Anthropogenic Air Pollution Delays Marine Stratocumulus Breakup to Open Cells
Marine stratocumulus cloud (Sc) decks with high cloud fraction typically breakup when sufficient drizzle forms. Cloud breakup leads to a lower cloud radiative effect due to the lower cloud amount. Here we use realistic Lagrangian large eddy simulations along a 3‐day trajectory, evaluated with satell...
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| Vydáno v: | Geophysical research letters Ročník 46; číslo 23; s. 14135 - 14144 |
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| Hlavní autoři: | , , , , |
| Médium: | Journal Article |
| Jazyk: | angličtina |
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Washington
John Wiley & Sons, Inc
16.12.2019
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| ISSN: | 0094-8276, 1944-8007 |
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| Abstract | Marine stratocumulus cloud (Sc) decks with high cloud fraction typically breakup when sufficient drizzle forms. Cloud breakup leads to a lower cloud radiative effect due to the lower cloud amount. Here we use realistic Lagrangian large eddy simulations along a 3‐day trajectory, evaluated with satellite observations, to investigate the timing of Sc breakup in response to aerosol conditions. We show that the timing of the breakup is strongly modulated by the diurnal cycle and large‐scale meteorology but varies systematically with the initial aerosol concentration: the more polluted the clouds, the later the breakup. This indicates that the cloud radiative effect via cloud cover adjustments is not saturated, in contrast to the effect of aerosol on cloud albedo at fixed cloudiness, which weakens with increasing aerosol levels. The results also show that the cloud radiative impact of anthropogenic aerosol is strongest far from its origin over land.
Key Points
Marine stratocumulus cloud breakup time is systematically delayed with increasing initial background aerosol concentration
Cloud cover response to aerosol is not saturated, in contrast to the effect of aerosol on cloud albedo at fixed cloudiness
Realistic Lagrangian large eddy simulations identify the roles of both aerosol and meteorology in determining cloud breakup time |
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| AbstractList | Marine stratocumulus cloud (Sc) decks with high cloud fraction typically breakup when sufficient drizzle forms. Cloud breakup leads to a lower cloud radiative effect due to the lower cloud amount. Here we use realistic Lagrangian large eddy simulations along a 3‐day trajectory, evaluated with satellite observations, to investigate the timing of Sc breakup in response to aerosol conditions. We show that the timing of the breakup is strongly modulated by the diurnal cycle and large‐scale meteorology but varies systematically with the initial aerosol concentration: the more polluted the clouds, the later the breakup. This indicates that the cloud radiative effect via cloud cover adjustments is not saturated, in contrast to the effect of aerosol on cloud albedo at fixed cloudiness, which weakens with increasing aerosol levels. The results also show that the cloud radiative impact of anthropogenic aerosol is strongest far from its origin over land. Marine stratocumulus cloud (Sc) decks with high cloud fraction typically breakup when sufficient drizzle forms. Cloud breakup leads to a lower cloud radiative effect due to the lower cloud amount. Here we use realistic Lagrangian large eddy simulations along a 3‐day trajectory, evaluated with satellite observations, to investigate the timing of Sc breakup in response to aerosol conditions. We show that the timing of the breakup is strongly modulated by the diurnal cycle and large‐scale meteorology but varies systematically with the initial aerosol concentration: the more polluted the clouds, the later the breakup. This indicates that the cloud radiative effect via cloud cover adjustments is not saturated, in contrast to the effect of aerosol on cloud albedo at fixed cloudiness, which weakens with increasing aerosol levels. The results also show that the cloud radiative impact of anthropogenic aerosol is strongest far from its origin over land. Key Points Marine stratocumulus cloud breakup time is systematically delayed with increasing initial background aerosol concentration Cloud cover response to aerosol is not saturated, in contrast to the effect of aerosol on cloud albedo at fixed cloudiness Realistic Lagrangian large eddy simulations identify the roles of both aerosol and meteorology in determining cloud breakup time Marine stratocumulus cloud (Sc) decks with high cloud fraction typically breakup when sufficient drizzle forms. Cloud breakup leads to a lower cloud radiative effect due to the lower cloud amount. Here we use realistic Lagrangian large eddy simulations along a 3‐day trajectory, evaluated with satellite observations, to investigate the timing of Sc breakup in response to aerosol conditions. We show that the timing of the breakup is strongly modulated by the diurnal cycle and large‐scale meteorology but varies systematically with the initial aerosol concentration: the more polluted the clouds, the later the breakup. This indicates that the cloud radiative effect via cloud cover adjustments is not saturated, in contrast to the effect of aerosol on cloud albedo at fixed cloudiness, which weakens with increasing aerosol levels. The results also show that the cloud radiative impact of anthropogenic aerosol is strongest far from its origin over land. Marine stratocumulus cloud breakup time is systematically delayed with increasing initial background aerosol concentration Cloud cover response to aerosol is not saturated, in contrast to the effect of aerosol on cloud albedo at fixed cloudiness Realistic Lagrangian large eddy simulations identify the roles of both aerosol and meteorology in determining cloud breakup time |
| Author | Kazil, Jan Yamaguchi, Takanobu Goren, Tom Hoffmann, Fabian Feingold, Graham |
| Author_xml | – sequence: 1 givenname: Tom orcidid: 0000-0001-5618-9402 surname: Goren fullname: Goren, Tom email: tom.goren@noaa.gov organization: NOAA Earth System Research Laboratory – sequence: 2 givenname: Jan orcidid: 0000-0003-3271-2451 surname: Kazil fullname: Kazil, Jan organization: NOAA Earth System Research Laboratory – sequence: 3 givenname: Fabian orcidid: 0000-0001-5136-0653 surname: Hoffmann fullname: Hoffmann, Fabian organization: NOAA Earth System Research Laboratory – sequence: 4 givenname: Takanobu orcidid: 0000-0001-8059-0757 surname: Yamaguchi fullname: Yamaguchi, Takanobu organization: NOAA Earth System Research Laboratory – sequence: 5 givenname: Graham orcidid: 0000-0002-0774-2926 surname: Feingold fullname: Feingold, Graham organization: NOAA Earth System Research Laboratory |
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| Snippet | Marine stratocumulus cloud (Sc) decks with high cloud fraction typically breakup when sufficient drizzle forms. Cloud breakup leads to a lower cloud radiative... |
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| SubjectTerms | Aerosol concentrations Aerosol effects Aerosols Aerosol‐cloud interaction Air pollution Albedo Anthropogenic air‐pollution Anthropogenic factors Breakup Cloud albedo Cloud amount Cloud cover Cloud transitions Cloudiness Clouds Decks Diurnal Diurnal cycle Diurnal variations Drizzle Human influences Large eddy simulation Large eddy simulations Marine pollution Marine stratocumulus clouds Meteorology Radiative forcing Satellite observation Stratocumulus clouds Trajectory analysis |
| Title | Anthropogenic Air Pollution Delays Marine Stratocumulus Breakup to Open Cells |
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