Metallosupramolecular Photonic Elastomers with Self‐Healing Capability and Angle‐Independent Color

Photonic elastomers that can change colors like a chameleon have shown great promise in various applications. However, it still remains a challenge to produce artificial photonic elastomers with desired optical and mechanical properties. Here, the generation of metallosupramolecular polymer‐based ph...

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Veröffentlicht in:	Advanced materials (Weinheim) Jg. 31; H. 6; S. e1805496 - n/a
Hauptverfasser:	Tan, Haiying, Lyu, Quanqian, Xie, Zhanjun, Li, Miaomiao, Wang, Kui, Wang, Ke, Xiong, Bijin, Zhang, Lianbin, Zhu, Jintao
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Germany Wiley Subscription Services, Inc 08.02.2019
Schlagworte:	angle‐independent Cerium Chlorides Color Elastomers Elongated structure Healing Materials science Mechanical properties metallosupramolecular coordination Modulus of elasticity Nanoparticles Optical coatings Optical properties photonic crystals Photonics Polydimethylsiloxane self‐healing Silicon dioxide Wearable technology photonic crystals elastomers angle-independent metallosupramolecular coordination self-healing
ISSN:	0935-9648, 1521-4095, 1521-4095
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Abstract	Photonic elastomers that can change colors like a chameleon have shown great promise in various applications. However, it still remains a challenge to produce artificial photonic elastomers with desired optical and mechanical properties. Here, the generation of metallosupramolecular polymer‐based photonic elastomers with tunable mechanical strength, angle‐independent structural color, and self‐healing capability is reported. The photonic elastomers are prepared by incorporating isotropically arranged monodispersed SiO2 nanoparticles within a supramolecular elastomeric matrix based on metal coordination interaction between amino‐terminated poly(dimethylsiloxane) and cerium trichloride. The photonic elastomers exhibit angle‐independent structural colors, while Young's modulus and elongation at break of the as‐formed photonic elastomers reach 0.24 MPa and 150%, respectively. The superior elasticity of photonic elastomers enables their chameleon‐skin‐like mechanochromic capability. Moreover, the photonic elastomers are capable of healing scratches or cuts to ensure sustainable optical and mechanical properties, which is crucial to their applications in wearable devices, optical coating, and visualized force sensing. Photonic elastomers with self‐healing capability and angle‐independent color are fabricated through the combination of a supramolecular elastomer with isotropic nanostructures, exhibiting chameleon‐skin‐like mechanochromic capability. Interestingly, the photonic elastomers are capable of healing scratches or cuts, ensuring the optical and mechanical properties.
AbstractList	Photonic elastomers that can change colors like a chameleon have shown great promise in various applications. However, it still remains a challenge to produce artificial photonic elastomers with desired optical and mechanical properties. Here, the generation of metallosupramolecular polymer‐based photonic elastomers with tunable mechanical strength, angle‐independent structural color, and self‐healing capability is reported. The photonic elastomers are prepared by incorporating isotropically arranged monodispersed SiO2 nanoparticles within a supramolecular elastomeric matrix based on metal coordination interaction between amino‐terminated poly(dimethylsiloxane) and cerium trichloride. The photonic elastomers exhibit angle‐independent structural colors, while Young's modulus and elongation at break of the as‐formed photonic elastomers reach 0.24 MPa and 150%, respectively. The superior elasticity of photonic elastomers enables their chameleon‐skin‐like mechanochromic capability. Moreover, the photonic elastomers are capable of healing scratches or cuts to ensure sustainable optical and mechanical properties, which is crucial to their applications in wearable devices, optical coating, and visualized force sensing. Photonic elastomers with self‐healing capability and angle‐independent color are fabricated through the combination of a supramolecular elastomer with isotropic nanostructures, exhibiting chameleon‐skin‐like mechanochromic capability. Interestingly, the photonic elastomers are capable of healing scratches or cuts, ensuring the optical and mechanical properties. Photonic elastomers that can change colors like a chameleon have shown great promise in various applications. However, it still remains a challenge to produce artificial photonic elastomers with desired optical and mechanical properties. Here, the generation of metallosupramolecular polymer-based photonic elastomers with tunable mechanical strength, angle-independent structural color, and self-healing capability is reported. The photonic elastomers are prepared by incorporating isotropically arranged monodispersed SiO2 nanoparticles within a supramolecular elastomeric matrix based on metal coordination interaction between amino-terminated poly(dimethylsiloxane) and cerium trichloride. The photonic elastomers exhibit angle-independent structural colors, while Young's modulus and elongation at break of the as-formed photonic elastomers reach 0.24 MPa and 150%, respectively. The superior elasticity of photonic elastomers enables their chameleon-skin-like mechanochromic capability. Moreover, the photonic elastomers are capable of healing scratches or cuts to ensure sustainable optical and mechanical properties, which is crucial to their applications in wearable devices, optical coating, and visualized force sensing.Photonic elastomers that can change colors like a chameleon have shown great promise in various applications. However, it still remains a challenge to produce artificial photonic elastomers with desired optical and mechanical properties. Here, the generation of metallosupramolecular polymer-based photonic elastomers with tunable mechanical strength, angle-independent structural color, and self-healing capability is reported. The photonic elastomers are prepared by incorporating isotropically arranged monodispersed SiO2 nanoparticles within a supramolecular elastomeric matrix based on metal coordination interaction between amino-terminated poly(dimethylsiloxane) and cerium trichloride. The photonic elastomers exhibit angle-independent structural colors, while Young's modulus and elongation at break of the as-formed photonic elastomers reach 0.24 MPa and 150%, respectively. The superior elasticity of photonic elastomers enables their chameleon-skin-like mechanochromic capability. Moreover, the photonic elastomers are capable of healing scratches or cuts to ensure sustainable optical and mechanical properties, which is crucial to their applications in wearable devices, optical coating, and visualized force sensing. Photonic elastomers that can change colors like a chameleon have shown great promise in various applications. However, it still remains a challenge to produce artificial photonic elastomers with desired optical and mechanical properties. Here, the generation of metallosupramolecular polymer‐based photonic elastomers with tunable mechanical strength, angle‐independent structural color, and self‐healing capability is reported. The photonic elastomers are prepared by incorporating isotropically arranged monodispersed SiO2 nanoparticles within a supramolecular elastomeric matrix based on metal coordination interaction between amino‐terminated poly(dimethylsiloxane) and cerium trichloride. The photonic elastomers exhibit angle‐independent structural colors, while Young's modulus and elongation at break of the as‐formed photonic elastomers reach 0.24 MPa and 150%, respectively. The superior elasticity of photonic elastomers enables their chameleon‐skin‐like mechanochromic capability. Moreover, the photonic elastomers are capable of healing scratches or cuts to ensure sustainable optical and mechanical properties, which is crucial to their applications in wearable devices, optical coating, and visualized force sensing. Photonic elastomers that can change colors like a chameleon have shown great promise in various applications. However, it still remains a challenge to produce artificial photonic elastomers with desired optical and mechanical properties. Here, the generation of metallosupramolecular polymer-based photonic elastomers with tunable mechanical strength, angle-independent structural color, and self-healing capability is reported. The photonic elastomers are prepared by incorporating isotropically arranged monodispersed SiO nanoparticles within a supramolecular elastomeric matrix based on metal coordination interaction between amino-terminated poly(dimethylsiloxane) and cerium trichloride. The photonic elastomers exhibit angle-independent structural colors, while Young's modulus and elongation at break of the as-formed photonic elastomers reach 0.24 MPa and 150%, respectively. The superior elasticity of photonic elastomers enables their chameleon-skin-like mechanochromic capability. Moreover, the photonic elastomers are capable of healing scratches or cuts to ensure sustainable optical and mechanical properties, which is crucial to their applications in wearable devices, optical coating, and visualized force sensing. Photonic elastomers that can change colors like a chameleon have shown great promise in various applications. However, it still remains a challenge to produce artificial photonic elastomers with desired optical and mechanical properties. Here, the generation of metallosupramolecular polymer‐based photonic elastomers with tunable mechanical strength, angle‐independent structural color, and self‐healing capability is reported. The photonic elastomers are prepared by incorporating isotropically arranged monodispersed SiO 2 nanoparticles within a supramolecular elastomeric matrix based on metal coordination interaction between amino‐terminated poly(dimethylsiloxane) and cerium trichloride. The photonic elastomers exhibit angle‐independent structural colors, while Young's modulus and elongation at break of the as‐formed photonic elastomers reach 0.24 MPa and 150%, respectively. The superior elasticity of photonic elastomers enables their chameleon‐skin‐like mechanochromic capability. Moreover, the photonic elastomers are capable of healing scratches or cuts to ensure sustainable optical and mechanical properties, which is crucial to their applications in wearable devices, optical coating, and visualized force sensing.
Author	Li, Miaomiao Lyu, Quanqian Xie, Zhanjun Zhang, Lianbin Tan, Haiying Wang, Ke Wang, Kui Xiong, Bijin Zhu, Jintao
Author_xml	– sequence: 1 givenname: Haiying surname: Tan fullname: Tan, Haiying organization: Huazhong University of Science and Technology – sequence: 2 givenname: Quanqian surname: Lyu fullname: Lyu, Quanqian organization: Huazhong University of Science and Technology – sequence: 3 givenname: Zhanjun surname: Xie fullname: Xie, Zhanjun organization: Huazhong University of Science and Technology – sequence: 4 givenname: Miaomiao surname: Li fullname: Li, Miaomiao organization: Huazhong University of Science and Technology – sequence: 5 givenname: Kui surname: Wang fullname: Wang, Kui organization: Huazhong University of Science and Technology – sequence: 6 givenname: Ke surname: Wang fullname: Wang, Ke organization: Huazhong University of Science and Technology – sequence: 7 givenname: Bijin surname: Xiong fullname: Xiong, Bijin organization: Huazhong University of Science and Technology – sequence: 8 givenname: Lianbin surname: Zhang fullname: Zhang, Lianbin email: zhanglianbin@hust.edu.cn organization: Huazhong University of Science and Technology – sequence: 9 givenname: Jintao orcidid: 0000-0002-8230-3923 surname: Zhu fullname: Zhu, Jintao email: jtzhu@mail.hust.edu.cn organization: Huazhong University of Science and Technology
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Keywords	photonic crystals elastomers angle-independent metallosupramolecular coordination self-healing
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Snippet	Photonic elastomers that can change colors like a chameleon have shown great promise in various applications. However, it still remains a challenge to produce...
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SubjectTerms	angle‐independent Cerium Chlorides Color Elastomers Elongated structure Healing Materials science Mechanical properties metallosupramolecular coordination Modulus of elasticity Nanoparticles Optical coatings Optical properties photonic crystals Photonics Polydimethylsiloxane self‐healing Silicon dioxide Wearable technology
Title	Metallosupramolecular Photonic Elastomers with Self‐Healing Capability and Angle‐Independent Color
URI	https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.201805496 https://www.ncbi.nlm.nih.gov/pubmed/30548887 https://www.proquest.com/docview/2177157904 https://www.proquest.com/docview/2157652800
Volume	31
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