Revealing Hydrogen Bond Effect in Rechargeable Aqueous Zinc‐Organic Batteries

The surrounding hydrogen bond (H‐bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to fulfill their roles as ion reservoirs in aqueous zinc‐organic batteries (ZOBs). Despite important, there are still no works could fully shed...

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Veröffentlicht in:	Angewandte Chemie International Edition Jg. 63; H. 29; S. e202406465 - n/a
Hauptverfasser:	Guo, Jun, Du, Jia‐Yi, Liu, Wan‐Qiang, Huang, Gang, Zhang, Xin‐Bo
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Germany Wiley Subscription Services, Inc 15.07.2024
Ausgabe:	International ed. in English
Schlagworte:	Air-Rechargeable Aqueous Zinc-Organic Batteries Electrode materials Hydrogen Bond Hydrogen bonds Organic Electrode Materials Quinone Quinones Zinc Aqueous Zinc-Organic Batteries Air-Rechargeable Organic Electrode Materials Quinone Hydrogen Bond
ISSN:	1433-7851, 1521-3773, 1521-3773
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Abstract	The surrounding hydrogen bond (H‐bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to fulfill their roles as ion reservoirs in aqueous zinc‐organic batteries (ZOBs). Despite important, there are still no works could fully shed its real effects light on. Herein, quinone‐based small molecules with a H‐bond evolution model has been rationally selected to disclose the regulation and equilibration of H‐bond interaction between OEMs, and OEM and the electrolyte. It has been found that only a suitable H‐bond interaction could make the OEMs fully liberate their potential performance. Accordingly, the 2,5‐diaminocyclohexa‐2,5‐diene‐1,4‐dione (DABQ) with elaborately designed H‐bond structure exhibits a capacity of 193.3 mAh g−1 at a record‐high mass loading of 66.2 mg cm−2 and 100 % capacity retention after 1500 cycles at 5 A g−1. In addition, the DABQ//Zn battery also possesses air‐rechargeable ability by utilizing the chemistry redox of proton. Our results put forward a specific pathway to precise utilization of H‐bond to liberate the performance of OEMs. A series of quinone‐based small molecules with progressive hydrogen bond (H‐bond) numbers has been rationally designed to reveal the real effects of H‐bond on the electrochemical performance of organic electrode materials (OEMs) in rechargeable aqueous zinc‐organic batteries (ZOBs). The appropriate number of H‐bonds in OEM improves its structure stability and utilization of active sites and reduces the battery polarization, contributing to the construction of high‐performance ZOBs.
AbstractList	The surrounding hydrogen bond (H-bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to fulfill their roles as ion reservoirs in aqueous zinc-organic batteries (ZOBs). Despite important, there are still no works could fully shed its real effects light on. Herein, quinone-based small molecules with a H-bond evolution model has been rationally selected to disclose the regulation and equilibration of H-bond interaction between OEMs, and OEM and the electrolyte. It has been found that only a suitable H-bond interaction could make the OEMs fully liberate their potential performance. Accordingly, the 2,5-diaminocyclohexa-2,5-diene-1,4-dione (DABQ) with elaborately designed H-bond structure exhibits a capacity of 193.3 mAh g at a record-high mass loading of 66.2 mg cm and 100 % capacity retention after 1500 cycles at 5 A g . In addition, the DABQ//Zn battery also possesses air-rechargeable ability by utilizing the chemistry redox of proton. Our results put forward a specific pathway to precise utilization of H-bond to liberate the performance of OEMs. The surrounding hydrogen bond (H‐bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to fulfill their roles as ion reservoirs in aqueous zinc‐organic batteries (ZOBs). Despite important, there are still no works could fully shed its real effects light on. Herein, quinone‐based small molecules with a H‐bond evolution model has been rationally selected to disclose the regulation and equilibration of H‐bond interaction between OEMs, and OEM and the electrolyte. It has been found that only a suitable H‐bond interaction could make the OEMs fully liberate their potential performance. Accordingly, the 2,5‐diaminocyclohexa‐2,5‐diene‐1,4‐dione (DABQ) with elaborately designed H‐bond structure exhibits a capacity of 193.3 mAh g −1 at a record‐high mass loading of 66.2 mg cm −2 and 100 % capacity retention after 1500 cycles at 5 A g −1 . In addition, the DABQ//Zn battery also possesses air‐rechargeable ability by utilizing the chemistry redox of proton. Our results put forward a specific pathway to precise utilization of H‐bond to liberate the performance of OEMs. The surrounding hydrogen bond (H‐bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to fulfill their roles as ion reservoirs in aqueous zinc‐organic batteries (ZOBs). Despite important, there are still no works could fully shed its real effects light on. Herein, quinone‐based small molecules with a H‐bond evolution model has been rationally selected to disclose the regulation and equilibration of H‐bond interaction between OEMs, and OEM and the electrolyte. It has been found that only a suitable H‐bond interaction could make the OEMs fully liberate their potential performance. Accordingly, the 2,5‐diaminocyclohexa‐2,5‐diene‐1,4‐dione (DABQ) with elaborately designed H‐bond structure exhibits a capacity of 193.3 mAh g−1 at a record‐high mass loading of 66.2 mg cm−2 and 100 % capacity retention after 1500 cycles at 5 A g−1. In addition, the DABQ//Zn battery also possesses air‐rechargeable ability by utilizing the chemistry redox of proton. Our results put forward a specific pathway to precise utilization of H‐bond to liberate the performance of OEMs. The surrounding hydrogen bond (H‐bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to fulfill their roles as ion reservoirs in aqueous zinc‐organic batteries (ZOBs). Despite important, there are still no works could fully shed its real effects light on. Herein, quinone‐based small molecules with a H‐bond evolution model has been rationally selected to disclose the regulation and equilibration of H‐bond interaction between OEMs, and OEM and the electrolyte. It has been found that only a suitable H‐bond interaction could make the OEMs fully liberate their potential performance. Accordingly, the 2,5‐diaminocyclohexa‐2,5‐diene‐1,4‐dione (DABQ) with elaborately designed H‐bond structure exhibits a capacity of 193.3 mAh g−1 at a record‐high mass loading of 66.2 mg cm−2 and 100 % capacity retention after 1500 cycles at 5 A g−1. In addition, the DABQ//Zn battery also possesses air‐rechargeable ability by utilizing the chemistry redox of proton. Our results put forward a specific pathway to precise utilization of H‐bond to liberate the performance of OEMs. A series of quinone‐based small molecules with progressive hydrogen bond (H‐bond) numbers has been rationally designed to reveal the real effects of H‐bond on the electrochemical performance of organic electrode materials (OEMs) in rechargeable aqueous zinc‐organic batteries (ZOBs). The appropriate number of H‐bonds in OEM improves its structure stability and utilization of active sites and reduces the battery polarization, contributing to the construction of high‐performance ZOBs. The surrounding hydrogen bond (H-bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to fulfill their roles as ion reservoirs in aqueous zinc-organic batteries (ZOBs). Despite important, there are still no works could fully shed its real effects light on. Herein, quinone-based small molecules with a H-bond evolution model has been rationally selected to disclose the regulation and equilibration of H-bond interaction between OEMs, and OEM and the electrolyte. It has been found that only a suitable H-bond interaction could make the OEMs fully liberate their potential performance. Accordingly, the 2,5-diaminocyclohexa-2,5-diene-1,4-dione (DABQ) with elaborately designed H-bond structure exhibits a capacity of 193.3 mAh g-1 at a record-high mass loading of 66.2 mg cm-2 and 100 % capacity retention after 1500 cycles at 5 A g-1. In addition, the DABQ//Zn battery also possesses air-rechargeable ability by utilizing the chemistry redox of proton. Our results put forward a specific pathway to precise utilization of H-bond to liberate the performance of OEMs.The surrounding hydrogen bond (H-bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to fulfill their roles as ion reservoirs in aqueous zinc-organic batteries (ZOBs). Despite important, there are still no works could fully shed its real effects light on. Herein, quinone-based small molecules with a H-bond evolution model has been rationally selected to disclose the regulation and equilibration of H-bond interaction between OEMs, and OEM and the electrolyte. It has been found that only a suitable H-bond interaction could make the OEMs fully liberate their potential performance. Accordingly, the 2,5-diaminocyclohexa-2,5-diene-1,4-dione (DABQ) with elaborately designed H-bond structure exhibits a capacity of 193.3 mAh g-1 at a record-high mass loading of 66.2 mg cm-2 and 100 % capacity retention after 1500 cycles at 5 A g-1. In addition, the DABQ//Zn battery also possesses air-rechargeable ability by utilizing the chemistry redox of proton. Our results put forward a specific pathway to precise utilization of H-bond to liberate the performance of OEMs.
Author	Zhang, Xin‐Bo Huang, Gang Guo, Jun Du, Jia‐Yi Liu, Wan‐Qiang
Author_xml	– sequence: 1 givenname: Jun surname: Guo fullname: Guo, Jun organization: Chinese Academy of Sciences – sequence: 2 givenname: Jia‐Yi surname: Du fullname: Du, Jia‐Yi organization: Chinese Academy of Sciences – sequence: 3 givenname: Wan‐Qiang surname: Liu fullname: Liu, Wan‐Qiang email: wqliu1979@126.com organization: Changchun University of Science and Technology – sequence: 4 givenname: Gang surname: Huang fullname: Huang, Gang email: ghuang@ciac.ac.cn organization: Chinese Academy of Sciences – sequence: 5 givenname: Xin‐Bo orcidid: 0000-0002-5806-159X surname: Zhang fullname: Zhang, Xin‐Bo email: xbzhang@ciac.ac.cn organization: Chinese Academy of Sciences
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Keywords	Aqueous Zinc-Organic Batteries Air-Rechargeable Organic Electrode Materials Quinone Hydrogen Bond
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Snippet	The surrounding hydrogen bond (H‐bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to... The surrounding hydrogen bond (H-bond) interaction around the active sites plays indispensable functions in enabling the organic electrode materials (OEMs) to...
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SubjectTerms	Air-Rechargeable Aqueous Zinc-Organic Batteries Electrode materials Hydrogen Bond Hydrogen bonds Organic Electrode Materials Quinone Quinones Zinc
Title	Revealing Hydrogen Bond Effect in Rechargeable Aqueous Zinc‐Organic Batteries
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