new paradigm of the skyrmion material family with promising prospects for future device applications.
Author Zheng, Dongxing
Zhang, Xi‐Xiang
Liu, Chen
Zhang, Qiang
Peng, Yong
Yuan, Youyou
Liu, Kai
Zhang, Chenhui
Li, Yan
Zhang, Junwei
Hou, Zhipeng
Yin, Gen
Wen, Yan
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  organization: King Abdullah University of Science and Technology (KAUST)
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  fullname: Liu, Chen
  organization: King Abdullah University of Science and Technology (KAUST)
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  surname: Zhang
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  organization: Lanzhou University
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  surname: Yuan
  fullname: Yuan, Youyou
  organization: King Abdullah University of Science and Technology (KAUST)
– sequence: 5
  givenname: Yan
  surname: Wen
  fullname: Wen, Yan
  organization: King Abdullah University of Science and Technology (KAUST)
– sequence: 6
  givenname: Yan
  surname: Li
  fullname: Li, Yan
  organization: King Abdullah University of Science and Technology (KAUST)
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  givenname: Dongxing
  surname: Zheng
  fullname: Zheng, Dongxing
  organization: King Abdullah University of Science and Technology (KAUST)
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  givenname: Qiang
  surname: Zhang
  fullname: Zhang, Qiang
  organization: New York University Abu Dhabi
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  givenname: Zhipeng
  surname: Hou
  fullname: Hou, Zhipeng
  organization: South China Normal University
– sequence: 10
  givenname: Gen
  surname: Yin
  fullname: Yin, Gen
  organization: Georgetown University
– sequence: 11
  givenname: Kai
  surname: Liu
  fullname: Liu, Kai
  organization: Georgetown University
– sequence: 12
  givenname: Yong
  surname: Peng
  fullname: Peng, Yong
  email: pengy@lzu.edu.cn
  organization: Lanzhou University
– sequence: 13
  givenname: Xi‐Xiang
  orcidid: 0000-0002-3478-6414
  surname: Zhang
  fullname: Zhang, Xi‐Xiang
  email: xixiang.zhang@kaust.edu.sa
  organization: King Abdullah University of Science and Technology (KAUST)
BackLink https://www.ncbi.nlm.nih.gov/pubmed/36245330$$D View this record in MEDLINE/PubMed
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ISSN 0935-9648
1521-4095
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Fri Jul 25 08:43:59 EDT 2025
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IsPeerReviewed true
IsScholarly true
Issue 1
Keywords chromium telluride
topological Hall effect
layered materials
self-intercalation
magnetic skyrmions
Language English
License 2022 Wiley-VCH GmbH.
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Snippet Room‐temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano‐spintronic devices. However, such...
Room-temperature magnetic skyrmion materials exhibiting robust topological Hall effect (THE) are crucial for novel nano-spintronic devices. However, such...
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SubjectTerms Chromium
chromium telluride
Crystal structure
Curie temperature
Electromagnetism
Hall effect
Hypothetical particles
Intercalation
layered materials
Low temperature
Magnetic anisotropy
magnetic skyrmions
Magnetism
Materials science
Particle theory
self‐intercalation
Tellurides
Temperature
topological Hall effect
Topology
Transition metal compounds
Title Room‐Temperature Magnetic Skyrmions and Large Topological Hall Effect in Chromium Telluride Engineered by Self‐Intercalation
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.202205967
https://www.ncbi.nlm.nih.gov/pubmed/36245330
https://www.proquest.com/docview/2760751736
https://www.proquest.com/docview/2725438967
Volume 35
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