Ultrasonically spray coated silver layers from designed precursor inks for flexible electronics
Integration of electronic circuit components onto flexible materials such as plastic foils, paper and textiles is a key challenge for the development of future smart applications. Therefore, conductive metal features need to be deposited on temperature sensitive substrates in a fast and straightforw...
Uloženo v:
| Vydáno v: | Nanotechnology Ročník 28; číslo 21; s. 215202 |
|---|---|
| Hlavní autoři: | , , , , , , , , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
| Vydáno: |
England
26.05.2017
|
| ISSN: | 1361-6528, 1361-6528 |
| On-line přístup: | Zjistit podrobnosti o přístupu |
| Tagy: |
Přidat tag
Žádné tagy, Buďte první, kdo vytvoří štítek k tomuto záznamu!
|
| Abstract | Integration of electronic circuit components onto flexible materials such as plastic foils, paper and textiles is a key challenge for the development of future smart applications. Therefore, conductive metal features need to be deposited on temperature sensitive substrates in a fast and straightforward way. The feasibility of these emerging (nano-) electronic technologies depends on the availability of well-designed deposition techniques and on novel functional metal inks. As ultrasonic spray coating (USSC) is one of the most promising techniques to meet the above requirements, innovative metal organic decomposition (MOD) inks are designed to deposit silver features on plastic foils. Various amine ligands were screened and their influence on the ink stability and the characteristics of the resulting metal depositions were evaluated to determine the optimal formulation. Eventually, silver layers with excellent performance in terms of conductivity (15% bulk silver conductivity), stability, morphology and adhesion could be obtained, while operating in a very low temperature window of 70 °C-120 °C. Moreover, the optimal deposition conditions were determined via an in-depth analysis of the ultrasonically sprayed silver layers. Applying these tailored MOD inks, the USSC technique enabled smooth, semi-transparent silver layers with a tunable thickness on large areas without time-consuming additional sintering steps after deposition. Therefore, this novel combination of nanoparticle-free Ag-inks and the USSC process holds promise for high throughput deposition of highly conductive silver features on heat sensitive substrates and even 3D objects. |
|---|---|
| AbstractList | Integration of electronic circuit components onto flexible materials such as plastic foils, paper and textiles is a key challenge for the development of future smart applications. Therefore, conductive metal features need to be deposited on temperature sensitive substrates in a fast and straightforward way. The feasibility of these emerging (nano-) electronic technologies depends on the availability of well-designed deposition techniques and on novel functional metal inks. As ultrasonic spray coating (USSC) is one of the most promising techniques to meet the above requirements, innovative metal organic decomposition (MOD) inks are designed to deposit silver features on plastic foils. Various amine ligands were screened and their influence on the ink stability and the characteristics of the resulting metal depositions were evaluated to determine the optimal formulation. Eventually, silver layers with excellent performance in terms of conductivity (15% bulk silver conductivity), stability, morphology and adhesion could be obtained, while operating in a very low temperature window of 70 °C-120 °C. Moreover, the optimal deposition conditions were determined via an in-depth analysis of the ultrasonically sprayed silver layers. Applying these tailored MOD inks, the USSC technique enabled smooth, semi-transparent silver layers with a tunable thickness on large areas without time-consuming additional sintering steps after deposition. Therefore, this novel combination of nanoparticle-free Ag-inks and the USSC process holds promise for high throughput deposition of highly conductive silver features on heat sensitive substrates and even 3D objects.Integration of electronic circuit components onto flexible materials such as plastic foils, paper and textiles is a key challenge for the development of future smart applications. Therefore, conductive metal features need to be deposited on temperature sensitive substrates in a fast and straightforward way. The feasibility of these emerging (nano-) electronic technologies depends on the availability of well-designed deposition techniques and on novel functional metal inks. As ultrasonic spray coating (USSC) is one of the most promising techniques to meet the above requirements, innovative metal organic decomposition (MOD) inks are designed to deposit silver features on plastic foils. Various amine ligands were screened and their influence on the ink stability and the characteristics of the resulting metal depositions were evaluated to determine the optimal formulation. Eventually, silver layers with excellent performance in terms of conductivity (15% bulk silver conductivity), stability, morphology and adhesion could be obtained, while operating in a very low temperature window of 70 °C-120 °C. Moreover, the optimal deposition conditions were determined via an in-depth analysis of the ultrasonically sprayed silver layers. Applying these tailored MOD inks, the USSC technique enabled smooth, semi-transparent silver layers with a tunable thickness on large areas without time-consuming additional sintering steps after deposition. Therefore, this novel combination of nanoparticle-free Ag-inks and the USSC process holds promise for high throughput deposition of highly conductive silver features on heat sensitive substrates and even 3D objects. Integration of electronic circuit components onto flexible materials such as plastic foils, paper and textiles is a key challenge for the development of future smart applications. Therefore, conductive metal features need to be deposited on temperature sensitive substrates in a fast and straightforward way. The feasibility of these emerging (nano-) electronic technologies depends on the availability of well-designed deposition techniques and on novel functional metal inks. As ultrasonic spray coating (USSC) is one of the most promising techniques to meet the above requirements, innovative metal organic decomposition (MOD) inks are designed to deposit silver features on plastic foils. Various amine ligands were screened and their influence on the ink stability and the characteristics of the resulting metal depositions were evaluated to determine the optimal formulation. Eventually, silver layers with excellent performance in terms of conductivity (15% bulk silver conductivity), stability, morphology and adhesion could be obtained, while operating in a very low temperature window of 70 °C-120 °C. Moreover, the optimal deposition conditions were determined via an in-depth analysis of the ultrasonically sprayed silver layers. Applying these tailored MOD inks, the USSC technique enabled smooth, semi-transparent silver layers with a tunable thickness on large areas without time-consuming additional sintering steps after deposition. Therefore, this novel combination of nanoparticle-free Ag-inks and the USSC process holds promise for high throughput deposition of highly conductive silver features on heat sensitive substrates and even 3D objects. |
| Author | Marchal, W Durand Sola, M A van den Ham, E J Calmont de Andrade Almeida, A D'Haen, J Van Bael, M K Drijkoningen, J Vandevenne, G Elen, K Hardy, A Deferme, W |
| Author_xml | – sequence: 1 givenname: W surname: Marchal fullname: Marchal, W organization: UHasselt, Hasselt University, Institute for Materials Research(IMO-IMOMEC), Inorganic and Physical Chemistry, Agoralaan, B-3590 Diepenbeek, Belgium. IMEC vzw, division IMOMEC, Agoralaan, B-3590 Diepenbeek, Belgium – sequence: 2 givenname: G surname: Vandevenne fullname: Vandevenne, G – sequence: 3 givenname: J surname: D'Haen fullname: D'Haen, J – sequence: 4 givenname: A surname: Calmont de Andrade Almeida fullname: Calmont de Andrade Almeida, A – sequence: 5 givenname: M A surname: Durand Sola fullname: Durand Sola, M A – sequence: 6 givenname: E J surname: van den Ham fullname: van den Ham, E J – sequence: 7 givenname: J surname: Drijkoningen fullname: Drijkoningen, J – sequence: 8 givenname: K surname: Elen fullname: Elen, K – sequence: 9 givenname: W surname: Deferme fullname: Deferme, W – sequence: 10 givenname: M K surname: Van Bael fullname: Van Bael, M K – sequence: 11 givenname: A surname: Hardy fullname: Hardy, A |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28471754$$D View this record in MEDLINE/PubMed |
| BookMark | eNpNkLtPwzAYxC1UREthZ0IeWUL9iB1nRBUvqRILnaMv9hcUcB7YCSL_PUEUxHSn-51uuFOyaLsWCbng7JozYzZcap5oJcwGQDsJR2T1Fy3--SU5jfGVMc6N4CdkKUya8UylK1Ls_RAgdm1twfuJxj7ARG0HAzoaa_-BgXqYMERaha6hDmP90s6sD2jHELtA6_ZthrOpPH7WpUeKHu0QvjfjGTmuwEc8P-ia7O9un7cPye7p_nF7s0uszNiQVJUTzpqU52CMU6ABnKhMXpYpZBmTyphUaqalZDJPhXKIYHOhAErHrM7Fmlz97Pahex8xDkVTR4veQ4vdGAtucs1SyZSaq5eH6lg26Io-1A2Eqfg9RXwBCv1oCw |
| CitedBy_id | crossref_primary_10_1002_smtd_202300638 crossref_primary_10_1177_24723444241303970 crossref_primary_10_1002_admt_201800243 crossref_primary_10_3390_ma11020290 crossref_primary_10_1016_j_orgel_2023_106890 crossref_primary_10_1002_admi_201901002 crossref_primary_10_3390_coatings13121977 crossref_primary_10_1007_s10853_019_03456_1 |
| ContentType | Journal Article |
| DBID | NPM 7X8 |
| DOI | 10.1088/1361-6528/aa6d3a |
| DatabaseName | PubMed MEDLINE - Academic |
| DatabaseTitle | PubMed MEDLINE - Academic |
| DatabaseTitleList | MEDLINE - Academic PubMed |
| Database_xml | – sequence: 1 dbid: NPM name: PubMed url: http://www.ncbi.nlm.nih.gov/entrez/query.fcgi?db=PubMed sourceTypes: Index Database – sequence: 2 dbid: 7X8 name: MEDLINE - Academic url: https://search.proquest.com/medline sourceTypes: Aggregation Database |
| DeliveryMethod | no_fulltext_linktorsrc |
| Discipline | Engineering Physics |
| EISSN | 1361-6528 |
| ExternalDocumentID | 28471754 |
| Genre | Journal Article |
| GroupedDBID | --- -~X 123 1JI 4.4 53G 5B3 5PX 5VS 5ZH 7.M 7.Q AAGCD AAJIO AAJKP AALHV AATNI ABHWH ABJNI ABQJV ABVAM ACAFW ACGFS ACHIP AEFHF AENEX AFYNE AKPSB ALMA_UNASSIGNED_HOLDINGS AOAED ASPBG ATQHT AVWKF AZFZN CBCFC CEBXE CJUJL CRLBU CS3 DU5 EBS EDWGO EJD EMSAF EPQRW EQZZN F5P IHE IJHAN IOP IZVLO KOT LAP M45 N5L N9A NPM NT- NT. P2P PJBAE R4D RIN RNS RO9 ROL RPA SY9 TN5 W28 XPP ZMT 7X8 ADEQX AEINN |
| ID | FETCH-LOGICAL-c370t-ffd2dc8419a88d5a6aad2f89bb4a77035884360633039425deeac925aabd0c692 |
| IEDL.DBID | 7X8 |
| ISICitedReferencesCount | 13 |
| ISICitedReferencesURI | http://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=Summon&SrcAuth=ProQuest&DestLinkType=CitingArticles&DestApp=WOS_CPL&KeyUT=000413074100001&url=https%3A%2F%2Fcvtisr.summon.serialssolutions.com%2F%23%21%2Fsearch%3Fho%3Df%26include.ft.matches%3Dt%26l%3Dnull%26q%3D |
| ISSN | 1361-6528 |
| IngestDate | Sun Nov 09 12:04:44 EST 2025 Thu Apr 03 07:01:10 EDT 2025 |
| IsPeerReviewed | true |
| IsScholarly | true |
| Issue | 21 |
| Language | English |
| LinkModel | DirectLink |
| MergedId | FETCHMERGED-LOGICAL-c370t-ffd2dc8419a88d5a6aad2f89bb4a77035884360633039425deeac925aabd0c692 |
| Notes | ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
| PMID | 28471754 |
| PQID | 1896043055 |
| PQPubID | 23479 |
| ParticipantIDs | proquest_miscellaneous_1896043055 pubmed_primary_28471754 |
| PublicationCentury | 2000 |
| PublicationDate | 2017-05-26 |
| PublicationDateYYYYMMDD | 2017-05-26 |
| PublicationDate_xml | – month: 05 year: 2017 text: 2017-05-26 day: 26 |
| PublicationDecade | 2010 |
| PublicationPlace | England |
| PublicationPlace_xml | – name: England |
| PublicationTitle | Nanotechnology |
| PublicationTitleAlternate | Nanotechnology |
| PublicationYear | 2017 |
| SSID | ssj0011821 |
| Score | 2.2918782 |
| Snippet | Integration of electronic circuit components onto flexible materials such as plastic foils, paper and textiles is a key challenge for the development of future... |
| SourceID | proquest pubmed |
| SourceType | Aggregation Database Index Database |
| StartPage | 215202 |
| Title | Ultrasonically spray coated silver layers from designed precursor inks for flexible electronics |
| URI | https://www.ncbi.nlm.nih.gov/pubmed/28471754 https://www.proquest.com/docview/1896043055 |
| Volume | 28 |
| WOSCitedRecordID | wos000413074100001&url=https%3A%2F%2Fcvtisr.summon.serialssolutions.com%2F%23%21%2Fsearch%3Fho%3Df%26include.ft.matches%3Dt%26l%3Dnull%26q%3D |
| hasFullText | |
| inHoldings | 1 |
| isFullTextHit | |
| isPrint | |
| link | http://cvtisr.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMwpV1JSwMxFA5qFfTgUre6EcFraGdPTiJi8aClByu9DVlBKDN1UoX-e9-bTq0XQfAyhxkCQ_KWL2_5HiE3joNpNJlgMokti0NlGHdWMItMIRZAv6wDbq9P2WDAx2MxbAJuvimrXNrE2lCbUmOMvBtwpBFBfqrb6TvDqVGYXW1GaKyTVgRQBqU6G6-yCICdm76rgKVJyJs0JShW9_tdV8rURPJ3gFk7mv7ef39xn-w2EJPeLWTigKzZok12fhAPtslWXfip_SHJR5NZJX1Zt0dO5tRPKzmnugQIaqh_w7ppOpGIyyl2olBTV3zAt2mFkXpfVhRTwBSwL3VIrqkmlq5m6_gjMuo_vNw_smboAtNR1psx50xoNI8DITk3iUylNKHjQqlYZmAesLE1gltPBL5PgMIbC6ZbhImUyvR0KsJjslGUhT0lNFJaOwBYqdYGcJ9TPaG0ClIDsA3WBh1yvdzHHIQaMxWysOWHz1c72SEni8PIpwv2jbz2p1kSn_1h9TnZDtEN97CS74K0HKi0vSSb-nP25qurWlrgORg-fwGf-8t5 |
| linkProvider | ProQuest |
| openUrl | ctx_ver=Z39.88-2004&ctx_enc=info%3Aofi%2Fenc%3AUTF-8&rfr_id=info%3Asid%2Fsummon.serialssolutions.com&rft_val_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Ajournal&rft.genre=article&rft.atitle=Ultrasonically+spray+coated+silver+layers+from+designed+precursor+inks+for+flexible+electronics&rft.jtitle=Nanotechnology&rft.au=Marchal%2C+W&rft.au=Vandevenne%2C+G&rft.au=D%27Haen%2C+J&rft.au=Calmont+de+Andrade+Almeida%2C+A&rft.date=2017-05-26&rft.eissn=1361-6528&rft.volume=28&rft.issue=21&rft.spage=215202&rft_id=info:doi/10.1088%2F1361-6528%2Faa6d3a&rft_id=info%3Apmid%2F28471754&rft_id=info%3Apmid%2F28471754&rft.externalDocID=28471754 |
| thumbnail_l | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/lc.gif&issn=1361-6528&client=summon |
| thumbnail_m | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/mc.gif&issn=1361-6528&client=summon |
| thumbnail_s | http://covers-cdn.summon.serialssolutions.com/index.aspx?isbn=/sc.gif&issn=1361-6528&client=summon |