Non-noble metal-based bifunctional electrocatalysts for hydrogen production

Hydrogen is a promising candidate for clean and sustainable energy resources to substitute fossil fuels to mitigate global environmental issues. Electrochemical hydrogen production has been regarded as a viable and promising strategy. The overall water splitting is currently the predominant electroc...

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Veröffentlicht in:	Rare metals Jg. 41; H. 7; S. 2169 - 2183
Hauptverfasser:	Wu, Tong, Sun, Ming-Zi, Huang, Bo-Long
Format:	Journal Article
Sprache:	Englisch
Veröffentlicht:	Beijing Nonferrous Metals Society of China 01.07.2022 Springer Nature B.V
Schlagworte:	Bifunctional electrocatalyst Biomaterials Chemistry and Materials Science Clean energy Electrocatalysts Energy Energy sources Energy‐saving hydrogen production Fossil fuels Hydrogen Hydrogen evolution reactions Hydrogen production Hydrogen-based energy Materials Engineering Materials Science Metallic Materials Mini Review Nanoscale Science and Technology Noble metals Non‐noble metal electrocatalysts Overall water splitting Oxidation Oxygen evolution reactions Physical Chemistry Production methods Renewable energy Water splitting Bifunctional electrocatalyst Energy-saving hydrogen production Overall water splitting Hydrogen production Non-noble metal electrocatalysts
ISSN:	1001-0521, 1867-7185
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Abstract	Hydrogen is a promising candidate for clean and sustainable energy resources to substitute fossil fuels to mitigate global environmental issues. Electrochemical hydrogen production has been regarded as a viable and promising strategy. The overall water splitting is currently the predominant electrochemical hydrogen production method, which could be driven by renewable energy to achieve sustainable production. However, the current challenges are the intrinsically sluggish and energy-intensive oxygen evolution reduction (OER) at the anode and the expensive noble metal-based catalysts for overall water splitting, which limit the practical applications. Extensive efforts have been made to develop bifunctional non-noble metal-based electrocatalysts to boost hydrogen production efficiency and lower the cost. Meanwhile, alternative oxidation reactions with faster kinetics and less energy requirement than OER are being explored as the anodic reaction to couple with the hydrogen evolution reaction for energy-saving hydrogen production. In this review, the non-noble metal-based bifunctional electrocatalysts for overall water splitting, as well as other novel energy-saving hydrogen productions have been introduced and summarized. Current challenges and outlooks are commented on at the end of the article. Graphical abstract
AbstractList	Hydrogen is a promising candidate for clean and sustainable energy resources to substitute fossil fuels to mitigate global environmental issues. Electrochemical hydrogen production has been regarded as a viable and promising strategy. The overall water splitting is currently the predominant electrochemical hydrogen production method, which could be driven by renewable energy to achieve sustainable production. However, the current challenges are the intrinsically sluggish and energy‐intensive oxygen evolution reduction (OER) at the anode and the expensive noble metal‐based catalysts for overall water splitting, which limit the practical applications. Extensive efforts have been made to develop bifunctional non‐noble metal‐based electrocatalysts to boost hydrogen production efficiency and lower the cost. Meanwhile, alternative oxidation reactions with faster kinetics and less energy requirement than OER are being explored as the anodic reaction to couple with the hydrogen evolution reaction for energy‐saving hydrogen production. In this review, the non‐noble metal‐based bifunctional electrocatalysts for overall water splitting, as well as other novel energy‐saving hydrogen productions have been introduced and summarized. Current challenges and outlooks are commented on at the end of the article. 氢气是清洁和可持续能源, 也是替代化石燃料从而缓解全球环境问题的最佳候选。电化学制氢被认为是一种可行且具备应用前景的重要策略。目前, 电化学催化水分解是目前最主要的电化学制氢方法, 该方法可以由可再生能源驱动从而实现可持续产氢过程。然而, 当前水分解催化制氢面临的挑战是阳极的析氧还原不仅动力学缓慢而且需要较高的过电势来驱动反应进行, 一般需要昂贵稀少的贵金属基催化剂来实现水分解制氢, 从而限制了大规模的工业应用前景。目前, 科学界已经进行了广泛的研究来开发双功能非贵金属基电催化剂用于水分解, 从而提高制氢效率并降低成本。与此同时, 作为与析氢反应耦合以实现高效节能制氢的阳极反应, 探索具有比析氧还原反应具有更快动力学和更少能量需求的替代氧化反应也成为了新的研究重点。在该综述中, 我们对于可用于整体水分解的非贵金属基双功能电催化剂进行了分类与总结, 并对其他新型可用于高效水分解制氢的替代氧化过程进行了介绍, 并在最后对当前的电化学制氢催化剂所面临的挑战和未来发展方向进行了全面的展望。 Hydrogen is a promising candidate for clean and sustainable energy resources to substitute fossil fuels to mitigate global environmental issues. Electrochemical hydrogen production has been regarded as a viable and promising strategy. The overall water splitting is currently the predominant electrochemical hydrogen production method, which could be driven by renewable energy to achieve sustainable production. However, the current challenges are the intrinsically sluggish and energy-intensive oxygen evolution reduction (OER) at the anode and the expensive noble metal-based catalysts for overall water splitting, which limit the practical applications. Extensive efforts have been made to develop bifunctional non-noble metal-based electrocatalysts to boost hydrogen production efficiency and lower the cost. Meanwhile, alternative oxidation reactions with faster kinetics and less energy requirement than OER are being explored as the anodic reaction to couple with the hydrogen evolution reaction for energy-saving hydrogen production. In this review, the non-noble metal-based bifunctional electrocatalysts for overall water splitting, as well as other novel energy-saving hydrogen productions have been introduced and summarized. Current challenges and outlooks are commented on at the end of the article. Hydrogen is a promising candidate for clean and sustainable energy resources to substitute fossil fuels to mitigate global environmental issues. Electrochemical hydrogen production has been regarded as a viable and promising strategy. The overall water splitting is currently the predominant electrochemical hydrogen production method, which could be driven by renewable energy to achieve sustainable production. However, the current challenges are the intrinsically sluggish and energy‐intensive oxygen evolution reduction (OER) at the anode and the expensive noble metal‐based catalysts for overall water splitting, which limit the practical applications. Extensive efforts have been made to develop bifunctional non‐noble metal‐based electrocatalysts to boost hydrogen production efficiency and lower the cost. Meanwhile, alternative oxidation reactions with faster kinetics and less energy requirement than OER are being explored as the anodic reaction to couple with the hydrogen evolution reaction for energy‐saving hydrogen production. In this review, the non‐noble metal‐based bifunctional electrocatalysts for overall water splitting, as well as other novel energy‐saving hydrogen productions have been introduced and summarized. Current challenges and outlooks are commented on at the end of the article. Graphical 摘要氢气是清洁和可持续能源, 也是替代化石燃料从而缓解全球环境问题的最佳候选。电化学制氢被认为是一种可行且具备应用前景的重要策略。目前, 电化学催化水分解是目前最主要的电化学制氢方法, 该方法可以由可再生能源驱动从而实现可持续产氢过程。然而, 当前水分解催化制氢面临的挑战是阳极的析氧还原不仅动力学缓慢而且需要较高的过电势来驱动反应进行, 一般需要昂贵稀少的贵金属基催化剂来实现水分解制氢, 从而限制了大规模的工业应用前景。目前, 科学界已经进行了广泛的研究来开发双功能非贵金属基电催化剂用于水分解, 从而提高制氢效率并降低成本。与此同时, 作为与析氢反应耦合以实现高效节能制氢的阳极反应, 探索具有比析氧还原反应具有更快动力学和更少能量需求的替代氧化反应也成为了新的研究重点。在该综述中, 我们对于可用于整体水分解的非贵金属基双功能电催化剂进行了分类与总结, 并对其他新型可用于高效水分解制氢的替代氧化过程进行了介绍, 并在最后对当前的电化学制氢催化剂所面临的挑战和未来发展方向进行了全面的展望。 Hydrogen is a promising candidate for clean and sustainable energy resources to substitute fossil fuels to mitigate global environmental issues. Electrochemical hydrogen production has been regarded as a viable and promising strategy. The overall water splitting is currently the predominant electrochemical hydrogen production method, which could be driven by renewable energy to achieve sustainable production. However, the current challenges are the intrinsically sluggish and energy-intensive oxygen evolution reduction (OER) at the anode and the expensive noble metal-based catalysts for overall water splitting, which limit the practical applications. Extensive efforts have been made to develop bifunctional non-noble metal-based electrocatalysts to boost hydrogen production efficiency and lower the cost. Meanwhile, alternative oxidation reactions with faster kinetics and less energy requirement than OER are being explored as the anodic reaction to couple with the hydrogen evolution reaction for energy-saving hydrogen production. In this review, the non-noble metal-based bifunctional electrocatalysts for overall water splitting, as well as other novel energy-saving hydrogen productions have been introduced and summarized. Current challenges and outlooks are commented on at the end of the article. Graphical abstract
Author	Huang, Bo-Long Sun, Ming-Zi Wu, Tong
Author_xml	– sequence: 1 givenname: Tong orcidid: 0000-0002-4621-8799 surname: Wu fullname: Wu, Tong organization: Department of Applied Biology and Chemical Technology, the Hong Kong Polytechnic University – sequence: 2 givenname: Ming-Zi orcidid: 0000-0001-5136-7265 surname: Sun fullname: Sun, Ming-Zi organization: Department of Applied Biology and Chemical Technology, the Hong Kong Polytechnic University – sequence: 3 givenname: Bo-Long orcidid: 0000-0002-2526-2002 surname: Huang fullname: Huang, Bo-Long email: bhuang@polyu.edu.hk organization: Department of Applied Biology and Chemical Technology, the Hong Kong Polytechnic University
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Publisher	Nonferrous Metals Society of China Springer Nature B.V
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SubjectTerms	Bifunctional electrocatalyst Biomaterials Chemistry and Materials Science Clean energy Electrocatalysts Energy Energy sources Energy‐saving hydrogen production Fossil fuels Hydrogen Hydrogen evolution reactions Hydrogen production Hydrogen-based energy Materials Engineering Materials Science Metallic Materials Mini Review Nanoscale Science and Technology Noble metals Non‐noble metal electrocatalysts Overall water splitting Oxidation Oxygen evolution reactions Physical Chemistry Production methods Renewable energy Water splitting
Title	Non-noble metal-based bifunctional electrocatalysts for hydrogen production
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