Largely enhanced dielectric properties of polymer composites with HfO2 nanoparticles for high-temperature film capacitors

Polymer dielectrics are preferred materials for high-energy-density capacitive energy storage. In particular, high-temperature dielectrics that can withstand harsh conditions, e.g., ≥150 °C, is of crucial importance for advanced electronics and electrical power systems. Herein, high-temperature diel...

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Published in:	Composites science and technology Vol. 201; p. 108528
Main Authors:	Ren, Lulu, Yang, Lijun, Zhang, Siyu, Li, He, Zhou, Yao, Ai, Ding, Xie, Zongliang, Zhao, Xuetong, Peng, Zongren, Liao, Ruijin, Wang, Qing
Format:	Journal Article
Language:	English
Published:	Barking Elsevier Ltd 05.01.2021 Elsevier BV
Subjects:	Dielectric properties Dielectrics Electric power systems Energy storage Flux density Hafnium oxide Hafnium oxide nanoparticles High temperature Leakage current Nanocomposites Nanoparticles Permittivity Polyetherimides Polymer matrix composites Polymer nanocomposites Polymers High temperature Hafnium oxide nanoparticles Dielectric properties Polymer nanocomposites Energy storage
ISSN:	0266-3538, 1879-1050
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Abstract	Polymer dielectrics are preferred materials for high-energy-density capacitive energy storage. In particular, high-temperature dielectrics that can withstand harsh conditions, e.g., ≥150 °C, is of crucial importance for advanced electronics and electrical power systems. Herein, high-temperature dielectric polymer composites composed of polyetherimide (PEI) matrix and hafnium oxide (HfO2) nanoparticles are presented. It is found that the incorporation of HfO2 with a moderate dielectric constant and a wide bandgap improves the dielectric constant and simultaneously reduces the high-field leakage current density of the PEI nanocomposites. As a result, the PEI/HfO2 composites exhibit superior energy storage performance to the current high-temperature engineering polymers at elevated temperatures. Specifically, the nanocomposite with 3 vol% HfO2 displays a discharged energy density of 2.82 J/cm3 at 150 °C, which is 77% higher than neat PEI. This work demonstrates the effectiveness of incorporation of the nanofiller with a medium dielectric constant into the polymer on the improvement of high-temperature capacitive properties of the polymer composites. [Display omitted]
AbstractList	Polymer dielectrics are preferred materials for high-energy-density capacitive energy storage. In particular, high-temperature dielectrics that can withstand harsh conditions, e.g., ≥150 °C, is of crucial importance for advanced electronics and electrical power systems. Herein, high-temperature dielectric polymer composites composed of polyetherimide (PEI) matrix and hafnium oxide (HfO2) nanoparticles are presented. It is found that the incorporation of HfO2 with a moderate dielectric constant and a wide bandgap improves the dielectric constant and simultaneously reduces the high-field leakage current density of the PEI nanocomposites. As a result, the PEI/HfO2 composites exhibit superior energy storage performance to the current high-temperature engineering polymers at elevated temperatures. Specifically, the nanocomposite with 3 vol% HfO2 displays a discharged energy density of 2.82 J/cm3 at 150 °C, which is 77% higher than neat PEI. This work demonstrates the effectiveness of incorporation of the nanofiller with a medium dielectric constant into the polymer on the improvement of high-temperature capacitive properties of the polymer composites. Polymer dielectrics are preferred materials for high-energy-density capacitive energy storage. In particular, high-temperature dielectrics that can withstand harsh conditions, e.g., ≥150 °C, is of crucial importance for advanced electronics and electrical power systems. Herein, high-temperature dielectric polymer composites composed of polyetherimide (PEI) matrix and hafnium oxide (HfO2) nanoparticles are presented. It is found that the incorporation of HfO2 with a moderate dielectric constant and a wide bandgap improves the dielectric constant and simultaneously reduces the high-field leakage current density of the PEI nanocomposites. As a result, the PEI/HfO2 composites exhibit superior energy storage performance to the current high-temperature engineering polymers at elevated temperatures. Specifically, the nanocomposite with 3 vol% HfO2 displays a discharged energy density of 2.82 J/cm3 at 150 °C, which is 77% higher than neat PEI. This work demonstrates the effectiveness of incorporation of the nanofiller with a medium dielectric constant into the polymer on the improvement of high-temperature capacitive properties of the polymer composites. [Display omitted]
ArticleNumber	108528
Author	Zhou, Yao Peng, Zongren Li, He Xie, Zongliang Yang, Lijun Zhao, Xuetong Ai, Ding Liao, Ruijin Ren, Lulu Wang, Qing Zhang, Siyu
Author_xml	– sequence: 1 givenname: Lulu surname: Ren fullname: Ren, Lulu organization: State Key Laboratory of Power Transmission Equipment & System Security and New Technology, Chongqing University, Chongqing, 400044, China – sequence: 2 givenname: Lijun surname: Yang fullname: Yang, Lijun organization: State Key Laboratory of Power Transmission Equipment & System Security and New Technology, Chongqing University, Chongqing, 400044, China – sequence: 3 givenname: Siyu surname: Zhang fullname: Zhang, Siyu organization: State Key Laboratory of Electrical Insulation and Power Equipment, Xi'an Jiaotong University, Xi'an, Shaanxi, 710049, China – sequence: 4 givenname: He orcidid: 0000-0002-4076-7279 surname: Li fullname: Li, He organization: Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA, 16802, USA – sequence: 5 givenname: Yao surname: Zhou fullname: Zhou, Yao organization: Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA, 16802, USA – sequence: 6 givenname: Ding surname: Ai fullname: Ai, Ding organization: Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA, 16802, USA – sequence: 7 givenname: Zongliang orcidid: 0000-0001-5965-332X surname: Xie fullname: Xie, Zongliang organization: State Key Laboratory of Electrical Insulation and Power Equipment, Xi'an Jiaotong University, Xi'an, Shaanxi, 710049, China – sequence: 8 givenname: Xuetong surname: Zhao fullname: Zhao, Xuetong email: zxt201314@cqu.edu.cn organization: State Key Laboratory of Power Transmission Equipment & System Security and New Technology, Chongqing University, Chongqing, 400044, China – sequence: 9 givenname: Zongren surname: Peng fullname: Peng, Zongren organization: State Key Laboratory of Electrical Insulation and Power Equipment, Xi'an Jiaotong University, Xi'an, Shaanxi, 710049, China – sequence: 10 givenname: Ruijin surname: Liao fullname: Liao, Ruijin organization: State Key Laboratory of Power Transmission Equipment & System Security and New Technology, Chongqing University, Chongqing, 400044, China – sequence: 11 givenname: Qing surname: Wang fullname: Wang, Qing email: wang@matse.psu.edu organization: Department of Materials Science and Engineering, The Pennsylvania State University, University Park, PA, 16802, USA
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Snippet	Polymer dielectrics are preferred materials for high-energy-density capacitive energy storage. In particular, high-temperature dielectrics that can withstand...
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SubjectTerms	Dielectric properties Dielectrics Electric power systems Energy storage Flux density Hafnium oxide Hafnium oxide nanoparticles High temperature Leakage current Nanocomposites Nanoparticles Permittivity Polyetherimides Polymer matrix composites Polymer nanocomposites Polymers
Title	Largely enhanced dielectric properties of polymer composites with HfO2 nanoparticles for high-temperature film capacitors
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