Photochemical degradation of nitrated PAHs in snow
Nitrated polycyclic aromatic hydrocarbons (NPAHs) are derived from PAHs, which are ubiquitous in the aqueous and atmospheric environments, and whose mutagenicity and carcinogenicity are much higher than that of PAHs. Therefore, their environmental transformation has attracted a lot of attention. In...
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| Vydané v: | Atmospheric environment (1994) Ročník 199; s. 260 - 264 |
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| Jazyk: | English |
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Elsevier Ltd
15.02.2019
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| ISSN: | 1352-2310, 1873-2844 |
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| Abstract | Nitrated polycyclic aromatic hydrocarbons (NPAHs) are derived from PAHs, which are ubiquitous in the aqueous and atmospheric environments, and whose mutagenicity and carcinogenicity are much higher than that of PAHs. Therefore, their environmental transformation has attracted a lot of attention. In the present study, direct and indirect UV photodegradation kinetics of two NPAHs (1-nitropyrene and 1,8-dinitropyrene) in snow were investigated. It was found that the kinetics followed the pseudo-first-order kinetics with the photochemical degradation rate 0.3773 h−1 for 48.98 nM 1-NP and 0.3653 h−1 for 41.00 nM 1,8-DNP. Photosensitizers (hydrogen peroxide and nitrate) promoted the photodegradation of NPAHs. Considering the lower temperature and less microorganisms in snow environment, the photodegradation can be a key factor in determining the fate of NPAHs in sunlit surface snow. To the best of our knowledge, this is the first report on the photodegradation of NPAHs in snow.
•It is first reported on photochemical behaviour of two NPAHs in snow.•Similar photochemical degradation rates were observed for 1-NP and 1,8-DNP in snow.•The promotion effect of hydrogen peroxide on the photodegradation of NPAHs was greater than that of nitrate. |
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| AbstractList | Nitrated polycyclic aromatic hydrocarbons (NPAHs) are derived from PAHs, which are ubiquitous in the aqueous and atmospheric environments, and whose mutagenicity and carcinogenicity are much higher than that of PAHs. Therefore, their environmental transformation has attracted a lot of attention. In the present study, direct and indirect UV photodegradation kinetics of two NPAHs (1-nitropyrene and 1,8-dinitropyrene) in snow were investigated. It was found that the kinetics followed the pseudo-first-order kinetics with the photochemical degradation rate 0.3773 h−1 for 48.98 nM 1-NP and 0.3653 h−1 for 41.00 nM 1,8-DNP. Photosensitizers (hydrogen peroxide and nitrate) promoted the photodegradation of NPAHs. Considering the lower temperature and less microorganisms in snow environment, the photodegradation can be a key factor in determining the fate of NPAHs in sunlit surface snow. To the best of our knowledge, this is the first report on the photodegradation of NPAHs in snow.
•It is first reported on photochemical behaviour of two NPAHs in snow.•Similar photochemical degradation rates were observed for 1-NP and 1,8-DNP in snow.•The promotion effect of hydrogen peroxide on the photodegradation of NPAHs was greater than that of nitrate. Nitrated polycyclic aromatic hydrocarbons (NPAHs) are derived from PAHs, which are ubiquitous in the aqueous and atmospheric environments, and whose mutagenicity and carcinogenicity are much higher than that of PAHs. Therefore, their environmental transformation has attracted a lot of attention. In the present study, direct and indirect UV photodegradation kinetics of two NPAHs (1-nitropyrene and 1,8-dinitropyrene) in snow were investigated. It was found that the kinetics followed the pseudo-first-order kinetics with the photochemical degradation rate 0.3773 h−1 for 48.98 nM 1-NP and 0.3653 h−1 for 41.00 nM 1,8-DNP. Photosensitizers (hydrogen peroxide and nitrate) promoted the photodegradation of NPAHs. Considering the lower temperature and less microorganisms in snow environment, the photodegradation can be a key factor in determining the fate of NPAHs in sunlit surface snow. To the best of our knowledge, this is the first report on the photodegradation of NPAHs in snow. |
| Author | Wang, Ying Zheng, Na Kang, Chunli Xue, Honghai Wang, Yuwei |
| Author_xml | – sequence: 1 givenname: Honghai orcidid: 0000-0003-0476-4000 surname: Xue fullname: Xue, Honghai organization: Key Laboratory of Songliao Aquatic Environment (Jilin Jianzhu University), Ministry of Education, Changchun, 130118, China – sequence: 2 givenname: Na orcidid: 0000-0003-0947-5240 surname: Zheng fullname: Zheng, Na organization: Key Laboratory of Groundwater Resources and Environment (Jilin University), Ministry of Education, Changchun, 130021, China – sequence: 3 givenname: Chunli surname: Kang fullname: Kang, Chunli email: kangcl@jlu.edu.cn organization: Key Laboratory of Groundwater Resources and Environment (Jilin University), Ministry of Education, Changchun, 130021, China – sequence: 4 givenname: Ying surname: Wang fullname: Wang, Ying organization: Key Laboratory of Songliao Aquatic Environment (Jilin Jianzhu University), Ministry of Education, Changchun, 130118, China – sequence: 5 givenname: Yuwei surname: Wang fullname: Wang, Yuwei organization: Key Laboratory of Songliao Aquatic Environment (Jilin Jianzhu University), Ministry of Education, Changchun, 130118, China |
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| CitedBy_id | crossref_primary_10_1016_j_jclepro_2021_130026 crossref_primary_10_1002_adsu_202100027 crossref_primary_10_1080_10406638_2019_1695218 crossref_primary_10_1080_10643389_2020_1748486 crossref_primary_10_1016_j_envres_2025_121749 |
| Cites_doi | 10.1016/j.chemosphere.2016.04.087 10.1021/es0714686 10.1080/10406630600760576 10.1080/00039896.1994.9937459 10.1016/j.jphotochem.2006.06.039 10.1007/BF01267771 10.5194/acp-7-4329-2007 10.1021/jp909205e 10.1016/j.atmosenv.2006.12.011 10.1016/j.scitotenv.2012.11.055 10.1021/jp108652p 10.1021/es990834l 10.1016/S1352-2310(02)00252-2 10.1016/j.atmosenv.2009.01.044 10.1002/recl.19871060403 10.1021/jp803051x 10.1016/j.atmosenv.2013.04.035 10.1021/es961067i 10.1016/j.atmosenv.2007.03.056 10.1080/03067310108044388 10.1016/j.jphotochem.2016.08.018 10.1007/s10311-009-0221-2 10.1016/S0304-3894(02)00120-6 10.1021/es1042172 10.2174/1385272821666171116161755 10.1002/adic.200590066 |
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| SubjectTerms | atmospheric chemistry carcinogenicity hydrogen peroxide Kinetics microorganisms mutagenicity Nitrated PAHs nitrates photolysis photosensitizing agents polycyclic aromatic hydrocarbons snow Snow photochemistry temperature |
| Title | Photochemical degradation of nitrated PAHs in snow |
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