Synthesis and optimization of energy integrated advanced distillation sequences

•Novel effective routes for eco-efficient separation by distillation sequences.•Simultaneous optimization of all design degrees of freedom in distillation sequences.•Optimal arrangement of complex columns sequencing for NGL separation. This paper explores the basis on which reliable screening of dis...

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Veröffentlicht in:Separation and purification technology Jg. 315; S. 123717
Hauptverfasser: Li, Qing, Finn, Adrian J., Doyle, Stephen J., Smith, Robin, Kiss, Anton A.
Format: Journal Article
Sprache:Englisch
Veröffentlicht: Elsevier B.V 15.06.2023
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ISSN:1383-5866, 1873-3794
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Abstract •Novel effective routes for eco-efficient separation by distillation sequences.•Simultaneous optimization of all design degrees of freedom in distillation sequences.•Optimal arrangement of complex columns sequencing for NGL separation. This paper explores the basis on which reliable screening of distillation sequences for energy-efficient separation of zeotropic multicomponent mixtures can be carried out. A case study for the separation of natural gas liquids is used to demonstrate the approach. To solve this generic problem, a screening algorithm has been developed using optimization of a superstructure for sequence synthesis using shortcut models, in conjunction with a transportation algorithm for the synthesis of the heat integration arrangement. Different approaches for the inclusion of heat integration are explored and compared. The best few designs from this screening are then evaluated using rigorous simulation. It has been found that separation problems of the type explored can be screened reliably using shortcut distillation models in conjunction with the synthesis of heat exchanger network designs. Non-integrated designs using thermally coupled complex columns show much better performance than the corresponding designs using simple columns. However, once heat integration is included the difference between designs using complex columns and simple columns narrows significantly.
AbstractList •Novel effective routes for eco-efficient separation by distillation sequences.•Simultaneous optimization of all design degrees of freedom in distillation sequences.•Optimal arrangement of complex columns sequencing for NGL separation. This paper explores the basis on which reliable screening of distillation sequences for energy-efficient separation of zeotropic multicomponent mixtures can be carried out. A case study for the separation of natural gas liquids is used to demonstrate the approach. To solve this generic problem, a screening algorithm has been developed using optimization of a superstructure for sequence synthesis using shortcut models, in conjunction with a transportation algorithm for the synthesis of the heat integration arrangement. Different approaches for the inclusion of heat integration are explored and compared. The best few designs from this screening are then evaluated using rigorous simulation. It has been found that separation problems of the type explored can be screened reliably using shortcut distillation models in conjunction with the synthesis of heat exchanger network designs. Non-integrated designs using thermally coupled complex columns show much better performance than the corresponding designs using simple columns. However, once heat integration is included the difference between designs using complex columns and simple columns narrows significantly.
ArticleNumber 123717
Author Kiss, Anton A.
Finn, Adrian J.
Smith, Robin
Doyle, Stephen J.
Li, Qing
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  fullname: Li, Qing
  organization: Department of Chemical Engineering, Delft University of Technology, Van der Maasweg 9, 2629 HZ Delft, the Netherlands
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  givenname: Adrian J.
  surname: Finn
  fullname: Finn, Adrian J.
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  organization: Centre for Process Integration, Department of Chemical Engineering, The University of Manchester, Sackville Street, Manchester M13 9PL, United Kingdom
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  surname: Smith
  fullname: Smith, Robin
  organization: Centre for Process Integration, Department of Chemical Engineering, The University of Manchester, Sackville Street, Manchester M13 9PL, United Kingdom
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  givenname: Anton A.
  surname: Kiss
  fullname: Kiss, Anton A.
  email: a.a.kiss@tudelft.nl
  organization: Department of Chemical Engineering, Delft University of Technology, Van der Maasweg 9, 2629 HZ Delft, the Netherlands
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Keywords Process design
Energy integration
Distillation sequencing
Process optimization
Process synthesis
Language English
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Snippet •Novel effective routes for eco-efficient separation by distillation sequences.•Simultaneous optimization of all design degrees of freedom in distillation...
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StartPage 123717
SubjectTerms Distillation sequencing
Energy integration
Process design
Process optimization
Process synthesis
Title Synthesis and optimization of energy integrated advanced distillation sequences
URI https://dx.doi.org/10.1016/j.seppur.2023.123717
Volume 315
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