Hypsochromic Shift of Multiple‐Resonance‐Induced Thermally Activated Delayed Fluorescence by Oxygen Atom Incorporation

Herein, we reported an ultrapure blue multiple‐resonance‐induced thermally activated delayed fluorescence (MR‐TADF) material (ν‐DABNA‐O‐Me) with a high photoluminescence quantum yield and a large rate constant for reverse intersystem crossing. Because of restricted π‐conjugation of the HOMO rather t...

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Published in:Angewandte Chemie International Edition Vol. 60; no. 33; pp. 17910 - 17914
Main Authors: Tanaka, Hiroyuki, Oda, Susumu, Ricci, Gaetano, Gotoh, Hajime, Tabata, Keita, Kawasumi, Ryosuke, Beljonne, David, Olivier, Yoann, Hatakeyama, Takuji
Format: Journal Article
Language:English
Published: WEINHEIM Wiley 09.08.2021
Wiley Subscription Services, Inc
Edition:International ed. in English
Subjects:
Chemistry
Chemistry, Multidisciplinary
Conjugation
deep blue
Fluorescence
Incorporation
Molecular orbitals
multiple resonance effect
narrowband emission
organic light-emitting diodes
Oxygen
Photoluminescence
Photons
Physical Sciences
Quantum efficiency
Resonance
Science & Technology
Service life assessment
thermally activated delayed fluorescence
BLUE
OLEDS
EMITTERS
organic light-emitting diodes
SINGLET
LIGHT-EMITTING-DIODES
MOLECULAR DESIGN
thermally activated delayed fluorescence
multiple resonance effect
narrowband emission
deep blue
EMISSION
DERIVATIVES
HIGH-EFFICIENCY
BORYLATION
ISSN:1433-7851, 1521-3773, 1521-3773
Online Access:Get full text
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Abstract Herein, we reported an ultrapure blue multiple‐resonance‐induced thermally activated delayed fluorescence (MR‐TADF) material (ν‐DABNA‐O‐Me) with a high photoluminescence quantum yield and a large rate constant for reverse intersystem crossing. Because of restricted π‐conjugation of the HOMO rather than the LUMO induced by oxygen atom incorporation, ν‐DABNA‐O‐Me shows a hypsochromic shift compared to the parent MR‐TADF material (ν‐DABNA). An organic light‐emitting diode based on this material exhibits an emission at 465 nm, with a small full‐width at half‐maximum of 23 nm and Commission Internationale de l'Eclairage coordinates of (0.13, 0.10), and a high maximum external quantum efficiency of 29.5 %. Moreover, ν‐DABNA‐O‐Me facilitates a drastically improved efficiency roll‐off and a device lifetime compared to ν‐DABNA, which demonstrates significant potential of the oxygen atom incorporation strategy. A multiple‐resonance‐induced thermally activated delayed fluorescence material that comprised oxygen, nitrogen, and boron atoms (ν‐DABNA‐O‐Me) was synthesized via one‐shot double borylation. An OLED device employing the fabricated ν‐DABNA‐O‐Me exhibits deep‐blue electroluminescence with a small full‐width at half‐maximum and a high external quantum efficiency with minimum efficiency roll‐off.
AbstractList Herein, we reported an ultrapure blue multiple‐resonance‐induced thermally activated delayed fluorescence (MR‐TADF) material (ν‐DABNA‐O‐Me) with a high photoluminescence quantum yield and a large rate constant for reverse intersystem crossing. Because of restricted π‐conjugation of the HOMO rather than the LUMO induced by oxygen atom incorporation, ν‐DABNA‐O‐Me shows a hypsochromic shift compared to the parent MR‐TADF material (ν‐DABNA). An organic light‐emitting diode based on this material exhibits an emission at 465 nm, with a small full‐width at half‐maximum of 23 nm and Commission Internationale de l'Eclairage coordinates of (0.13, 0.10), and a high maximum external quantum efficiency of 29.5 %. Moreover, ν‐DABNA‐O‐Me facilitates a drastically improved efficiency roll‐off and a device lifetime compared to ν‐DABNA, which demonstrates significant potential of the oxygen atom incorporation strategy.
Herein, we reported an ultrapure blue multiple‐resonance‐induced thermally activated delayed fluorescence (MR‐TADF) material (ν‐DABNA‐O‐Me) with a high photoluminescence quantum yield and a large rate constant for reverse intersystem crossing. Because of restricted π‐conjugation of the HOMO rather than the LUMO induced by oxygen atom incorporation, ν‐DABNA‐O‐Me shows a hypsochromic shift compared to the parent MR‐TADF material (ν‐DABNA). An organic light‐emitting diode based on this material exhibits an emission at 465 nm, with a small full‐width at half‐maximum of 23 nm and Commission Internationale de l'Eclairage coordinates of (0.13, 0.10), and a high maximum external quantum efficiency of 29.5 %. Moreover, ν‐DABNA‐O‐Me facilitates a drastically improved efficiency roll‐off and a device lifetime compared to ν‐DABNA, which demonstrates significant potential of the oxygen atom incorporation strategy. A multiple‐resonance‐induced thermally activated delayed fluorescence material that comprised oxygen, nitrogen, and boron atoms (ν‐DABNA‐O‐Me) was synthesized via one‐shot double borylation. An OLED device employing the fabricated ν‐DABNA‐O‐Me exhibits deep‐blue electroluminescence with a small full‐width at half‐maximum and a high external quantum efficiency with minimum efficiency roll‐off.
Herein, we reported an ultrapure blue multiple‐resonance‐induced thermally activated delayed fluorescence (MR‐TADF) material ( ν‐DABNA‐O‐Me ) with a high photoluminescence quantum yield and a large rate constant for reverse intersystem crossing. Because of restricted π‐conjugation of the HOMO rather than the LUMO induced by oxygen atom incorporation, ν‐DABNA‐O‐Me shows a hypsochromic shift compared to the parent MR‐TADF material ( ν‐DABNA ). An organic light‐emitting diode based on this material exhibits an emission at 465 nm, with a small full‐width at half‐maximum of 23 nm and Commission Internationale de l'Eclairage coordinates of (0.13, 0.10), and a high maximum external quantum efficiency of 29.5 %. Moreover, ν‐DABNA‐O‐Me facilitates a drastically improved efficiency roll‐off and a device lifetime compared to ν‐DABNA , which demonstrates significant potential of the oxygen atom incorporation strategy.
Herein, we reported an ultrapure blue multiple-resonance-induced thermally activated delayed fluorescence (MR-TADF) material (ν-DABNA-O-Me) with a high photoluminescence quantum yield and a large rate constant for reverse intersystem crossing. Because of restricted π-conjugation of the HOMO rather than the LUMO induced by oxygen atom incorporation, ν-DABNA-O-Me shows a hypsochromic shift compared to the parent MR-TADF material (ν-DABNA). An organic light-emitting diode based on this material exhibits an emission at 465 nm, with a small full-width at half-maximum of 23 nm and Commission Internationale de l'Eclairage coordinates of (0.13, 0.10), and a high maximum external quantum efficiency of 29.5 %. Moreover, ν-DABNA-O-Me facilitates a drastically improved efficiency roll-off and a device lifetime compared to ν-DABNA, which demonstrates significant potential of the oxygen atom incorporation strategy.Herein, we reported an ultrapure blue multiple-resonance-induced thermally activated delayed fluorescence (MR-TADF) material (ν-DABNA-O-Me) with a high photoluminescence quantum yield and a large rate constant for reverse intersystem crossing. Because of restricted π-conjugation of the HOMO rather than the LUMO induced by oxygen atom incorporation, ν-DABNA-O-Me shows a hypsochromic shift compared to the parent MR-TADF material (ν-DABNA). An organic light-emitting diode based on this material exhibits an emission at 465 nm, with a small full-width at half-maximum of 23 nm and Commission Internationale de l'Eclairage coordinates of (0.13, 0.10), and a high maximum external quantum efficiency of 29.5 %. Moreover, ν-DABNA-O-Me facilitates a drastically improved efficiency roll-off and a device lifetime compared to ν-DABNA, which demonstrates significant potential of the oxygen atom incorporation strategy.
Herein, we reported an ultrapure blue multiple-resonance-induced thermally activated delayed fluorescence (MR-TADF) material (nu-DABNA-O-Me) with a high photoluminescence quantum yield and a large rate constant for reverse intersystem crossing. Because of restricted pi-conjugation of the HOMO rather than the LUMO induced by oxygen atom incorporation, nu-DABNA-O-Me shows a hypsochromic shift compared to the parent MR-TADF material (nu-DABNA). An organic light-emitting diode based on this material exhibits an emission at 465 nm, with a small full-width at half-maximum of 23 nm and Commission Internationale de l'Eclairage coordinates of (0.13, 0.10), and a high maximum external quantum efficiency of 29.5 %. Moreover, nu-DABNA-O-Me facilitates a drastically improved efficiency roll-off and a device lifetime compared to nu-DABNA, which demonstrates significant potential of the oxygen atom incorporation strategy.
Author Olivier, Yoann
Kawasumi, Ryosuke
Hatakeyama, Takuji
Tanaka, Hiroyuki
Oda, Susumu
Ricci, Gaetano
Gotoh, Hajime
Beljonne, David
Tabata, Keita
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  surname: Tanaka
  fullname: Tanaka, Hiroyuki
  organization: JNC Petrochemical Corporation
– sequence: 2
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  orcidid: 0000-0003-1088-1932
  surname: Oda
  fullname: Oda, Susumu
  organization: Kwansei Gakuin University
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  givenname: Gaetano
  surname: Ricci
  fullname: Ricci, Gaetano
  organization: Université de Namur
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  givenname: Hajime
  surname: Gotoh
  fullname: Gotoh, Hajime
  organization: Kwansei Gakuin University
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  givenname: Keita
  surname: Tabata
  fullname: Tabata, Keita
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  fullname: Kawasumi, Ryosuke
  organization: JNC Petrochemical Corporation
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  fullname: Beljonne, David
  organization: Université de Mons
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  givenname: Yoann
  orcidid: 0000-0003-2193-1536
  surname: Olivier
  fullname: Olivier, Yoann
  organization: Université de Namur
– sequence: 9
  givenname: Takuji
  orcidid: 0000-0002-7483-9525
  surname: Hatakeyama
  fullname: Hatakeyama, Takuji
  email: hatake@kwansei.ac.jp
  organization: Kwansei Gakuin University
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Issue 33
Keywords BLUE
OLEDS
EMITTERS
organic light-emitting diodes
SINGLET
LIGHT-EMITTING-DIODES
MOLECULAR DESIGN
thermally activated delayed fluorescence
multiple resonance effect
narrowband emission
deep blue
EMISSION
DERIVATIVES
HIGH-EFFICIENCY
BORYLATION
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Snippet Herein, we reported an ultrapure blue multiple‐resonance‐induced thermally activated delayed fluorescence (MR‐TADF) material (ν‐DABNA‐O‐Me) with a high...
Herein, we reported an ultrapure blue multiple‐resonance‐induced thermally activated delayed fluorescence (MR‐TADF) material ( ν‐DABNA‐O‐Me ) with a high...
Herein, we reported an ultrapure blue multiple-resonance-induced thermally activated delayed fluorescence (MR-TADF) material (nu-DABNA-O-Me) with a high...
Herein, we reported an ultrapure blue multiple-resonance-induced thermally activated delayed fluorescence (MR-TADF) material (ν-DABNA-O-Me) with a high...
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SubjectTerms Chemistry
Chemistry, Multidisciplinary
Conjugation
deep blue
Fluorescence
Incorporation
Molecular orbitals
multiple resonance effect
narrowband emission
organic light-emitting diodes
Oxygen
Photoluminescence
Photons
Physical Sciences
Quantum efficiency
Resonance
Science & Technology
Service life assessment
thermally activated delayed fluorescence
Title Hypsochromic Shift of Multiple‐Resonance‐Induced Thermally Activated Delayed Fluorescence by Oxygen Atom Incorporation
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.202105032
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https://www.proquest.com/docview/2533317615
Volume 60
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